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Register a new userSingle-Shot Electron Diffraction using a Cold Atom Electron Source
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Added by
Rory Speirs BSc(ScSchProg)(Hons)
Publication date
2015
fields
Physics
and research's language is
English
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Cold atom electron sources are a promising alternative to traditional photocathode sources for use in ultrafast electron diffraction due to greatly reduced electron temperature at creation, and the potential for a corresponding increase in brightness. Here we demonstrate single-shot, nanosecond electron diffraction from monocrystalline gold using cold electron bunches generated in a cold atom electron source. The diffraction patterns have sufficient signal to allow registration of multiple single-shot images, generating an averaged image with significantly higher signal-to-noise ratio than obtained with unregistered averaging. Reflection high-energy electron diffraction (RHEED) was also demonstrated, showing that cold atom electron sources may be useful in resolving nanosecond dynamics of nanometre scale near-surface structures.
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We present a method for producing sub-100 fs electron bunches that are suitable for single-shot ultrafast electron diffraction experiments in the 100 keV energy range. A combination of analytical results and state-of-the-art numerical simulations show that it is possible to create 100 keV, 0.1 pC, 20 fs electron bunches with a spotsize smaller than 500 micron and a transverse coherence length of 3 nm, using established technologies in a table-top set-up. The system operates in the space-charge dominated regime to produce energy-correlated bunches that are recompressed by established radio-frequency techniques. With this approach we overcome the Coulomb expansion of the bunch, providing an entirely new ultrafast electron diffraction source concept.
We propose a new concept of an electron source for ultrafast electron diffraction with sub-10~fs temporal resolution. Electrons are generated in a laser-plasma accelerator, able to deliver femtosecond electron bunches at 5 MeV energy with kHz repetition rate. The possibility of producing this electron source is demonstrated using Particle-In-Cell simulations. We then use particle tracking simulations to show that this electron beam can be transported and manipulated in a realistic beamline, in order to reach parameters suitable for electron diffraction. The beamline consists of realistic static magnetic optics and introduces no temporal jitter. We demonstrate numerically that electron bunches with 5~fs duration and containing 1.5~fC per bunch can be produced, with a transverse coherence length exceeding 2~nm, as required for electron diffraction.
Features of forward diffracted Parametric X-Radiation (PXR) were investigated at experiments with the 855 MeV electron beam of the Mainz Microtron MAMI employing a 410 micrometer thick tungsten single crystal. Virtual photons from the electron field are diffracted by the (10-1) plane at a Bragg angle of 3.977 degree. Forward emitted radiation was analyzed at an energy of 40 keV with the (111) lattice planes of a flat silicon single crystal in Bragg geometry. Clear peak structures were observed in an angular scan of the tungsten single crystal. The results were analyzed with a model which describes forward diffracted PXR under real experimental conditions. The experiments show that forward diffracted PXR may be employed to diagnose bending radii of lattice planes in large area single crystals.
Single-shot absorption measurements have been performed using the multi-keV X-rays generated by a laser wakefield accelerator. A 200 TW laser was used to drive a laser wakefield accelerator in a mode which produced broadband electron beams with a maximum energy above 1 GeV and a broad divergence of $approx15$ miliradians FWHM. Betatron oscillations of these electrons generated $1.2pm0.2times10^6$ photons/eV in the 5 keV region, with a signal-to-noise ratio of approximately 300:1. This was sufficient to allow high-resolution XANES measurements at the K-edge of a titanium sample in a single shot. We demonstrate that this source is capable of single-shot, simultaneous measurements of both the electron and ion distributions in matter heated to eV temperatures by comparison with DFT simulations. The unique combination of a high-flux, large bandwidth, few femtosecond duration X-ray pulse synchronised to a high-power laser will enable key advances in the study of ultra-fast energetic processes such as electron-ion equilibration.
Electron paramagnetic resonance (EPR) spectroscopy is an important technology in physics, chemistry, materials science, and biology. Sensitive detection with a small sample volume is a key objective in these areas, because it is crucial, for example, for the readout of a highly packed spin based quantum memory or the detection of unlabeled metalloproteins in a single cell. In conventional EPR spectrometers, the energy transfer from the spins to the cavity at a Purcell enhanced rate plays an essential role and requires the spins to be resonant with the cavity, however the size of the cavity (limited by the wavelength) makes it difficult to improve the spatial resolution. Here, we demonstrate a novel EPR spectrometer using a single artificial atom as a sensitive detector of spin magnetization. The artificial atom, a superconducting flux qubit, provides advantages both in terms of its quantum properties and its much stronger coupling with magnetic fields. We have achieved a sensitivity of $sim$400 spins/$sqrt{mathrm{Hz}}$ with a magnetic sensing volume around $10^{-14} lambda^3$ (50 femto-liters). This corresponds to an improvement of two-order of magnitude in the magnetic sensing volume compared with the best cavity based spectrometers while maintaining a similar sensitivity as those spectrometers . Our artificial atom is suitable for scaling down and thus paves the way for measuring single spins on the nanometer scale.
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