We elucidate the effects of defect disorder and $e$-$e$ interaction on the spectral density of the defect states emerging in the Mott-Hubbard gap of doped transition-metal oxides, such as Y$_{1-x}$Ca$_{x}$VO$_{3}$. A soft gap of kinetic origin develops in the defect band and survives defect disorder for $e$-$e$ interaction strengths comparable to the defect potential and hopping integral values above a doping dependent threshold, otherwise only a pseudogap persists. These two regimes naturally emerge in the statistical distribution of gaps among different defect realizations, which turns out to be of Weibull type. Its shape parameter $k$ determines the exponent of the power-law dependence of the density of states at the chemical potential ($k-1$) and hence distinguishes between the soft gap ($kgeq2$) and the pseudogap ($k<2$) regimes. Both $k$ and the effective gap scale with the hopping integral and the $e$-$e$ interaction in a wide doping range. The motion of doped holes is confined by the closest defect potential and the overall spin-orbital structure. Such a generic behavior leads to complex non-hydrogen-like defect states that tend to preserve the underlying $C$-type spin and $G$-type orbital order and can be detected and analyzed via scanning tunneling microscopy.
The simultaneous interplay of strong electron-electron correlations, topological zero-energy states, and disorder is yet an unexplored territory but of immense interest due to their inevitable presence in many materials. Copper oxide high-temperature superconductors (cuprates) with pair breaking edges host a flat band of topological zero-energy states, making them an ideal playground where strong correlations, topology, and disorder are strongly intertwined. Here we show that this interplay in cuprates generates a new phase of matter: a fully gapped phase crystal state that breaks both translational and time reversal invariance, characterized by a modulation of the $d$-wave superconducting phase co-existing with a modulating extended $s$-wave superconducting order. In contrast to conventional wisdom, we find that this phase crystal state is remarkably robust to omnipresent disorder, but only in the presence of strong correlations, thus giving a clear route to its experimental realization.
We explore the competiton of doped holes and defects that leads to the loss of orbital order in vanadate perovskites. In compounds such as La$_{1-{sf x}}$Ca$_{,sf x}$VO$_3$ spin and orbital order result from super-exchange interactions described by an extended three-orbital degenerate Hubbard-Hund model for the vanadium $t_{2g}$ electrons. Long-range Coulomb potentials of charged Ca$^{2+}$ defects and $e$-$e$ interactions control the emergence of defect states inside the Mott gap. The quadrupolar components of the Coulomb fields of doped holes induce anisotropic orbital rotations of degenerate orbitals. These rotations modify the spin-orbital polaron clouds and compete with orbital rotations induced by defects. Both mechanisms lead to a mixing of orbitals, and cause the suppression of the asymmetry of kinetic energy in the $C$-type magnetic phase. We find that the gradual decline of orbital order with doping, a characteristic feature of the vanadates, however, has its origin not predominantly in the charge carriers, but in the off-diagonal couplings of orbital rotations induced by the charges of the doped ions.
The topological Anderson and Mott insulators are two phases that have so far been separately and widely explored beyond topological band insulators. Here we combine the two seemingly different topological phases into a system of spin-1/2 interacting fermionic atoms in a disordered optical lattice. We find that the topological Anderson and Mott insulators in the noninteracting and clean limits can be adiabatically connected without gap closing in the phase diagram of our model. Lying between the two phases, we uncover a disordered correlated topological insulator, which is induced from a trivial band insulator by the combination of disorder and interaction, as the generalization of topological Anderson insulators to the many-body interacting regime. The phase diagram is determined by computing various topological properties and confirmed by unsupervised and automated machine learning. We develop an approach to provide a unified and clear description of topological phase transitions driven by interaction and disorder. The topological phases can be detected from disorder/interaction induced edge excitations and charge pumping in optical lattices.
We study the surface of a three-dimensional spin chiral $mathrm{Z}_2$ topological insulator (class CII), demonstrating the possibility of its localization. This arises through an interplay of interaction and statistically-symmetric disorder, that confines the gapless fermionic degrees of freedom to a network of one-dimensional helical domain-walls that can be localized. We identify two distinct regimes of this gapless insulating phase, a `clogged regime wherein the network localization is induced by its junctions between otherwise metallic helical domain-walls, and a `fully localized regime of localized domain-walls. The experimental signatures of these regimes are also discussed.
We demonstrate that a combination of disorder and interactions in a two-dimensional bulk topological insulator can generically drive its helical edge insulating. We establish this within the framework of helical Luttinger liquid theory and exact Emery-Luther mapping. The gapless glassy edge state spontaneously breaks time-reversal symmetry in a `spin glass fashion, and may be viewed as a localized state of solitons which carry half integer charge. Such a qualitatively distinct edge state provides a simple explanation for heretofore puzzling experimental observations. This phase exhibits a striking non-monotonicity, with the edge growing less localized in both the weak and strong disorder limits.
Adolfo Avella
,Andrzej M. Oles
,Peter Horsch
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(2015)
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"Defects, disorder and strong electron correlations in orbital degenerate, doped Mott insulators"
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Adolfo Avella
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