Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userDroplet spreading on rough surfaces: tackling the contact line boundary condition
108
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
The complicated dynamics of the contact line of a moving droplet on a solid substrate often hamper the efficient modeling of microfluidic systems. In particular, the selection of the effective boundary conditions, specifying the contact line motion, is a controversial issue since the microscopic physics that gives rise to this displacement is still unknown. Here, a sharp interface, continuum-level, novel modeling approach, accounting for liquid/solid micro-scale interactions assembled in a disjoining pressure term, is presented. By following a unified conception (the model applies both to the liquid/solid and the liquid/ambient interfaces), the friction forces at the contact line, as well as the dynamic contact angle are derived implicitly as a result of the disjoining pressure and viscous effects interplay in the vicinity of the substrates intrinsic roughness. Previous hydrodynamic model limitations, of imposing the contact line boundary condition to an unknown number and reconfigurable contact lines, when modeling the spreading dynamics on textured substrates, are now overcome. The validity of our approach is tested against experimental data of a droplet impacting on a horizontal solid surface. The study of the early spreading stage on hierarchically structured and chemically patterned solid substrates reveal an inertial regime where the contact radius grows according to a universal power law, perfectly agreeing with recently published experimental findings.
rate research
Read More
We study experimentally and theoretically the equilibrium adhesive contact between a smooth glass lens and a rough rubber surface textured with spherical microasperities with controlled height and spatial distributions. Measurements of the real contact area $A$ versus load $P$ are performed under compression by imaging the light transmitted at the microcontacts. $A(P)$ is found to be non-linear and to strongly depend on the standard deviation of the asperity height distribution. Experimental results are discussed in the light of a discrete version of Fuller and Tabors (FT) original model (textit{Proceedings of the Royal Society A} textbf{345} (1975) 327), which allows to take into account the elastic coupling arising from both microasperities interactions and curvature of the glass lens. Our experimental data on microcontact size distributions are well captured by our discrete extended model. We show that the elastic coupling arising from the lens curvature has a significant contribution to the $A(P)$ relationship. Our discrete model also clearly shows that the adhesion-induced effect on $A$ remains significant even for vanishingly small pull-off forces. Last, at the local asperity length scale, our measurements show that the pressure dependence of the microcontacts density can be simply described by the original FT model.
We report on normal contact and friction measurements of model multicontact interfaces formed between smooth surfaces and substrates textured with a statistical distribution of spherical micro-asperities. Contacts are either formed between a rigid textured lens and a smooth rubber, or a flat textured rubber and a smooth rigid lens. Measurements of the real area of contact $A$ versus normal load $P$ are performed by imaging the light transmitted at the microcontacts. For both interfaces, $A(P)$ is found to be sub-linear with a power law behavior. Comparison to two multi-asperity contact models, which extend Greenwood-Williamson (J. Greenwood, J. Williamson, textit{Proc. Royal Soc. London Ser. A} textbf{295}, 300 (1966)) model by taking into account the elastic interaction between asperities at different length scales, is performed, and allows their validation for the first time. We find that long range elastic interactions arising from the curvature of the nominal surfaces are the main source of the non-linearity of $A(P)$. At a shorter range, and except for very low pressures, the pressure dependence of both density and area of micro-contacts remains well described by Greenwood-Williamsons model, which neglects any interaction between asperities. In addition, in steady sliding, friction measurements reveal that the mean shear stress at the scale of the asperities is systematically larger than that found for a macroscopic contact between a smooth lens and a rubber. This suggests that frictional stresses measured at macroscopic length scales may not be simply transposed to microscopic multicontact interfaces.
Frictional properties of contacts between a smooth viscoelastic rubber and rigid surfaces are investigated using a torsional contact configuration where a glass lens is continuously rotated on the rubber surface. From the inversion of the displacement field measured at the surface of the rubber, spatially resolved values of the steady state frictional shear stress are determined within the non homogeneous pressure and velocity fields of the contact. For contacts with a smooth lens, a velocity dependent but pressure independent local shear stress is retrieved from the inversion. On the other hand, the local shear stress is found to depend both on velocity and applied contact pressure when a randomly rough (sand blasted) glass lens is rubbed against the rubber surface. As a result of changes in the density of micro-asperity contacts, the amount of light transmitted by the transparent multi-contact interface is observed to vary locally as a function of both contact pressure and sliding velocity. Under the assumption that the intensity of light transmitted by the rough interface is proportional to the proportion of area into contact, it is found that the local frictional stress can be expressed experimentally as the product of a purely velocity dependent term, $k(v)$, by a term representing the pressure and velocity dependence of the actual contact area, $A/A_0$. A comparison between $k(v)$ and the frictional shear stress of smooth contacts suggests that nanometer scale dissipative processes occurring at the interface predominate over viscoelastic dissipation at micro-asperity scale.
When a drop of water is placed on a rough surface, there are two possible extreme regimes of wetting: the one called Cassie-Baxter (CB) with air pockets trapped underneath the droplet and the one characterized by the homogeneous wetting of the surface, called the Wenzel (W) state. A way to investigate the transition between these two states is by means of evaporation experiments, in which the droplet starts in a CB state and, as its volume decreases, penetrates the surfaces grooves, reaching a W state. Here we present a theoretical model based on the global interfacial energies for CB and W states that allows us to predict the thermodynamic wetting state of the droplet for a given volume and surface texture. We first analyze the influence of the surface geometric parameters on the droplets final wetting state with constant volume, and show that it depends strongly on the surface texture. We then vary the volume of the droplet keeping fixed the geometric surface parameters to mimic evaporation and show that the drop experiences a transition from the CB to the W state when its volume reduces, as observed in experiments. To investigate the dependency of the wetting state on the initial state of the droplet, we implement a cellular Potts model in three dimensions. Simulations show a very good agreement with theory when the initial state is W, but it disagrees when the droplet is initialized in a CB state, in accordance with previous observations which show that the CB state is metastable in many cases. Both simulations and theoretical model can be modified to study other types of surface.
We investigate the effects of roughness and fractality on the normal contact stiffness of rough surfaces. Samples of isotropically roughened aluminium surfaces are considered. The roughness and fractal dimension were altered through blasting using different sized particles. Subsequently, surface mechanical attrition treatment (SMAT) was applied to the surfaces in order to modify the surface at the microscale. The surface topology was characterised by interferometry based profilometry. The normal contact stiffness was measured through nanoindentation with a flat tip utilising the partial unloading method. We focus on establishing the relationships between surface stiffness and roughness, combined with the effects of fractal dimension. The experimental results, for a wide range of surfaces, showed that the measured contact stiffness depended very closely on surfaces root mean squared (RMS) slope and their fractal dimension, with correlation coefficients of around 90%, whilst a relatively weak correlation coefficient of 57% was found between the contact stiffness and RMS roughness.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
