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Register a new userSpectroscopy of metal superatom nanoclusters and high-$T_c$ superconducting pairing
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A unique property of metal nanoclusters is the superatom shell structure of their delocalized electrons. The electronic shell levels are highly degenerate and therefore represent sharp peaks in the density of states. This can enable exceptionally strong electron pairing in certain clusters composed of tens to hundreds of atoms. In a finite system, such as a free nanocluster or a nucleus, pairing is observed most clearly via its effect on the energy spectrum of the constituent fermions. Accordingly, we performed a photoionization spectroscopy study of size-resolved aluminum nanoclusters and observed a rapid rise of the near-threshold density of states of several clusters ($Al_{37,44,66,68}$) with decreasing temperature. The characteristics of this behavior are consistent with compression of the density of states by a pairing transition into a high-temperature superconducting state with $T_c$>~100 K. This value exceeds that of bulk aluminum by two orders of magnitude. These results highlight the potential of novel pairing effects in size-quantized systems and the possibility to attain even higher critical temperatures by optimizing the particles size and composition. As a new class of high-temperature superconductors, such metal nanocluster particles are promising building blocks for high-$T_c$ materials, devices, and networks.
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A unique property of size-resolved metal nanocluster particles is their superatom-like electronic shell structure. The shell levels are highly degenerate, and it has been predicted that this can enable exceptionally strong superconducting-type electron pair correlations in certain clusters composed of just tens to hundreds of atoms. Here we report on the observation of a possible spectroscopic signature of such an effect. A bulge-like feature appears in the photoionization yield curve of a free cold aluminum cluster and shows a rapid rise as the temperature approaches approximately 100 K. This is an unusual effect, not previously reported for clusters. Its characteristics are consistent with an increase in the effective density of states accompanying a pairing transition, which suggests a high-temperature superconducting state with Tc>~100 K. Our results highlight the promise of metal nanoclusters as high-Tc building blocks for materials and networks.
Topological superconductors represent a newly predicted phase of matter that is topologically distinct from conventional superconducting condensates of Cooper pairs. As a manifestation of their topological character, topological superconductors support solid-state realizations of Majorana fermions at their boundaries. The recently discovered superconductor CuxBi2Se3 has been theoretically proposed as an odd-parity superconductor in the time-reversal-invariant topological superconductor class and point-contact spectroscopy measurements have reported the observation of zero-bias conductance peaks corresponding to Majorana states in this material. Here we report scanning tunneling spectroscopy (STS) measurements of the superconducting energy gap in CuxBi2Se3 as a function of spatial position and applied magnetic field. The tunneling spectrum shows that the density of states at the Fermi level is fully gapped without any in-gap states. The spectrum is well described by the Bardeen-Cooper-Schrieffer (BCS) theory with a momentum independent order parameter, which suggests that Cu0.2Bi2Se3 is a classical s-wave superconductor contrary to previous expectations and measurements.
We study a superconducting hetro-junction with one side characterized by the unconventional chiral $p$-wave gap function $p_xpm ip_y$ and the other side the conventional $s$-wave one. Though a relative phase of $pm frac{pi}{2}$ between any two components of gap functions is favored in the junction region, mutual phase differences cannot achieve $pm frac{pi}{2}$ simultaneously, which results in frustration. Based on a Ginzburg-Landau free energy analysis, the frustrated pattern is determined to be $s+ ieta_1 (e^{ ieta_2 varphi/2}p_x +eta_3 e^{- ieta_2 varphi/2}p_y)$ with $eta_j=pm 1$ ($j=1,2,3$), where $varphi$ is the phase difference between the $p_x$- and $p_y$-wave gap functions. Furthermore, we find that the junction exhibits an anisotropic magnetoelectric effect, manifesting itself as an anisotropic spin magnetization along the edge of the junction.
We studied experimentally and theoretically the electronic local density of states (LDOS) near single step edges at the surface of exfoliated graphite. In scanning tunneling microscopy measurements, we observed the $(sqrt{3} times sqrt{3}) R 30^{circ}$ and honeycomb superstructures extending over 3$-$4 nm both from the zigzag and armchair edges. Calculations based on a density-functional derived non-orthogonal tight-binding model show that these superstructures can coexist if the two types of edges admix each other in real graphite step edges. Scanning tunneling spectroscopy measurements near the zigzag edge reveal a clear peak in the LDOS at an energy below the Fermi energy by 20 meV. No such a peak was observed near the armchair edge. We concluded that this peak corresponds to the edge state theoretically predicted for graphene ribbons, since a similar prominent LDOS peak due to the edge state is obtained by the first principles calculations.
We suggest to use `fluctuation spectroscopy as a method to detect granularity in a disordered metal close to a superconducting transition. We show that with lowering temperature $T$ the resistance $R(T)$ of a system of relatively large grains initially grows due to the fluctuation suppression of the one-electron tunneling but decreases with further lowering $T$ due to the coherent charge transfer of the fluctuation Cooper pairs. Under certain conditions, such a maximum in $R(T)$ turns out to be sensitive to weak magnetic fields due to a novel Maki -- Thompson type mechanism.
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