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Power Law Liquid - A Unified Form of Low-Energy Nodal Electronic Interactions in Hole Doped Cuprate Superconductors

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 Added by Daniel Dessau
 Publication date 2015
  fields Physics
and research's language is English




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The strange-metal phase of the cuprate high temperature superconductors, above where the superconductivity sets in as a function of temperature, is widely considered more exotic and mysterious than the superconductivity itself. Here, based upon detailed angle resolved photoemission spectroscopy measurements of Bi$_2$Sr$_2$CaCu$_2$O$_8$$_+$$_delta$ over a wide range of doping levels, we present a new unifying phenomenology for the non-Fermi liquid normal-state interactions (scattering rates) in the nodal direction. This new phenomenology has a continuously varying power law exponent (hence named a Power Law Liquid or PLL), which with doping varies smoothly from a quadratic Fermi Liquid to a linear Marginal Fermi Liquid and beyond. Using the extracted PLL parameters we can calculate the optics and resistivity over a wide range of doping and normal-state temperature values, with the results closely matching the experimental curves. This agreement includes the presence of the $$pseudogap$$ temperature scale observed in the resistivity curves including the apparent quantum critical point. This breaks the direct link to the pseudogapping of antinodal spectral weight observed at similar (but here argued to be different) temperature scales, and also gives a new direction for searches of the microscopic mechanism at the heart of these and perhaps many other non-Fermi-liquid systems.



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The superconductivity of cuprates, which has been a mystery ever since its discovery decades ago, is created through doping electrons or holes into a Mott insulator. There, however, exists an inherent electron-hole asymmetry in cuprates. The layered crystal structures of cuprates enable collective charge excitations fundamentally different from those of three-dimensional metals, i.e., acoustic plasmons. Acoustic plasmons have been recently observed in electron-doped cuprates by resonant inelastic X-ray scattering (RIXS); in contrast, there is no evidence for acoustic plasmons in hole-doped cuprates, despite extensive measurements. This contrast led us to investigate whether the doped holes in cuprates La$_{2-x}$Sr$_x$CuO$_4$ are conducting carriers or are too incoherent to induce collective charge excitation. Here we present momentum-resolved RIXS measurements and calculations of collective charge response via the loss function to reconcile the aforementioned issues. Our results provide unprecedented spectroscopic evidence for the acoustic plasmons and long sought conducting p holes in hole-doped cuprates.
Hole-doped cuprate high temperature superconductors have ushered in the modern era of high temperature superconductivity (HTS) and have continued to be at center stage in the field. Extensive studies have been made, many compounds discovered, voluminous data compiled, numerous models proposed, many review articles written, and various prototype devices made and tested with better performance than their nonsuperconducting counterparts. The field is indeed vast. We have therefore decided to focus on the major cuprate materials systems that have laid the foundation of HTS science and technology and present several simple scaling laws that show the systematic and universal simplicity amid the complexity of these material systems, while referring readers interested in the HTS physics and devices to the review articles. Developments in the field are mostly presented in chronological order, sometimes with anecdotes, in an attempt to share some of the moments of excitement and despair in the history of HTS with readers, especially the younger ones.
A microscopic theory for electronic spectrum of the CuO2 plane within an effective p-d Hubbard model is proposed. Dyson equation for the single-electron Green function in terms of the Hubbard operators is derived which is solved self-consistently for the self-energy evaluated in the noncrossing approximation. Electron scattering on spin fluctuations induced by kinematic interaction is described by a dynamical spin susceptibility with a continuous spectrum. Doping and temperature dependence of electron dispersions, spectral functions, the Fermi surface and the coupling constant are studied in the hole doped case. At low doping, an arc-type Fermi surface and a pseudogap in the spectral function are observed.
We have computed alpha^2Fs for the hole-doped cuprates within the framework of the one-band Hubbard model, where the full magnetic response of the system is treated properly. The d-wave pairing weight alpha^2F_d is found to contain not only a low energy peak due to excitations near (pi,pi) expected from neutron scattering data, but to also display substantial spectral weight at higher energies due to contributions from other parts of the Brillouin zone as well as pairbreaking ferromagnetic excitations at low energies. The resulting solutions of the Eliashberg equations yield transition temperatures and gaps comparable to the experimentally observed values, suggesting that magnetic excitations of both high and low energies play an important role in providing the pairing glue in the cuprates.
A residual linear term is observed in the thermal conductivity of optimally-doped Bi-2212 at very low temperatures whose magnitude is in excellent agreement with the value expected from Fermi-liquid theory and the d-wave energy spectrum measured by photoemission spectroscopy, with no adjustable parameters. This solid basis allows us to make a quantitative analysis of thermodynamic properties at low temperature and establish that thermally-excited quasiparticles are a significant, perhaps even the dominant mechanism in suppressing the superfluid density in cuprate superconductors Bi-2212 and YBCO.
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