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A Kondo route to spin inhomogeneities in the honeycomb Kitaev model

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 Added by Vikram Tripathi
 Publication date 2015
  fields Physics
and research's language is English




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Paramagnetic impurities in a quantum spin-liquid can result in Kondo effects with highly unusual properties. We have studied the effect of locally exchange-coupling a paramagnetic impurity with the spin-1/2 honeycomb Kitaev model in its gapless spin-liquid phase. The (impurity) scaling equations are found to be insensitive to the sign of the coupling. The weak and strong coupling fixed points are stable, with the latter corresponding to a noninteracting vacancy and an interacting, spin-1 defect for the antiferromagnetic and ferromagnetic cases respectively. The ground state in the strong coupling limit in both cases has a nontrivial topology associated with a finite Z2 flux at the impurity site. For the antiferromagnetic case, this result can be obtained straightforwardly owing to the integrability of the Kitaev model with a vacancy. The strong-coupling limit of the ferromagnetic case is however nonintegrable, and we address this problem through exact-diagonalization calculations with finite Kitaev fragments. Our exact diagonalization calculations indicate that that the weak to strong coupling transition and the topological phase transition occur rather close to each other and are possibly coincident. We also find an intriguing similarity between the magnetic response of the defect and the impurity susceptibility in the two-channel Kondo problem.



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In this work we investigate whether the Kitaev honeycomb model can serve as a starting point to realize the intriguing physics of the Sachdev-Ye-Kitaev model. The starting point is to strain the system which leads to flat bands reminiscent of Landau levels, thereby quenching the kinetic energy. The presence of weak residual perturbations, such as Heisenberg interactions and the $gamma$-term, creates effective interactions between the Majorana modes when projected into the flux-free sector. Taking into account a disordered boundary results in an interaction that is effectively random. While we find that in a strained nearest-neighbor Kitaev honeycomb model it is unlikely to find the Sachdev-Ye-Kitaev model, it appears possible to realize a bipartite variant with similar properties. We furthermore argue that next-nearest-neighbor terms can lead to actual Sachdev-Ye-Kitaev physics, if large enough.
We consider the quasi-two-dimensional pseudo-spin-1/2 Kitaev - Heisenberg model proposed for A2IrO3 (A=Li, Na) compounds. The spin-wave excitation spectrum, the sublattice magnetization, and the transition temperatures are calculated in the random phase approximation (RPA) for four different ordered phases, observed in the parameter space of the model: antiferomagnetic, stripe, ferromagnetic, and zigzag phases. The N{e}el temperature and temperature dependence of the sublattice magnetization are compared with the experimental data on Na2IrO3.
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The S=3/2 Kitaev honeycomb model (KHM) has defied an analytical as well as numerical understanding because it is not exactly soluble like its S=1/2 brethren and in contrast to other spin-S Kitaev models numerical methods are plagued by a massive pile up of low energy states. Here, we uncover the phase diagram of the S=3/2 KHM and find gapped and gapless quantum spin liquids (QSLs) generally coexisting with spin quadrupolar orders. Employing an SO(6) Majorana fermion representation of spin-3/2s, we find an exact representation of the conserved plaquette fluxes in terms of static Z$_2$ gauge fields akin to the S=1/2 KHM which enables us to treat the remaining interacting matter fermion sector in a parton mean-field theory. The latter provides an explanation for the extensive near degeneracy of low energy states in the gapless phase via the appearance of almost flat Majorana bands close to zero energy. Our parton description is in remarkable quantitative agreement with numerical simulations using the density matrix renormalization group method, and is furthermore corroborated by the addition of a single ion anisotropy which continuously connects the gapless Dirac QSL of our model with that of the S=1/2 KHM. We discuss the implications of our findings for materials realization of higher S=3/2 KHMs and the stability of the QSL phase with respect to additional interactions.
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