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Register a new userPlasma filtering techniques for nuclear waste remediation
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Nuclear waste cleanup is challenged by the handling of feed stocks that are both unknown and complex. Plasma filtering, operating on dissociated elements, offers advantages over chemical methods in processing such wastes. The costs incurred by plasma mass filtering for nuclear waste pretreatment, before ultimate disposal, are similar to those for chemical pretreatment. However, significant savings might be achieved in minimizing the waste mass. This advantage may be realized over a large range of chemical waste compositions, thereby addressing the heterogeneity of legacy nuclear waste.
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We show experimentally that the terahertz (THz) emission of a plasma, generated in air by a two-color laser pulse (containing a near IR frequency and its second harmonic), can be enhanced by the addition of an 800-nm pulse. We observed enhancements of the THz electric field by a factor of up to 30. This provides a widely accessible means for researchers using optical parametric amplifiers (OPA) to increase their THz yields by simply adding the residual pump beam of the OPA to the plasma generating beam. We investigate the dependence of the THz electric field enhancement factor on the powers of the two-color beam as well as the 800-nm enhancement beam. Numerical calculations using the well-known photocurrent model are in excellent agreement with the experimental observations.
Rare earth elements recycling has been proposed to alleviate supply risks and market volatility. In this context, the potential of a new recycling pathway, namely plasma mass separation, is uncovered through the example of nedodymium - iron - boron magnets recycling. Plasma mass separation is shown to address some of the shortcomings of existing rare earth elements recycling pathways, in particular detrimental environmental effects. A simplified mass separation model suggests that plasma separation performances could compare favourably with existing recycling options. In addition, simple energetic considerations of plasma processing suggest that the cost of these techniques may not be prohibitive, particularly considering that energy costs from solar may become significantly cheaper. Further investigation and experimental demonstration of plasma separation techniques should permit asserting the potential of these techniques against other recycling techniques currently under development.
Recently, two novel techniques for the extraction of the phase-shift map (Tomassini {it et.~al.}, Applied Optics {bf 40} 35 (2001)) and the electronic density map estimation (Tomassini P. and Giulietti A., Optics Communication {bf 199}, pp 143-148 (2001)) have been proposed. In this paper we apply both methods to a sample laser-plasma interferogram obtained with femtoseconds probe pulse, in an experimental setup devoted to laser particle acceleration studies.
Computational modeling is an important aspect of the research on nuclear waste materials. In particular, atomistic simulations, when used complementary to experimental efforts, contribute to the scientific basis of safety case for nuclear waste repositories. Here we discuss the state-of-the-art and perspectives of atomistic modeling for nuclear waste management on a few cases of successful synergy of atomistic simulations and experiments. In particular, we discuss here: (1) the potential of atomistic simulations to investigate the uranium oxidation state in mixed valence uranium oxides and (2) the ability of cementitious barrier materials to retain radionuclides such as 226Ra and 90Sr, and of studtite/metastudtite secondary peroxide phases to incorporate actinides such as Np and Am. The new contribution we make here is the computation of the incorporation of Sr by C-S-H (calcium silicate hydrate) phases.
We report the highest compression reached in laboratory plasmas using eight laser beams, E$_{laser}$$approx$12 kJ, $tau_{laser}$=2 ns in third harmonic on a CD$_2$ target at the ShenGuang-II Upgrade (SGII-Up) facility in Shanghai, China. We estimate the deuterium density $rho_D$= 2.0 $pm$ 0.9 kg/cm$^{3}$, and the average kinetic energy of the plasma ions less than 1 keV. The highest reached areal density $Lambda rho_{D}$=4.8 $pm$ 1.5 g/cm$^{2}$ was obtained from the measured ratio of the sequential ternary fusion reactions (dd$rightarrow$t+p and t+d$rightarrow$$alpha$+n) and the two body reaction fusions (dd$rightarrow$$^3$He+n). At such high densities, sequential ternary and also quaternary nuclear reactions become important as well (i.e. n(14.1 MeV) + $^{12}$C $rightarrow$ n+$^{12}$C* etc.) resulting in a shift of the neutron (and proton) kinetic energies from their birth values. The Down Scatter Ratio (DSR-quaternary nuclear reactions) method, i.e. the ratio of the 10-12MeV neutrons divided by the total number of 14.1MeV neutrons produced, confirms the high densities reported above. The estimated lifetime of the highly compressed plasma is 52 $pm$ 9 ps, much smaller than the lasers pulse duration.
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