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Register a new userMagnetotransport study of the pressure-induced antiferromagnetic phase in FeSe
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The resistivity $rho$ and Hall resistivity $rho_H$ are measured on FeSe at pressures up to $P$ = 28.3 kbar in magnetic fields up to $B$ = 14.5 T. The $rho(B)$ and $rho_H(B)$ curves are analyzed with multicarrier models to estimate the carrier density and mobility as a function of $P$ and temperature ($ Tleqslant$ 110 K). It is shown that the pressure-induced antiferromagnetic transition is accompanied by an abrupt reduction of the carrier density and scattering. This indicates that the electronic structure is reconstructed significantly by the antiferromagnetic order.
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We report measurements of resistance and ac magnetic susceptibility on FeSe single crystals under high pressure up to 27.2 kbar. The structural phase transition is quickly suppressed with pressure, and the associated anomaly is not seen above $sim$18 kbar. The superconducting transition temperature evolves nonmonotonically with pressure, showing a minimum at $sim12$ kbar. We find another anomaly at 21.2 K at 11.6 kbar. This anomaly most likely corresponds to the antiferromagnetic phase transition found in $mu$SR measurements [M. Bendele textit{et al.}, Phys. Rev. Lett. textbf{104}, 087003 (2010)]. The antiferromagnetic and superconducting transition temperatures both increase with pressure up to $sim25$ kbar and then level off. The width of the superconducting transition anomalously broadens in the pressure range where the antiferromagnetism coexists.
The pressure dependence of the structural ($T_s$), antiferromagnetic ($T_m$), and superconducting ($T_c$) transition temperatures in FeSe is investigated on the basis of the 16-band $d$-$p$ model. At ambient pressure, a shallow hole pocket disappears due to the correlation effect, as observed in the angular-resolved photoemission spectroscopy (ARPES) and quantum oscillation (QO) experiments, resulting in the suppression of the antiferromagnetic order, in contrast to the other iron pnictides. The orbital-polarization interaction between the Fe $d$ orbital and Se $p$ orbital is found to drive the ferro-orbital order responsible for the structural transition without accompanying the antiferromagnetic order. The pressure dependence of the Fermi surfaces is derived from the first-principles calculation and is found to well account for the opposite pressure dependences of $T_s$ and $T_m$, around which the enhanced orbital and magnetic fluctuations cause the double-dome structure of the eigenvalue $lambda$ in the Eliashberg equation, as consistent with that of $T_c$ in FeSe.
We present $beta$-FeSe magnetotransport data, and describe them theoretically. Using a simplified microscopic model with two correlated effective orbitals, we determined the normal state electrical conductivity and Hall coefficient, using Kubo formalism. With model parameters relevant for Fe-chalcogenides, we describe the observed effect of the structural transition on the ab-plane electrical resistivity, as well as on the magnetoresistance. Temperature-dependent Hall coefficient data were measured at 16 Tesla, and their theoretical description improves upon inclusion of moderate electron correlations. We confirm the effect of the structural transition on the electronic structure, finding deformation-induced band splittings comparable to those reported in angle-resolved photoemission.
The effects of pressure on antiferromagnetic (AFM) and superconducting phase transitions of 112-type Ca$_{1-x}$La$_{x}$FeAs$_{2}$ were studied, and the in-plane electrical resistivity $rho_{ab}$ was measured with an indenter-type pressure cell. The AFM phase transition temperatures of $T_{rm N}$ = 47, 63, and 63 K at ambient pressure for $x$ = 0.18, 0.21, and 0.26 was suppressed by applying pressure $P$, with superconductivity emerging at critical pressures of $P_{rm c}$ $simeq$ 0, 1.5, and 3.4 GPa, respectively. Correspondingly, the slope of $T_{rm N}$ against $P$ decreased as $dT_{rm N}/P$ $simeq$ $-$15 and $-$2 K/GPa for $x$ = 0.21 and 0.26, respectively. Thus, although the AFM phase was stabilized with La doping $x$, the AFM phase was suppressed by pressure, and superconductivity eventually emerged.
We present high-energy x-ray diffraction data under applied pressures up to p = 29 GPa, neutron diffraction measurements up to p = 1.1 GPa, and electrical resistance measurements up to p = 5.9 GPa, on SrCo2As2. Our x-ray diffraction data demonstrate that there is a first-order transition between the tetragonal (T) and collapsed-tetragonal (cT) phases, with an onset above approximately 6 GPa at T = 7 K. The pressure for the onset of the cT phase and the range of coexistence between the T and cT phases appears to be nearly temperature independent. The compressibility along the a-axis is the same for the T and cT phases whereas, along the c-axis, the cT phase is significantly stiffer, which may be due to the formation of an As-As bond in the cT phase. Our resistivity measurements found no evidence of superconductivity in SrCo2As2 for p <= 5.9 GPa and T >= 1.8 K. The resistivity data also show signatures consistent with a pressure-induced phase transition for p >= 5.5 GPa. Single-crystal neutron diffraction measurements performed up to 1.1 GPa in the T phase found no evidence of stripe-type or A-type antiferromagnetic ordering down to 10 K. Spin-polarized total-energy calculations demonstrate that the cT phase is the stable phase at high pressure with a c/a ratio of 2.54. Furthermore, these calculations indicate that the cT phase of SrCo2As2 should manifest either A-type antiferromagnetic or ferromagnetic order.
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