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Register a new userThermal-Light-Induced Coherent Dynamics in Atoms and Molecules -- an Exact Quantum Mechanical Treatment
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The question of whether sunlight induces coherent dynamics in biological systems is under debate. Here we show, on the basis of an exact fully quantum mechanical treatment, that thermal light induces excited-state coherences in matter similar to those induced by a coherent state. We demonstrate the phenomenon on a V-type model system and a two-state Born-Oppenheimer molecular system. Remarkably, wavepacket-like dynamics is induced in the excited molecular potential-energy surface.
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We present a generalization of the diagrammatic pump-probe approach to coherent backscattering (CBS) of intense laser light for atoms with degenerate energy levels. We employ this approach for a characterization of the double scattering signal from optically pumped atoms with the transition $J_grightarrow J_e=J_g+1$ in the helicity preserving polarization channel. We show that, in the saturation regime, the internal degeneracy becomes manifest for atoms with $J_ggeq 1$, leading to a faster decrease of the CBS enhancement factor with increasing saturation parameter than in the non-degenerate case.
By using the coherent backscattering interference effect, we investigate experimentally and theoretically how coherent transport of light inside a cold atomic vapour is affected by the residual motion of atomic scatterers. As the temperature of the atomic cloud increases, the interference contrast dramatically decreases emphazising the role of motion-induced decoherence for resonant scatterers even in the sub-Doppler regime of temperature. We derive analytical expressions for the corresponding coherence time.
It has recently been discovered that the optical analogue of a gradient echo in an optically thick material could form the basis of a optical memory that is both completely efficient and noise free. Here we present analytical calculation showing this is the case. There is close analogy between the operation of the memory and an optical system with two beam splitters. We can use this analogy to calculate efficiencies as a function of optical depth for a number of quantum memory schemes based on controlled inhomogeneous broadening. In particular we show that multiple switching leads to a net 100% retrieval efficiency for the optical gradient echo even in the optically thin case.
We report on the modification of the optical and mechanical properties of a silicon 1D optomechanical crystal cavity due to thermo-optic effects in a high phonon/photon population regime. The cavity heats up due to light absorption in a way that shifts the optical modes towards longer wavelengths and the mechanical modes to lower frequencies. By combining the experimental optical results with finite-difference time-domain simulations we establish a direct relation between the observed wavelength drift and the actual effective temperature increase of the cavity. By assuming that the Youngs modulus decreases accordingly to the temperature increase, we find a good agreement between the mechanical mode drift predicted using a finite element method and the experimental one.
We show that coherent multiple light scattering, or diffuse light propagation, in a disordered atomic medium, prepared at ultra-low temperatures, can be be effectively delayed in the presence of a strong control field initiating a stimulated Raman process. On a relatively short time scale, when the atomic system can preserve its configuration and effects of atomic motion can be ignored, the scattered signal pulse, diffusely propagating via multiple coherent scattering through the medium, can be stored in the spin subsystem through its stimulated Raman-type conversion into spin coherence. We demonstrate how this mechanism, potentially interesting for developing quantum memories, would work for the example of a coherent light pulse propagating through an alkali-metal atomic vapor under typical conditions attainable in experiments with ultracold atoms.
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