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Register a new userClassical effect for enhanced high harmonic yield in ultrashort laser pulses with a moderate laser intensity
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We study the influence of the pulse duration on high harmonic generation (HHG) with exploring a wide laser-parameter region theoretically. Previous studies have showed that for high laser intensities near to the saturation ionization intensity, the HHG inversion efficiency is higher for shorter pulses since the ground-state depletion is weaker in the latter. Surprisingly, our simulations show this high efficiency also appears even for a moderate laser intensity at which the ionization is not strong. A classical effect relating to shorter travel distances of the rescattering electron in shorter pulses, is found to contribute importantly to this high efficiency. The effect can be amplified significantly as a two-color laser field is used, suggesting an effective approach for increasing the HHG yield.
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The dispersion scan (d-scan) technique has emerged as a simple-to-implement characterization method for ultrashort laser pulses. D-scan traces are intuitive to interpret and retrieval algorithms that are both fast and robust have been developed to obtain the spectral phase and the temporal pulse profile. Here, we give a review of the d-scan technique based on second harmonic generation. We describe and compare recent implementations for the characterization of few- and multi-cycle pulses as well as two different approaches for recording d-scan traces in single-shot, thus showing the versatility of the technique.
We study a model for frustrated tunneling ionization using ultrashort laser pulses. The model is based on the strong field approximation and it employs the saddle point approximation to predict quasiclassical trajectories that are captured on Rydberg states. We present a classification of the saddle-point solutions and explore their behavior as functions of angular momentum of the final state, as well as the carrier--envelope phase (CEP) of the laser pulse. We compare the final state population computed by the model to results obtained by numerical propagation of the time-dependent Schrodinger equation (TDSE) for the hydrogen atom. While we find qualitative agreement in the CEP dependence of the populations in principal quantum numbers, $n$, the populations to individual angular momentum channels, $ell$, are found to be inconsistent between model and TDSE. Thus, our results show that improvements of the quasiclassical trajectories are in order for a quantitative model of frustrated tunneling ionizaiton.
The acceleration of super-heavy ions (SHIs) from plasmas driven by ultrashort (tens of femtoseconds) laser pulses is a challenging topic waiting for breakthrough. The detecting and controlling of the ionization process, and the adoption of the optimal acceleration scheme are crucial for the generation of highly energetic SHIs. Here, we report the experimental results on the generation of deeply ionized super-heavy ions (Au) with unprecedented energy of 1.2 GeV utilizing ultrashort laser pulses (22 fs) at the intensity of 10^22 W/cm2. A novel self-calibrated diagnostic method was developed to acquire the absolute energy spectra and charge state distributions of Au ions abundant at the charge state of 51+ and reaching up to 61+. The measured charge state distributions supported by 2D particle-in-cell simulations serves as an additional tool to inspect the ionization dynamics associated with SHI acceleration, revealing that the laser intensity is the crucial parameter for the acceleration of Au ions over the pulse duration. The use of double-layer targets results in a prolongation of the acceleration time without sacrificing the strength of acceleration field, which is highly favorable for the generation of high-energy super heavy ions.
An ideal plasma lens can provide the focusing power of a small f-number, solid-state focusing optic at a fraction of the diameter. An ideal plasma lens, however, relies on a steady-state, linear laser pulse-plasma interaction. Ultrashort multi-petawatt (MPW) pulses possess broad bandwidths and extreme intensities, and, as a result, their interaction with the plasma lens is neither steady state nor linear. Here we examine nonlinear and time-dependent modifications to plasma lens focusing, and show that these result in chromatic and phase aberrations and amplitude distortion. We find that a plasma lens can provide enhanced focusing for 30 fs pulses with peak power up to ~1 PW. The performance degrades through the MPW regime, until finally a focusing penalty is incurred at ~10 PW.
We show that high-order harmonics generated from molecules by intense laser pulses can be expressed as the product of a returning electron wave packet and the photo-recombination cross section (PRCS) where the electron wave packet can be obtained from simple strong-field approximation (SFA) or from a companion atomic target. Using these wave packets but replacing the PRCS obtained from SFA or from the atomic target by the accurate PRCS from molecules, the resulting HHG spectra are shown to agree well with the benchmark results from direct numerical solution of the time-dependent Schrodinger equation, for the case of H$_2^+$ in laser fields. The result illustrates that these powerful theoretical tools can be used for obtaining high-order harmonic spectra from molecules. More importantly, the results imply that the PRCS extracted from laser-induced HHG spectra can be used for time-resolved dynamic chemical imaging of transient molecules with temporal resolutions down to a few femtoseconds.
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