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Register a new userNonlinear Phase Control and Anomalous Phase Matching in Plasmonic Metasurfaces
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Metasurfaces, and in particular those containing plasmonic-based metallic elements, constitute a particularly attractive set of materials. By means of modern nanolithographic fabrication techniques, flat, ultrathin optical elements may be constructed. However, in spite of their strong optical nonlinearities, plasmonic metasurfaces have so far been investigated mostly in the linear regime. Here we introduce full nonlinear phase control over plasmonic elements in metasurfaces. We show that for nonlinear interactions in a phase-gradient nonlinear metasurface a new anomalous nonlinear phase matching condition prevails, which is the nonlinear analog of the generalized Snell law demonstrated for linear metasurfaces. This phase matching condition is very different from the other known phase matching schemes. The subwavelength phase control of optical nonlinearities provides a foundation for the design of flat nonlinear optical elements based on metasurfaces. Our demonstrated flat nonlinear elements (i.e. lenses) act as generators and manipulators of the frequency-converted signal.
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Motivated by the recent growing demand in dynamically-controlled flat optics, we take advantage of a hybrid phase-change plasmonic metasurface (MS) to effectively tailor the amplitude, phase, and polarization responses of the incident beam within a unique structure. Such a periodic architecture exhibits two fundamental modes; pronounced counter-propagating short-range surface plasmon polariton (SR-SPP) coupled to the Ge2Sb2Te5 (GST) alloy as the feed gap, and the propagative surface plasmon polariton (PR-SPP) resonant modes tunneling to the GST nanostripes. By leveraging the multistate phase transition of alloy from amorphous to the crystalline, which induces significant complex permittivity change, the interplay between such enhanced modes can be drastically modified. Accordingly, in the intermediate phases, the proposed system experiences a coupled condition of operational over-coupling and under-coupling regimes leading to an inherently broadband response. We wisely addressing each gate-tunable meta-atom to achieve robust control over the reflection characteristics, wide phase agility up to 315? or considerable reflectance modulation up to 60%, which facilitate a myriad of on-demand optical functionalities in the telecommunication band. Based on the revealed underlying physics and electro-thermal effects in the GST alloy, a simple systematic approach for realization of an electro-optically tunable multifunctional metadevice governing anomalous reflection angle control (e.g., phased array antenna), near-perfect absorption (e.g., modulator), and polarization conversion (e.g., wave plate) is presented. As a promising alternative to their passive counterparts, such high-speed, non-volatile MSs offer an smart paradigm for reversible, energy-efficient, and programmable optoelectronic devices such as holograms, switches, and polarimeters.
For transmissive applications of electromagnetic metasurfaces, an array of subwavelength Huygens metaatoms are typically used to eliminate reflection and achieve a high transmission power efficiency together with a wide transmission phase coverage. We show that the underlying principle of low reflection and full control over transmission is asymmetric scattering into the specular reflection and transmission directions that results from a superposition of symmetric and anti-symmetric scattering components, with Huygens meta-atoms being one example configuration. Available for oblique illumination in TM polarization, a meta-atom configuration comprising normal and tangential electric polarizations is presented, which is capable of reflectionless, fullpower transmission and a $2pi$ transmission phase coverage as well as full absorption. For lossy metasurfaces, we show that a complete phase coverage is still available for reflectionless designs for any value of absorptance. Numerical examples in the microwave and optical regimes are provided.
The nonlinear optical response of materials to exciting light is enhanced by resonances between the incident laser frequencies and the energy levels of the excited material. Traditionally, in molecular nonlinear spectroscopy one tunes the input laser frequencies to the molecular energy levels for highly enhanced doubly or triply resonant interactions. With metasurfaces the situation is different, and by proper design of the nanostructures, one may tune the material energy levels to match the incoming laser frequencies. Here we use multi-parameter genetic algorithm methodologies to optimize the nonlinear Four Wave Mixing response, and show that the intuitive conventional approach of trying to match the transmission spectrum to the relevant laser frequencies indeed leads to strong enhancement, but not necessarily to the optimal design. We demonstrate, experimentally and by direct nonlinear field calculations, that the near field mode distribution and spatial modes overlap are the dominant factor for optimized design.
Metasurfaces are optically thin metamaterials that promise complete control of the wavefront of light but are primarily used to control only the phase of light. Here, we present an approach, simple in concept and in practice, that uses meta-atoms with a varying degree of form birefringence and rotation angles to create high-efficiency dielectric metasurfaces that control both the optical amplitude and phase at one or two frequencies. This opens up applications in computer-generated holography, allowing faithful reproduction of both the phase and amplitude of a target holographic scene without the iterative algorithms required in phase-only holography. We demonstrate all-dielectric metasurface holograms with independent and complete control of the amplitude and phase at up to two optical frequencies simultaneously to generate two- and three-dimensional holographic objects. We show that phase-amplitude metasurfaces enable a few features not attainable in phase-only holography; these include creating artifact-free two-dimensional holographic images, encoding phase and amplitude profiles separately at the object plane, encoding intensity profiles at the metasurface and object planes separately, and controlling the surface textures of three-dimensional holographic objects.
Nonlinear metasurfaces that dynamically manipulate the phase of a passing light beam are of interest for a wide range of applications. The controlled operation of such devices requires accurate measurements of the optical transmission phase in both the linear and nonlinear regime, an experimentally challenging task. In this paper we show that this phase information can be extracted directly from simple transmission measurements, using a Hilbert transform approach, removing the need for complicated, interferometric experimental set-ups, and enabling direct measurements of the phase in conditions not suitable for other traditional approaches, such Z-scan measurements.
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