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Nonlinear Phase Control and Anomalous Phase Matching in Plasmonic Metasurfaces

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 Added by Yehiam Prior
 Publication date 2015
  fields Physics
and research's language is English




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Metasurfaces, and in particular those containing plasmonic-based metallic elements, constitute a particularly attractive set of materials. By means of modern nanolithographic fabrication techniques, flat, ultrathin optical elements may be constructed. However, in spite of their strong optical nonlinearities, plasmonic metasurfaces have so far been investigated mostly in the linear regime. Here we introduce full nonlinear phase control over plasmonic elements in metasurfaces. We show that for nonlinear interactions in a phase-gradient nonlinear metasurface a new anomalous nonlinear phase matching condition prevails, which is the nonlinear analog of the generalized Snell law demonstrated for linear metasurfaces. This phase matching condition is very different from the other known phase matching schemes. The subwavelength phase control of optical nonlinearities provides a foundation for the design of flat nonlinear optical elements based on metasurfaces. Our demonstrated flat nonlinear elements (i.e. lenses) act as generators and manipulators of the frequency-converted signal.

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Motivated by the recent growing demand in dynamically-controlled flat optics, we take advantage of a hybrid phase-change plasmonic metasurface (MS) to effectively tailor the amplitude, phase, and polarization responses of the incident beam within a unique structure. Such a periodic architecture exhibits two fundamental modes; pronounced counter-propagating short-range surface plasmon polariton (SR-SPP) coupled to the Ge2Sb2Te5 (GST) alloy as the feed gap, and the propagative surface plasmon polariton (PR-SPP) resonant modes tunneling to the GST nanostripes. By leveraging the multistate phase transition of alloy from amorphous to the crystalline, which induces significant complex permittivity change, the interplay between such enhanced modes can be drastically modified. Accordingly, in the intermediate phases, the proposed system experiences a coupled condition of operational over-coupling and under-coupling regimes leading to an inherently broadband response. We wisely addressing each gate-tunable meta-atom to achieve robust control over the reflection characteristics, wide phase agility up to 315? or considerable reflectance modulation up to 60%, which facilitate a myriad of on-demand optical functionalities in the telecommunication band. Based on the revealed underlying physics and electro-thermal effects in the GST alloy, a simple systematic approach for realization of an electro-optically tunable multifunctional metadevice governing anomalous reflection angle control (e.g., phased array antenna), near-perfect absorption (e.g., modulator), and polarization conversion (e.g., wave plate) is presented. As a promising alternative to their passive counterparts, such high-speed, non-volatile MSs offer an smart paradigm for reversible, energy-efficient, and programmable optoelectronic devices such as holograms, switches, and polarimeters.
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Metasurfaces are optically thin metamaterials that promise complete control of the wavefront of light but are primarily used to control only the phase of light. Here, we present an approach, simple in concept and in practice, that uses meta-atoms with a varying degree of form birefringence and rotation angles to create high-efficiency dielectric metasurfaces that control both the optical amplitude and phase at one or two frequencies. This opens up applications in computer-generated holography, allowing faithful reproduction of both the phase and amplitude of a target holographic scene without the iterative algorithms required in phase-only holography. We demonstrate all-dielectric metasurface holograms with independent and complete control of the amplitude and phase at up to two optical frequencies simultaneously to generate two- and three-dimensional holographic objects. We show that phase-amplitude metasurfaces enable a few features not attainable in phase-only holography; these include creating artifact-free two-dimensional holographic images, encoding phase and amplitude profiles separately at the object plane, encoding intensity profiles at the metasurface and object planes separately, and controlling the surface textures of three-dimensional holographic objects.
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