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Register a new userPressure-Induced Superconductivity from Doping-Induced Antiferromagnetic Phase of 112-type Ca$_{1-x}$La$_{x}$FeAs$_{2}$
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The effects of pressure on antiferromagnetic (AFM) and superconducting phase transitions of 112-type Ca$_{1-x}$La$_{x}$FeAs$_{2}$ were studied, and the in-plane electrical resistivity $rho_{ab}$ was measured with an indenter-type pressure cell. The AFM phase transition temperatures of $T_{rm N}$ = 47, 63, and 63 K at ambient pressure for $x$ = 0.18, 0.21, and 0.26 was suppressed by applying pressure $P$, with superconductivity emerging at critical pressures of $P_{rm c}$ $simeq$ 0, 1.5, and 3.4 GPa, respectively. Correspondingly, the slope of $T_{rm N}$ against $P$ decreased as $dT_{rm N}/P$ $simeq$ $-$15 and $-$2 K/GPa for $x$ = 0.21 and 0.26, respectively. Thus, although the AFM phase was stabilized with La doping $x$, the AFM phase was suppressed by pressure, and superconductivity eventually emerged.
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We report the discovery and characterization of a novel 112-type iron pnictide EuFeAs2, with La-doping induced superconductivity in a series of Eu1-xLaxFeAs2. The polycrystalline samples were synthesized through solid state reaction method only within a very narrow temperature window around 1073 K. Small single crystals were also grown from a flux method with the size about 100 um. The crystal structure was identified by single crystal X-ray diffraction analysis as a monoclinic structure with space group of P21/m. From resistivity and magnetic susceptibility measurements, we found that the parent compound EuFeAs2 shows a Fe2+ related antiferromagnetic/structural phase transition near 110 K and a Eu2+ related antiferromagnetic phase transition near 40 K. La doping suppressed the both phase transitions and induced superconducting transition with a Tc ~ 11 K for Eu0.85La0.15FeAs2.
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