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Register a new userHigh resolution transient and permanent spectral hole burning in Ce$^{3+}$:Y$_2$SiO$_5$ at liquid helium temperatures
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We perform hole burning with a low drift stabilized laser within the zero phonon line of the 4f-5d transition in Ce$^{3+}$:Y$_2$SiO$_5$ at 2K. The narrowest spectral holes appear for small applied magnetic fields and are $6pm4$ MHz wide (FWHM). This puts an upper bound on the homogeneous linewidth of the transition to $3pm2$ MHz, which is close to lifetime limited. The spin level relaxation time is measured to $72pm21$ ms with a magnetic field of 10 mT. A slow permanent hole burning mechanism is observed. If the excitation frequency is not changed the fluorescence intensity is reduced by more than 50$%$ after a couple of minutes of continuous excitation. The spectral hole created by the permanent hole burning has a width in the tens of MHz range, which indicates that a trapping mechanism occurs via the 5d-state.
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We experimentally study a broadband implementation of the atomic frequency comb (AFC) rephasing protocol with a cryogenically cooled Pr$^{3+}$:Y$_2$SiO$_5$ crystal. To allow for storage of broadband pulses, we explore a novel regime where the input photonic bandwidth closely matches the inhomogeneous broadening of the material $(sim5,textrm{GHz})$, thereby significantly exceeding the hyperfine ground and excited state splitting $(sim10,textrm{MHz})$. Through an investigation of different AFC preparation parameters, we measure a maximum efficiency of $10%$ after a rephasing time of $12.5,$ns. With a suboptimal AFC, we witness up to 12 rephased temporal modes.
We present and analyze four frequency measurements designed to characterize the performance of an optical frequency reference based on spectral hole burning in EuYSO. The first frequency comparison, between a single unperturbed spectral hole and a hydrogen maser, demonstrates a fractional frequency drift rate of $5 times 10^{-18}$ s$^{-1}$. Optical-frequency comparisons between a pattern of spectral holes, a Fabry-Perot cavity, and an Al$^+$ optical atomic clock show a short-term fractional frequency stability of $1 times10^{-15} tau^{-1/2}$ that averages down to $2.5^{+1.1}_{-0.5} times 10^{-16}$ at $tau = 540~s$ (with linear frequency drift removed). Finally, spectral hole patterns in two different EuYSO crystals located in the same cryogenic vessel are compared, yielding a short-term stability of $7 times10^{-16} tau^{-1/2}$ that averages down to $5.5^{+1.8}_{-0.9} times 10^{-17}$ at $tau = 204$~s (with quadratic frequency drift removed).
Interfacing photonic and solid-state qubits within a hybrid quantum architecture offers a promising route towards large scale distributed quantum computing. In that respect, hybrid quantum systems combining circuit QED with ions doped into solids are an attractive platform. There, the ions serve as coherent memory elements and reversible conversion elements of microwave to optical qubits. Among many possible spin-doped solids, erbium ions offer the unique opportunity of a coherent conversion of microwave photons into the telecom C-band at $1.54,mu$m employed for long distance communication. In our work, we perform a time-resolved electron spin resonance study of an Er$^{3+}$:Y$_2$SiO$_5$ spin ensemble at milli-Kelvin temperatures and demonstrate multimode storage and retrieval of up to 16 coherent microwave pulses. The memory efficiency is measured to be 10$^{-4}$ at the coherence time of $T_2=5.6,mu$s.
Er:YSO crystal is promising candidate with great variety of its potential applications in quantum information processing and quantum communications ranging from optical/microwave quantum memories to circuit QED and microwave-to-optics frequency converters. Some of the above listed applications require ultra-low temperature environment, i.e. temperatures $Tlesssim0.1~$K. Most of the experiments with erbium doped crystals have been so far carried out at temperatures above 1.5 K. Therefore, only little information is known about Er:YSO coherence properties at millikelvins. Here, we investigate optical decoherence of $^{167}$Er:Y$_2$SiO$_5$ crystal by performing 2- and 3-pulse echo experiments at sub-Kelvin temperature range and at weak and moderate magnetic fields. We show that the deep freezing of the crystal results in an increase of optical coherence time by one order of magnitude below 1.5 Kelvin at the field of $sim$0.2 T. We further describe the detailed investigation of the decoherence mechanisms in this regime.
Efficient optical pumping is an important tool for state initialization in quantum technologies, such as optical quantum memories. In crystals doped with Kramers rare-earth ions, such as erbium and neodymium, efficient optical pumping is challenging due to the relatively short population lifetimes of the electronic Zeeman levels, of the order of 100 ms at around 4 K. In this article we show that optical pumping of the hyperfine levels in isotopically enriched $^{145}$Nd$^{3+}$:Y$_2$SiO$_5$ crystals is more efficient, owing to the longer population relaxation times of hyperfine levels. By optically cycling the population many times through the excited state a nuclear-spin flip can be forced in the ground-state hyperfine manifold, in which case the population is trapped for several seconds before relaxing back to the pumped hyperfine level. To demonstrate the effectiveness of this approach in applications we perform an atomic frequency comb memory experiment with 33% storage efficiency in $^{145}$Nd$^{3+}$:Y$_2$SiO$_5$, which is on a par with results obtained in non-Kramers ions, e.g. europium and praseodymium, where optical pumping is generally efficient due to the quenched electronic spin. Efficient optical pumping in neodymium-doped crystals is also of interest for spectral filtering in biomedical imaging, as neodymium has an absorption wavelength compatible with tissue imaging. In addition to these applications, our study is of interest for understanding spin dynamics in Kramers ions with nuclear spin.
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