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Direct Measurement of the Mass Difference of Ho163 and Dy163 Solves the Q-Value Puzzle for the Neutrino Mass Determination

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 Added by Sergey Eliseev
 Publication date 2016
  fields Physics
and research's language is English




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The atomic mass difference of 163Ho and 163Dy has been directly measured with the Penning trap mass spectrometer SHIPTRAP applying the novel phase imaging ion cyclotron resonance technique. Our measurement has solved the long standing problem of large discrepancies in the Q value of the electron capture in 163Ho determined by different techniques. Our measured mass difference shifts the current Q value of 2555(16) eV evaluated in the Atomic Mass Evaluation 2012 [G. Audi et al., Chin. Phys. C 36, 1157 (2012)] by more than 7 sigma to 2833(30stat)(15sys) eV/c2. With the new mass difference it will be possible, e.g., to reach in the first phase of the ECHo experiment a statistical sensitivity to the neutrino mass below 10 eV, which will reduce its present upper limit by more than an order of magnitude.



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For the first time a direct determination of the atomic mass difference of 187Re and 187Os has been performed with the Penning-trap mass spectrometer SHIPTRAP applying the novel phase-imaging ion-cyclotron-resonance technique. The obtained value of 2492(30stat)(15sys) eV is in excellent agreement with the Q values determined indirectly with microcalorimetry and thus resolves a long-standing discrepancy with older proportional counter measurements. This is essential for the determination of the neutrino mass from the beta-decay of 187Re as planned in future microcalorimetric measurements. In addition, an accurate mass difference of 187Re and 187Os is also important for the assessment of 187Re for cosmochronology.
Background: The understanding and description of forbidden decays provides interesting challenges for nuclear theory. These calculations could help to test underlying nuclear models and interpret experimental data. Purpose: Compare a direct measurement of the $^{138}$La $beta$-decay $Q$ value with the $beta$-decay spectrum end-point energy measured by Quarati et al. using LaBr$_3$ detectors [Appl. Radiat. Isot. 108, 30 (2016)]. Use new precise measurements of the $^{138}$La $beta$-decay and electron capture (EC) $Q$ values to improve theoretical calculations of the $beta$-decay spectrum and EC probabilities. Method: High-precision Penning trap mass spectrometry was used to measure cyclotron frequency ratios of $^{138}$La, $^{138}$Ce and $^{138}$Ba ions from which $beta$-decay and EC $Q$ values for $^{138}$La were obtained. Results: The $^{138}$La $beta$-decay and EC $Q$ values were measured to be $Q$ = 1052.42(41) keV and $Q_{EC}$ = 1748.41(34) keV, improving the precision compared to the values obtained in the most recent atomic mass evaluation [Wang, et al., Chin. Phys. C 41, 030003 (2017)] by an order of magnitude. These results are used for improved calculations of the $^{138}$La $beta$-decay shape factor and EC probabilities. New determinations for the $^{138}$Ce 2EC $Q$ value and the atomic masses of $^{138}$La, $^{138}$Ce, and $^{138}$Ba are also reported. Conclusion: The $^{138}$La $beta$-decay $Q$ value measured by Quarati et al. is in excellent agreement with our new result, which is an order of magnitude more precise. Uncertainties in the shape factor calculations for $^{138}$La beta-decay using our new $Q$ value are reduced by an order of magnitude. Uncertainties in the EC probability ratios are also reduced and show improved agreement with experimental data.
In this contribution we review the status and perspectives of direct neutrino mass experiments. These experiments investigate the kinematics of $beta$-decays of specific isotopes ($^3$H, $^{187}$Re, $^{163}$Ho) to derive model-independent information on the averaged electron (anti-) neutrino mass, which is formed by the incoherent sum of the neutrino mass eigenstates contributing to the electron neutrino. We first review the kinematics of $beta$-decay and the determination of the neutrino mass, before giving a brief overview of past neutrino mass measurements (SN1987a-ToF studies, Mainz and Troitsk experiments for $^3$H, cryo-bolometers for $^{187}$Re). We then describe the Karlsruhe Tritium Neutrino (KATRIN) experiment which is currently under construction at Karlsruhe Institute of Technology. The large-scale setup will use the MAC-E-Filter principle pioneered earlier to push the sensitivity down to a value of 200 meV(90% C.L.). KATRIN faces many technological challenges that have to be resolved with regard to source intensity and stability, as well as precision energy analysis and low background rate close to the kinematic endpoint of tritium $beta$-decay at 18.6 keV. We then review new experimental approaches such as the MARE, ECHO and Project8 experiments, which offer the promise to perform an independent measurement of the neutrino mass in the sub-eV region. This variety of methods and the novel technologies developed in all present and future experiments demonstrate the great potential of direct neutrino mass experiments in providing vital information on the absolute mass scale of neutrinos.
The European Research Council has recently funded HOLMES, a project with the aim of performing a calorimetric measurement of the electron neutrino mass measuring the energy released in the electron capture decay of 163Ho. The baseline for HOLMES are microcalorimeters coupled to Transition Edge Sensors (TESs) read out with rf-SQUIDs, for microwave multiplexing purposes. A promising alternative solution is based on superconducting microwave resonators, that have undergone rapid development in the last decade. These detectors, called Microwave Kinetic Inductance Detectors (MKIDs), are inherently multiplexed in the frequency domain and suitable for even larger-scale pixel arrays, with theoretical high energy resolution and fast response. The aim of our activity is to develop arrays of microresonator detectors for X-ray spectroscopy and suitable for the calorimetric measurement of the energy spectra of 163Ho. Superconductive multilayer films composed by a sequence of pure Titanium and stoichiometric TiN layers show many ideal properties for MKIDs, such as low loss, large sheet resistance, large kinetic inductance, and tunable critical temperature $T_c$. We developed Ti/TiN multilayer microresonators with $T_c$ within the range from 70 mK to 4.5 K and with good uniformity. In this contribution we present the design solutions adopted, the fabrication processes and the characterization results.
The HOLMES experiment will perform a precise calorimetric measurement of the end point of the Electron Capture (EC) decay spectrum of 163Ho in order to extract information on neutrino mass with a sensitivity below 2 eV. In its final configuration, HOLMES will deploy 1000 detectors of low-temperature microcalorimeters with implanted 163Ho nuclei. The baseline sensors for HOLMES are Mo/Cu TESs (Transition Edge Sensors) on SiNx membrane with gold absorbers. Considering the large number of pixels and an event rate of about 300 Hz/pixel, a large multiplexing factor and a large bandwidth are needed. To fulfill this requirement, HOLMES will exploit recent advances in microwave multiplexing. In this contribution, we present the status of the activities in development, the performances of the developed microwave-multiplexed readout system, and the results obtained with the detectors specifically designed for HOLMES in terms of noise, time, and energy resolutions
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