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Register a new userVisualizing the evolution from the Mott insulator to a charge ordered insulator in lightly doped cuprates
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A central question in the high temperature cuprate superconductors is the fate of the parent Mott insulator upon charge doping. Here we use scanning tunneling microscopy to investigate the local electronic structure of lightly doped cuprate in the antiferromagnetic insulating regime. We show that the doped charge induces a spectral weight transfer from the high energy Hubbard bands to the low energy in-gap states. With increasing doping, a V-shaped density of state suppression occurs at the Fermi level, which is accompanied by the emergence of checkerboard charge order. The new STM perspective revealed here is the cuprates first become a charge ordered insulator upon doping. Subsequently, with further doping, Fermi surface and high temperature superconductivity grow out of it.
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Because the cuprate superconductors are doped Mott insulators, it would be advantageous to solve even a toy model that exhibits both Mottness and superconductivity. We consider the Hatsugai-Kohmoto model, an exactly solvable system that is a prototypical Mott insulator above a critical interaction strength at half filling. Upon doping or reducing the interaction strength, our exact calculations show that the system becomes a non-Fermi liquid metal with a superconducting instability. In the presence of a weak pairing interaction, the instability produces a thermal transition to a superconducting phase, which is distinct from the BCS state, as evidenced by a gap-to-transition temperature ratio exceeding the universal BCS limit. The elementary excitations of this superconductor are not Bogoliubov quasiparticles but rather superpositions of doublons and holons, composite excitations signaling that the superconducting ground state of the doped Mott insulator inherits the non-Fermi liquid character of the normal state. An unexpected feature of this model is that it exhibits a superconductivity-induced transfer of spectral weight from high to low energies as seen in the cuprates as well as a suppression of the superfluid density relative to that in BCS theory.
We present a systematic study of spin dynamics in a superconducting ground state, which itself is a doped-Mott-insulator and can correctly reduce to an antiferromagnetic (AF) state at half-filling with an AF long-range order (AFLRO). Such a doped Mott insulator is described by a mean-field theory based on the phase string formulation of the t-J model. We show that the spin wave excitation in the AFLRO state at half-filling evolves into a resonancelike peak at a finite energy in the superconducting state, which is located around the AF wave vectors. The width of such a resonancelike peak in momentum space decides a spin correlation length scale which is inversely proportional to the square root of doping concentration, while the energy of the resonancelike peak scales linearly with the doping concentration at low doping. An important prediction of the theory is that, while the total spin sum rule is satisfied at different doping concentrations, the weight of the resonancelike peak does not vanish, but is continuously saturated to the weight of the AFLRO at zero-doping limit. Besides the low-energy resonancelike peak, we also show that the high-energy excitations still track the spin wave dispersion in momentum space, contributing to a significant portion of the total spin sum rule. The fluctuational effect beyond the mean-field theory is also examined, which is related to the broadening of the resonancelike peak in energy space. In particular, we discuss the incommensurability of the spin dynamics by pointing out that its visibility is strongly tied to the low-energy fluctuations below the resonancelike peak. We finally investigate the interlayer coupling effect on the spin dynamics as a function of doping, by considering a bilayer system.
By studying the optical conductivity of BSLCO and YCBCO, we show that the metal-to-insulator transition (MIT) in these hole-doped cuprates is driven by the opening of a small gap at low T in the far infrared. Its width is consistent with the observations of Angle-Resolved Photoemission Spectroscopy in other cuprates, along the nodal line of the k-space. The gap forms as the Drude term turns into a far-infrared absorption, whose peak frequency can be approximately predicted on the basis of a Mott-like transition. Another band in the mid infrared softens with doping but is less sensitive to the MIT.
The low-energy excitations of the lightly doped cuprates were studied by angle-resolved photoemission spectroscopy. A finite gap was measured over the entire Brillouin zone, including along the d_{x^2 - y^2} nodal line. This effect was observed to be generic to the normal states of numerous cuprates, including hole-doped La_{2-x}Sr_{x}CuO_{4} and Ca_{2-x}Na_{x}CuO_{2}Cl_{2} and electron-doped Nd_{2-x}Ce_{x}CuO_{4}. In all compounds, the gap appears to close with increasing carrier doping. We consider various scenarios to explain our results, including the possible effects of chemical disorder, electronic inhomogeneity, and a competing phase.
The formation of domains comprising alternating hole rich and hole poor ladders recently observed by Scanning Tunneling Microscopy by Kohsaka et al., on lightly hole doped cuprates, is interpreted in terms of an attractive mechanism which favors the presence of doped holes on Cu sites located each on one side of an oxygen atom. This mechanism leads to a geometrical pattern of alternating hole-rich and hole-poor ladders with a periodicity equal to 4 times the lattice spacing in the CuO plane, as observed experimentally. To cite this article: G. Deutscher, P.-G. de Gennes, C. R. Physique 8 (2007).
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