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Register a new userTalbot effect for exciton-polaritons
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We demonstrate, experimentally and theoretically, a Talbot effect for hybrid light-matter waves -- exciton-polariton condensate formed in a semiconductor microcavity with embedded quantum wells. The characteristic Talbot carpet is produced by loading the exciton-polariton condensate into a microstructured one dimensional periodic array of mesa traps, which creates an array of sources for coherent polariton flow in the plane of the quantum wells. The spatial distribution of the Talbot fringes outside the mesas mimics the near-field diffraction of a monochromatic wave on a periodic amplitude and phase grating with the grating period comparable to the wavelength. Despite the lossy nature of the polariton system, the Talbot pattern persists for distances exceeding the size of the mesas by an order of magnitude.
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We present experimental observations of a non-resonant dynamic Stark shift in strongly coupled microcavity quantum well exciton-polaritons - a system which provides a rich variety of solid-state collective phenomena. The Stark effect is demonstrated in a GaAs/AlGaAs system at 10K by femtosecond pump-probe measurements, with the blue shift approaching the meV scale for a pump fluence of 2 mJcm^-2 and 50 meV red detuning, in good agreement with theory. The energy level structure of the strongly coupled polariton Rabi-doublet remains unaffected by the blue shift. The demonstrated effect should allow generation of ultrafast density-independent potentials and imprinting well-defined phase profiles on polariton condensates, providing a powerful tool for manipulation of these condensates, similar to dipole potentials in cold atom systems.
Microcavity exciton-polaritons, known to exhibit non-equilibrium Bose condensation at high critical temperatures, can be also brought in thermal equilibrium with the surrounding medium and form a quantum degenerate Bose-Einstein distribution. It happens when their thermalization time in the regime of positive detunings -- or, alternatively, for high-finesse microcavities -- becomes shorter than their lifetime. Here we present the self-consistent finite-temperature Hartree-Fock-Bogoliubov description for such a system of polaritons, universally addressing the excitation spectrum, momentum-dependent interactions, condensate depletion, and the background population of dark excitons that contribute to the systems chemical potential. Employing the derived expressions, we discuss the implications for the Bogoliubov sound velocity, confirmed by existing experiments, and define the critical temperatures of (quasi-)condensation and the integral particle lifetime dependencies on the detuning. Large positive detunings are shown to provide conditions for the total lifetime reaching nanosecond timescales. This allows realization of thermodynamically-equilibrium polariton systems with Bose-Einstein condensate forming at temperatures as high as tens of Kelvin.
Bose-Einstein condensate of exciton polaritons in a semiconductor microcavity is a macroscopically populated coherent quantum state subject to concurrent pumping and decay. Debates about the fundamental nature of the condensed phase in this open quantum system still persist. Here, we gain a new insight into the spontaneous condensation process by imaging long-lifetime exciton polaritons in a high-quality inorganic microcavity in the single-shot optical excitation regime, without averaging over multiple condensate realisations. In this highly non-stationary regime, a condensate is strongly influenced by the `hot incoherent reservoir, and reservoir depletion is critical for the transition to the ground energy and momentum state. Condensates formed by more photonic exciton polaritons exhibit dramatic reservoir-induced density filamentation and shot-to-shot fluctuations. In contrast, condensates of more excitonic quasiparticles display smooth density and are second-order coherent. Our observations show that the single-shot measurements offer a unique opportunity to study formation of macroscopic phase coherence during a quantum phase transition in a solid state system.
Strong light matter coupling between excitons and microcavity photons, as described in the framework of cavity quantum electrodynamics, leads to the hybridization of light and matter excitations. The regime of collective strong coupling arises, when various excitations from different host media are strongly coupled to the same optical resonance. This leads to a well-controllable admixture of various matter components in three hybrid polariton modes. Here, we study a cavity device with four embedded GaAs quantum wells hosting excitons that are spectrally matched to the A-valley exciton resonance of a MoSe2 monolayer. The formation of hybrid polariton modes is evidenced in momentum resolved photoluminescence and reflectivity studies. We describe the energy and k-vector distribution of exciton-polaritons along the hybrid modes by a thermodynamic model, which yields a very good agreement with the experiment.
We study both experimentally and theoretically, considering bosonic atoms in a periodic potential, the influence of interactions in a Talbot interferometer. While interactions decrease the contrast of the revivals, we find that over a wide range of interactions the Talbot signal is still proportional to the phase coherence of the matter wave field. Our results confirm that Talbot interferometry can be a useful tool to study finite range phase correlations in an optical lattice even in the presence of interactions. The relative robustness of the Talbot signal is supported by the first demonstration of the three-dimensional Talbot effect.
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