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Register a new userElastic Cheerios effect: self-assembly of cylinders on a soft solid
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A rigid cylinder placed on a soft gel deforms its surface. When multiple cylinders are placed on the surface, they interact with each other via the topography of the deformed gel which serves as an energy landscape; as they move, the landscape changes which in turn changes their interaction. We use a combination of experiments, simple scaling estimates and numerical simulations to study the self-assembly of cylinders in this elastic analog of the Cheerios effect for capillary interactions on a fluid interface. Our results show that the effective two body interaction can be well described by an exponential attraction potential as a result of which the dynamics also show an exponential behavior with respect to the separation distance. When many cylinders are placed on the gel, the cylinders cluster together if they are not too far apart; otherwise their motion gets elastically arrested.
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Soft electroactive materials can undergo large deformation subjected to either mechanical or electrical stimulus, and hence they can be excellent candidates for designing extremely flexible and adaptive structures and devices. This paper proposes a simple one-dimensional soft phononic crystal cylinder made of dielectric elastomer to show how large deformation and electric field can be used jointly to tune the longitudinal waves propagating in the PC. A series of soft electrodes are placed periodically along the dielectric elastomer cylinder, and hence the material can be regarded as uniform in the undeformed state. This is also the case for the uniformly pre-stretched state induced by a static axial force only. The effective periodicity of the structure is then achieved through two loading paths, i.e. by maintaining the longitudinal stretch and applying an electric voltage over any two neighbouring electrodes, or by holding the axial force and applying the voltage. All physical field variables for both configurations can be determined exactly based on the nonlinear theory of electroelasticity. An infinitesimal wave motion is further superimposed on the pre-deformed configurations and the corresponding dispersion equations are derived analytically by invoking the linearized theory for incremental motions. Numerical examples are finally considered to show the tunability of wave propagation behavior in the soft PC cylinder. The outstanding performance regarding the band gap (BG) property of the proposed soft dielectric PC is clearly demonstrated by comparing with the conventional design adopting the hard piezoelectric material. Note that soft dielectric PCs are susceptible to various kinds of failure (buckling, electromechanical instability, electric breakdown, etc.), imposing corresponding limits on the external stimuli.
Spontaneous self-assembly in molecular systems is a fundamental route to both biological and engineered soft matter. Simple micellisation, emulsion formation, and polymer mixing principles are well understood. However, the principles behind emergence of structures with competing length scales in soft matter systems remain an open question. Examples include the droplet-inside-droplet assembly in many biomacromolecular systems undergoing liquid-liquid phase separation, analogous multiple emulsion formation in oil-surfactant-water formulations, and polymer core-shell particles with internal structure. We develop here a microscopic theoretical model based on effective interactions between the constituents of a soft matter system to explain self-organization both at single and multiple length scales. The model identifies how spatial ordering at multiple length scales emerges due to competing interactions between the system components, e.g. molecules of different sizes and different chemical properties. As an example of single and multiple-length-scale assembly, we map out a generic phase diagram for a solution with two solute species differing in their mutual and solvent interactions. By performing molecular simulations on a block-copolymer system, we further demonstrate how the phase diagram can be connected to a molecular system that has a transition from regular single-core polymer particles to multi-core aggregates that exhibit multiple structural length scales. The findings provide guidelines to understanding the length scales rising spontaneously in biological self-assembly, but also open new venues to the development and engineering of biomolecular and polymeric functional materials.
We report measurements of elastic moduli of hcp solid $^4$He down to 15 mK when the samples are rotated unidirectionally. Recent investigations have revealed that the elastic behavior of solid $^4$He is dominated by gliding of dislocations and pinning of them by $^3$He impurities, which move in the solid like Bloch waves (impuritons). Motivated by the recent controversy of torsional oscillator studies, we have preformed direct measurements of shear and Youngs moduli of annular solid $^4$He using pairs of quarter-circle shape piezoelectric transducers (PZTs) while the whole apparatus is rotated with angular velocity $Omega$ up to 4 rad/s. We have found that shear modulus $mu$ is suppressed by rotation below 80 mK, when shear strain applied by PZT exceeds a critical value, above which $mu$ decreases because the shear strain unbinds dislocations from $^3$He impurities. The rotation - induced decrement of $mu$ at $Omega = 4$ rad/s is about 14.7 (12.3) % of the total change of temperature dependent $mu$ for solid samples of pressure 3.6 (5.4) MPa. The decrements indicate that the probability of pinning of $^3$He on dislocation segment, $G$, decreases by several orders of magnitude. We propose that the motion of $^3$He impuritons under rotation becomes strongly anisotropic by the Coriolis force, resulting a decrease in $G$ for dislocation lines aligning parallel to the rotation axis.
The protein shells, or capsids, of all sphere-like viruses adopt icosahedral symmetry. In the present paper we propose a statistical thermodynamic model for viral self-assembly. We find that icosahedral symmetry is not expected for viral capsids constructed from structurally identical protein subunits and that this symmetry requires (at least) two internal switching configurations of the protein. Our results indicate that icosahedral symmetry is not a generic consequence of free energy minimization but requires optimization of internal structural parameters of the capsid proteins.
Our understanding of the elasticity and rheology of disordered materials, such as granular piles, foams, emulsions or dense suspensions relies on improving experimental tools to characterize their behaviour at the particle scale. While 2D observations are now routinely carried out in laboratories, 3D measurements remain a challenge. In this paper, we use a simple model system, a packing of soft elastic spheres, to illustrate the capability of X-ray microtomography to characterise the internal structure and local behaviour of granular systems. Image analysis techniques can resolve grain positions, shapes and contact areas; this is used to investigate the materials microstructure and its evolution upon strain. In addition to morphological measurements, we develop a technique to quantify contact forces and estimate the internal stress tensor. As will be illustrated in this paper, this opens the door to a broad array of static and dynamical measurements in 3D disordered systems
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