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Spin-polarized supercurrents for spintronics: a review of current progress

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 Added by Matthias Eschrig
 Publication date 2015
  fields Physics
and research's language is English
 Authors M. Eschrig




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During the past 15 years a new field has emerged, which combines superconductivity and spintronics, with the goal to pave a way for new types of devices for applications combining the virtues of both by offering the possibility of long-range spin-polarized supercurrents. Such supercurrents constitute a fruitful basis for the study of fundamental physics as they combine macroscopic quantum coherence with microscopic exchange interactions, spin selectivity, and spin transport. This report follows recent developments in the controlled creation of long-range equal-spin triplet supercurrents in ferromagnets and its contribution to spintronics. The mutual proximity-induced modification of order in superconductor-ferromagnet hybrid structures introduces in a natural way such evasive phenomena as triplet superconductivity, odd-frequency pairing, Fulde-Ferrell-Larkin-Ovchinnikov pairing, long-range equal-spin supercurrents, $pi$-Josephson junctions, as well as long-range magnetic proximity effects. All these effects were rather exotic before 2000, when improvements in nanofabrication and materials control allowed for a new quality of hybrid structures. Guided by pioneering theoretical studies, experimental progress evolved rapidly, and since 2010 triplet supercurrents are routinely produced and observed. We have entered a new stage of studying new phases of matter previously out of our reach, and of merging the hitherto disparate fields of superconductivity and spintronics to a new research direction: super-spintronics.



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116 - Roland Grein , Tomas Lofwander , 2013
We discuss the Josephson effect in strongly spin-polarized ferromagnets where triplet correlations are induced by means of spin-active interface scattering, extending our earlier work [Phys. Rev. Lett. 102, 227005 (2009)] by including impurity scattering in the ferromagnetic bulk and the inverse proximity effect in a fully self-consistent way. Our quasiclassical approach accounts for the differences of Fermi momenta and Fermi velocities between the two spin bands of the ferromagnet, and thereby overcomes an important short-coming of previous work within the framework of Usadel theory. We show that non-magnetic disorder in conjunction with spin-dependent Fermi velocities may induce a reversal of the spin-current as a function of temperature.
We propose a mechanism whereby spin supercurrents can be manipulated in superconductor/ferromagnet proximity systems via nonequilibrium spin injection. We find that if a spin supercurrent exists in equilibrium, a nonequilibrium spin accumulation will exert a torque on the spins transported by this current. This interaction causes a new spin supercurrent contribution to manifest out of equilibrium, which is proportional to and polarized perpendicularly to both the injected spins and equilibrium spin current. This is interesting for several reasons: as a fundamental physical effect; due to possible applications as a way to control spin supercurrents; and timeliness in light of recent experiments on spin injection in proximitized superconductors.
Here, we present a study on Si(111)/-Ta($150$AA )/-IrMn($150$AA )/-NiFe($50$AA )/-Nb($x$)/-NiFe($50$AA )/-Ta($50$AA ) and Si(111)/-Ta($150$AA )/-NiFe($50$AA )/-Nb($x$)/-NiFe($50$AA )/-IrMn($150$AA )/-Ta($50$AA ) spin-valves with $x=100$ to $500$AA . For both sample families, above a specific critical thickness of the Nb-layer and below $T_c$, the superconducting Nb-layer contributes strongly to the magnetization. These systems show an anomalous hysteresis loop in the magnetization of the superconducting layer; the hysteresis loop is similar to what is generally expected from hard superconductors and many superconductor/ferromagnet hybrid systems, but the direction of the hysteresis loop is inverted, compared to what is generally observed (paramagnetic for up sweeping fields and diamagnetic for down sweeping fields). This means that the respective samples exhibit a magnetization, which is contrary to what should be expected from the Lenz rule.
We report that spin supercurrents in magnetic superconductors and superconductor/ferromagnetic insulator bilayers can induce the Dzyaloshinskii-Moriya interaction which strength is proportional to the superconducting order parameter amplitude. This effect leads to the existence of inhomogeneous parity-breaking ground states combining the chiral magnetic helix and the pair density wave orders. The formation of such states takes place via the penetration of chiral domain walls at the threshold temperature below the superconducting transition. We find regimes with both the single and the re-entrant transitions into the inhomogeneous states with decreasing temperature. The predicted hybrid chiral states can be found in the existing structures with realistic parameters and materials combinations.
The spin valve effect for the superconducting current based on the superconductor/ferromagnet proximity effect has been studied for a CoO_x/Fe1/Cu/Fe2/Cu/Pb multilayer. The magnitude of the effect $Delta T_c$ = T_c^{AP} - T_c^{P}, where T_c^{P} and T_c^{AP} are the superconducting transition temperatures for the parallel (P) and antiparallel (AP) orientation of magnetizations, respectively, has been measured for different thicknesses of the Fe1 layer d_{Fe1}. The obtained dependence of the effect on d_{Fe1} reveals that $Delta T_c$ can be increased in comparison with the case of a half-infinite Fe1 layer considered by the previous theory. A maximum of the spin valve effect occurs at d_{Fe1} ~ d_{Fe2}. At the optimal value of d_{Fe1}, almost full switching from the normal to the superconducting state when changing the mutual orientation of magnetizations of the iron layers Fe1 and Fe2 from P to AP is demonstrated.
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