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We introduce the concept of nonlinear graphene metasurfaces employing the controllable interaction between a graphene layer and a planar metamaterial. Such hybrid metasurfaces support two types of subradiant resonant modes, asymmetric modes of structured metamaterial elements (metamolecules) and graphene plasmons exhibiting strong mutual coupling and avoided dispersion crossing. High tunability of graphene plasmons facilitates strong interaction between the subradiant modes, modifying the spectral position and lifetime of the associated Fano resonances. We demonstrate that strong resonant interaction, combined with the subwavelength localization of plasmons, leads to the enhanced nonlinear response and high efficiency of the second-harmonic generation.
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Artificial magnetic fields are revolutionizing our ability to manipulate neutral particles, by enabling the emulation of exotic phenomena once thought to be exclusive to charged particles. In particular, pseudo-magnetic fields generated by nonuniform strain in artificial lattices have attracted considerable interest because of their simple geometrical origin. However, to date, these strain-induced pseudo-magnetic fields have failed to emulate the tunability of real magnetic fields because they are dictated solely by the strain configuration. Here, we overcome this apparent limitation for polaritons supported by strained metasurfaces, which can be realized with classical dipole antennas or quantum dipole emitters. Without altering the strain configuration, we unveil how one can tune the pseudo-magnetic field by modifying the electromagnetic environment via an enclosing photonic cavity which modifies the nature of the interactions between the dipoles. Remarkably, due to the competition between short-range Coulomb interactions and long-range photon-mediated interactions, we find that the pseudo-magnetic field can be entirely switched off at a critical cavity height for any strain configuration. Consequently, by varying only the cavity height, we demonstrate a tunable Lorentz-like force that can be switched on/off and an unprecedented collapse and revival of polariton Landau levels. Unlocking this tunable pseudo-magnetism for the first time poses new intriguing questions beyond the paradigm of conventional tight-binding physics.
Coherent perfect absorber (CPA) was proposed as the time-reversed counterpart to laser: a resonator containing lossy medium instead of gain medium can absorb the coherent optical fields completely. Here, we exploit a monolayer graphene to realize the CPA in a non-resonant manner. It is found that quasi-CPA point exists in the terahertz regime for suspending monolayer graphene, and the CPA can be implemented with the assistant of proper phase modulation among two incident beams at the quasi-CPA frequencies. The graphene based CPA is found of broadband angular selectivity: CPA point splits into two frequency bands for the orthogonal $s$ and $p$ polarizations at oblique incidence, and the two bands cover a wide frequency range starting from zero frequency. Furthermore, the coherent absorption can be tuned substantially by varying the gate-controlled Fermi energy. The findings of CPA with non-resonant graphene sheet can be generalized for potential applications in terahertz/infrared detections and signal processing with two-dimensional optoelectronic materials.
We exploited graphene nanoribbons based meta-surface to realize coherent perfect absorption (CPA) in the mid-infrared regime. It was shown that quasi-CPA frequencies, at which CPA can be demonstrated with proper phase modulations, exist for the graphene meta-surface with strong resonant behaviors. The CPA can be tuned substantially by merging the geometric design of the meta-surface and the electrical tunability of graphene. Furthermore, we found that the graphene nanoribbon meta-surface based CPA is realizable with experimental graphene data. The findings of CPA with graphene meta-surface can be generalized for potential applications in optical detections and signal processing with two-dimensional optoelectronic materials.
Nonlinear optics is an increasingly important field for scientific and technological applications, owing to its relevance and potential for optical and optoelectronic technologies. Currently, there is an active search for suitable nonlinear material systems with efficient conversion and small material footprint. Ideally, the material system should allow for chip-integration and room-temperature operation. Two-dimensional materials are highly interesting in this regard. Particularly promising is graphene, which has demonstrated an exceptionally large nonlinearity in the terahertz regime. Yet, the light-matter interaction length in two-dimensional materials is inherently minimal, thus limiting the overall nonlinear-optical conversion efficiency. Here we overcome this challenge using a metamaterial platform that combines graphene with a photonic grating structure providing field enhancement. We measure terahertz third-harmonic generation in this metamaterial and obtain an effective third-order nonlinear susceptibility with a magnitude as large as 3$cdot$10$^{-8}$m$^2$/V$^2$, or 21 esu, for a fundamental frequency of 0.7 THz. This nonlinearity is 50 times larger than what we obtain for graphene without grating. Such an enhancement corresponds to third-harmonic signal with an intensity that is three orders of magnitude larger due to the grating. Moreover, we demonstrate a field conversion efficiency for the third harmonic of up to $sim$1% using a moderate field strength of $sim$30 kV/cm. Finally we show that harmonics beyond the third are enhanced even more strongly, allowing us to observe signatures of up to the 9$^{rm th}$ harmonic. Grating-graphene metamaterials thus constitute an outstanding platform for commercially viable, CMOS compatible, room temperature, chip-integrated, THz nonlinear conversion applications.
Hexagonal boron nitride (hBN) is a natural hyperbolic material which can also accommodate highly dispersive surface phonon-polariton modes. In this paper, we examine theoretically the mid-infrared optical properties of graphene-hBN heterostructures derived from their coupled plasmon-phonon modes. We found that the graphene plasmon couples differently with the phonons of the two Reststrahlen bands, owing to their different hyperbolicity. This also leads to distinctively different interaction between an external quantum emitter and the plasmon-phonon modes in the two bands, leading to substantial modification of its spectrum. The coupling to graphene plasmons allows for additional gate tunability in the Purcell factor, and narrow dips in its emission spectra.
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