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Register a new userMicrowave multimode memory with an Er$^{3+}$:Y$_2$SiO$_5$ spin ensemble
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Interfacing photonic and solid-state qubits within a hybrid quantum architecture offers a promising route towards large scale distributed quantum computing. In that respect, hybrid quantum systems combining circuit QED with ions doped into solids are an attractive platform. There, the ions serve as coherent memory elements and reversible conversion elements of microwave to optical qubits. Among many possible spin-doped solids, erbium ions offer the unique opportunity of a coherent conversion of microwave photons into the telecom C-band at $1.54,mu$m employed for long distance communication. In our work, we perform a time-resolved electron spin resonance study of an Er$^{3+}$:Y$_2$SiO$_5$ spin ensemble at milli-Kelvin temperatures and demonstrate multimode storage and retrieval of up to 16 coherent microwave pulses. The memory efficiency is measured to be 10$^{-4}$ at the coherence time of $T_2=5.6,mu$s.
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We experimentally study a broadband implementation of the atomic frequency comb (AFC) rephasing protocol with a cryogenically cooled Pr$^{3+}$:Y$_2$SiO$_5$ crystal. To allow for storage of broadband pulses, we explore a novel regime where the input photonic bandwidth closely matches the inhomogeneous broadening of the material $(sim5,textrm{GHz})$, thereby significantly exceeding the hyperfine ground and excited state splitting $(sim10,textrm{MHz})$. Through an investigation of different AFC preparation parameters, we measure a maximum efficiency of $10%$ after a rephasing time of $12.5,$ns. With a suboptimal AFC, we witness up to 12 rephased temporal modes.
We performed magnetic field and frequency tunable electron paramagnetic resonance spectroscopy of an Er$^{3+}$ doped Y$_2$SiO$_5$ crystal by observing the change in flux induced on a direct current-superconducting quantum interference device (dc-SQUID) loop of a tunable Josephson bifurcation amplifer. The observed spectra show multiple transitions which agree well with the simulated energy levels, taking into account the hyperfine and quadrupole interactions of $^{167}$Er. The sensing volume is about 0.15 pl, and our inferred measurement sensitivity (limited by external flux noise) is approximately $1.5times10^4$ electron spins for a 1 s measurement. The sensitivity value is two orders of magnitude better than similar schemes using dc-SQUID switching readout.
Electron-spin nitrogen-vacancy color centers in diamond are a natural candidate to act as a quantum memory for superconducting qubits because of their large collective coupling and long coherence times. We report here the first demonstration of strong coupling and coherent exchange of a single quantum of energy between a flux-qubit and an ensemble of nitrogen-vacancy color centers.
Interactions are essential for the creation of correlated quantum many-body states. While two-body interactions underlie most natural phenomena, three- and four-body interactions are important for the physics of nuclei [1], exotic few-body states in ultracold quantum gases [2], the fractional quantum Hall effect [3], quantum error correction [4], and holography [5, 6]. Recently, a number of artificial quantum systems have emerged as simulators for many-body physics, featuring the ability to engineer strong interactions. However, the interactions in these systems have largely been limited to the two-body paradigm, and require building up multi-body interactions by combining two-body forces. Here, we demonstrate a pure N-body interaction between microwave photons stored in an arbitrary number of electromagnetic modes of a multimode cavity. The system is dressed such that there is collectively no interaction until a target total photon number is reached across multiple distinct modes, at which point they interact strongly. The microwave cavity features 9 modes with photon lifetimes of $sim 2$ ms coupled to a superconducting transmon circuit, forming a multimode circuit QED system with single photon cooperativities of $sim10^9$. We generate multimode interactions by using cavity photon number resolved drives on the transmon circuit to blockade any multiphoton state with a chosen total photon number distributed across the target modes. We harness the interaction for state preparation, preparing Fock states of increasing photon number via quantum optimal control pulses acting only on the cavity modes. We demonstrate multimode interactions by generating entanglement purely with uniform cavity drives and multimode photon blockade, and characterize the resulting two- and three-mode W states using a new protocol for multimode Wigner tomography.
Efficient optical pumping is an important tool for state initialization in quantum technologies, such as optical quantum memories. In crystals doped with Kramers rare-earth ions, such as erbium and neodymium, efficient optical pumping is challenging due to the relatively short population lifetimes of the electronic Zeeman levels, of the order of 100 ms at around 4 K. In this article we show that optical pumping of the hyperfine levels in isotopically enriched $^{145}$Nd$^{3+}$:Y$_2$SiO$_5$ crystals is more efficient, owing to the longer population relaxation times of hyperfine levels. By optically cycling the population many times through the excited state a nuclear-spin flip can be forced in the ground-state hyperfine manifold, in which case the population is trapped for several seconds before relaxing back to the pumped hyperfine level. To demonstrate the effectiveness of this approach in applications we perform an atomic frequency comb memory experiment with 33% storage efficiency in $^{145}$Nd$^{3+}$:Y$_2$SiO$_5$, which is on a par with results obtained in non-Kramers ions, e.g. europium and praseodymium, where optical pumping is generally efficient due to the quenched electronic spin. Efficient optical pumping in neodymium-doped crystals is also of interest for spectral filtering in biomedical imaging, as neodymium has an absorption wavelength compatible with tissue imaging. In addition to these applications, our study is of interest for understanding spin dynamics in Kramers ions with nuclear spin.
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