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Register a new userUltracold chemical reactions of a single Rydberg atom in a dense gas
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Added by
Michael Schlagm\\\"uller
Publication date
2016
fields
Physics
and research's language is
English
Authors
Michael Schlagmuller
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Within a dense environment ($rho approx 10^{14},$atoms/cm$^3$) at ultracold temperatures ($T < 1,mu{}text{K}$), a single atom excited to a Rydberg state acts as a reaction center for surrounding neutral atoms. At these temperatures almost all neutral atoms within the Rydberg orbit are bound to the Rydberg core and interact with the Rydberg atom. We have studied the reaction rate and products for $nS$ $^{87}$Rb Rydberg states and we mainly observe a state change of the Rydberg electron to a high orbital angular momentum $l$, with the released energy being converted into kinetic energy of the Rydberg atom. Unexpectedly, the measurements show a threshold behavior at $napprox 100$ for the inelastic collision time leading to increased lifetimes of the Rydberg state independent of the densities investigated. Even at very high densities ($rhoapprox4.8times 10^{14},text{cm}^{-3}$), the lifetime of a Rydberg atom exceeds $10,mutext{s}$ at $n > 140$ compared to $1,mutext{s}$ at $n=90$. In addition, a second observed reaction mechanism, namely Rb$_2^+$ molecule formation, was studied. Both reaction products are equally probable for $n=40$ but the fraction of Rb$_2^+$ created drops to below 10$,$% for $nge90$.
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