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Register a new userSpin Fluctuations from Hertz to Terahertz on a Triangular Lattice
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The temporal magnetic correlations of the triangular lattice antiferromagnet NiGa$_2$S$_4$ are examined through thirteen decades ($10^{-13}-1$~sec) using ultra-high-resolution inelastic neutron scattering, muon spin relaxation, AC and nonlinear susceptibility measurements. Unlike the short-ranged {it spatial} correlations, the temperature dependence of the {it temporal} correlations show distinct anomalies. The spin fluctuation rate decreases precipitously upon cooling towards $T^{ast}=8.5$~K, but fluctuations on the microsecond time scale then persist in an anomalous dynamical regime for 4 K $<Tle T^{ast}$. As this time scale exceeds that of single site dynamics by six orders of magnitude, these fluctuations bear evidence of emergent degrees of freedom within the short-range correlated incommensurate state of NiGa$_2$S$_4$.
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We calculate the fermionic spectral function $A_k (omega)$ in the spiral spin-density-wave (SDW) state of the Hubbard model on a quasi-2D triangular lattice at small but finite temperature $T$. The spiral SDW order $Delta (T)$ develops below $T = T_N$ and has momentum ${ bf K} = (4pi/3,0)$. We pay special attention to fermions with momenta ${bf k}$, for which ${bf k}$ and ${bf k} + {bf K}$ are close to Fermi surface in the absence of SDW. At the mean field level, $A_k (omega)$ for such fermions has peaks at $omega = pm Delta (T)$ at $T < T_N$ and displays a conventional Fermi liquid behavior at $T > T_N$. We show that this behavior changes qualitatively beyond mean-field due to singular self-energy contributions from thermal fluctuations in a quasi-2D system. We use a non-perturbative eikonal approach and sum up infinite series of thermal self-energy terms. We show that $A_k (omega)$ shows peak/dip/hump features at $T < T_N$, with the peak position at $Delta (T)$ and hump position at $Delta (T=0)$. Above $T_N$, the hump survives up to $T = T_p > T_N$, and in between $T_N$ and $T_p$ the spectral function displays the pseudogap behavior. We show that the difference between $T_p$ and $T_N$ is controlled by the ratio of in-plane and out-of-plane static spin susceptibilities, which determines the combinatoric factors in the diagrammatic series for the self-energy. For certain values of this ratio, $T_p = T_N$, i.e., the pseudogap region collapses. In this last case, thermal fluctuations are logarithmically singular, yet they do not give rise to pseudogap behavior. Our computational method can be used to study pseudogap physics due to thermal fluctuations in other systems.
The S=2 anisotropic triangular lattice alpha-NaMnO2 is studied by neutron inelastic scattering. Antiferromagnetic order occurs at T ~ 45 K with opening of a spin gap. The spectral weight of the magnetic dynamics above the gap (Delta ~ 7.5 meV) has been analysed by the single-mode approximation. Excellent agreement with the experiment is achieved when a dominant exchange interaction (|J|/k_B ~ 73 K), along the monoclinic b-axis and a sizeable easy-axis magnetic anisotropy (|D|/k_B ~ 3 K) are considered. Despite earlier suggestions for two-dimensional spin interactions, the dynamics illustrate strongly coupled antiferromagnetic S=2 chains and cancellation of the interchain exchange due to the lattice topology. alpha-NaMnO2 therefore represents a model system where the geometric frustration is resolved through the lowering of the dimensionality of the spin interactions.
Broad interest in quantum spin liquid (QSL) phases was triggered by the notion that they can be viewed as insulating phases with preexisting electron-pairs, such that upon light doping they might automatically yield superconductivity. Yet despite intense efforts, definitive evidence is lacking. We address the problem of a lightly doped QSL through a large-scale density-matrix renormalization group study of the $t$-$J$ model on the triangular lattice with a small but non-zero concentration of doped holes. The ground state is consistent with a Luther-Emery liquid with power-law superconducting and charge-density-wave correlations associated with partially-filled charge stripes. In particular, the superconducting correlations are dominant on both four-leg and six-leg cylinders at all hole doping concentrations. Our results provide direct evidences that doping a QSL can naturally lead to robust superconductivity.
We investigated the spin dynamics by electron spin resonance (ESR) of the Yb-based, effective spin-1/2 delafossites NaYbO$_{2}$, AgYbO$_{2}$, LiYbS$_{2}$, NaYbS$_{2}$, and NaYbSe$_{2}$ which all show an absence of magnetic order down to lowest reachable temperatures and thus are prime candidates to host a quantum spin-liquid ground state in the vicinity of long range magnetic order. Clearly resolved ESR spectra allow to obtain well-defined $g$ values which are determined by the crystal field of the distorted octahedral surrounding of the Yb-ions in trigonal symmetry. This local crystal field information provides important input to characterize the effective $S = 1/2$ Kramers doublet as well as the anisotropic exchange coupling between the Yb ions which is crucial for the nature of the groundstate. The ESR linewidth $Delta B$ is characterised by the spin dynamics and is mainly determined by the anisotropic exchange coupling. We discuss and compare $Delta B$ of the above mentioned delafossites focussing on the low temperature behaviour which is dominated by the growing influence of spin correlations.
We study the effects of quantum fluctuations on the dynamical generation of a gap and on the evolution of the spin-wave spectra of a frustrated magnet on a triangular lattice with bond-dependent Ising couplings, analog of the Kitaev honeycomb model. The quantum fluctuations lift the subextensive degeneracy of the classical ground-state manifold by a quantum order-by-disorder mechanism. Nearest-neighbor chains remain decoupled and the surviving discrete degeneracy of the ground state is protected by a hidden model symmetry. We show how the four-spin interaction, emergent from the fluctuations, generates a spin gap shifting the nodal lines of the linear spin-wave spectrum to finite energies.
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