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Ground-State Electromagnetic Moments of Calcium Isotopes

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 Publication date 2015
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High-resolution bunched-beam collinear laser spectroscopy was used to measure the optical hyperfine spectra of the $^{43-51}$Ca isotopes. The ground state magnetic moments of $^{49,51}$Ca and quadrupole moments of $^{47,49,51}$Ca were measured for the first time, and the $^{51}$Ca ground state spin $I=3/2$ was determined in a model-independent way. Our results provide a critical test of modern nuclear theories based on shell-model calculations using phenomenological as well as microscopic interactions. The results for the neutron-rich isotopes are in excellent agreement with predictions using interactions derived from chiral effective field theory including three-nucleon forces, while lighter isotopes illustrate the presence of particle-hole excitations of the $^{40}$Ca core in their ground state.



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The hyperfine coupling constants of neutron deficient $^{37}$Ca were deduced from the atomic hyperfine spectrum of the $4s~^2S_{1/2}$ $leftrightarrow$ $4p~^2P_{3/2}$ transition in Ca II, measured using the collinear laser spectroscopy technique. The ground-state magnetic-dipole and spectroscopic electric-quadrupole moments were determined for the first time as $mu = +0.7453(72) mu_N$ and $Q = -15(11)$ $e^2$fm$^2$, respectively. The experimental values agree well with nuclear shell model calculations using the universal sd model-space Hamiltonia
In-source resonant ionization laser spectroscopy of the even-$A$ polonium isotopes $^{192-210,216,218}$Po has been performed using the $6p^37s$ $^5S_2$ to $6p^37p$ $^5P_2$ ($lambda=843.38$ nm) transition in the polonium atom (Po-I) at the CERN ISOLDE facility. The comparison of the measured isotope shifts in $^{200-210}$Po with a previous data set allows to test for the first time recent large-scale atomic calculations that are essential to extract the changes in the mean-square charge radius of the atomic nucleus. When going to lighter masses, a surprisingly large and early departure from sphericity is observed, which is only partly reproduced by Beyond Mean Field calculations.
Collinear laser spectroscopy measurements were performed on $^{69,71,73}$Ge isotopes ($Z = 32$) at ISOLDE-CERN. The hyperfine structure of the $4s^2 4p^2 , ^3P_1 rightarrow 4s^2 4p 5s , ^3P_1^o$ transition of the germanium atom was probed with laser light of 269 nm, produced by combining the frequency-mixing and frequency-doubling techniques. The hyperfine fields for both atomic levels were calculated using state-of-the-art atomic relativistic Fock-space coupled-cluster calculations. A new $^{73}$Ge quadrupole moment was determined from these calculations and previously measured precision hyperfine parameters, yielding $Q_{rm s}$ = $-$0.198(4) b, in excellent agreement with the literature value from molecular calculations. The moments of $^{69}$Ge have been revised: $mu$ = +0.920(5) $mu_{N}$ and $Q_{rm s}$= +0.114(8) b, and those of $^{71}$Ge have been confirmed. The experimental moments around $N = 40$ are interpreted with large-scale shell-model calculations using the JUN45 interaction, revealing rather mixed wave function configurations, although their $g$-factors are lying close to the effective single-particle values. Through a comparison with neighboring isotones, the structural change from the single-particle nature of nickel to deformation in germanium is further investigated around $N = 40$.
item[Background] Ground-state spins and magnetic moments are sensitive to the nuclear wave function, thus they are powerful probes to study the nuclear structure of isotopes far from stability. item[Purpose] Extend our knowledge about the evolution of the $1/2^+$ and $3/2^+$ states for K isotopes beyond the $N = 28$ shell gap. item[Method] High-resolution collinear laser spectroscopy on bunched atomic beams. item[Results] From measured hyperfine structure spectra of K isotopes, nuclear spins and magnetic moments of the ground states were obtained for isotopes from $N = 19$ up to $N = 32$. In order to draw conclusions about the composition of the wave functions and the occupation of the levels, the experimental data were compared to shell-model calculations using SDPF-NR and SDPF-U effective interactions. In addition, a detailed discussion about the evolution of the gap between proton $1d_{3/2}$ and $2s_{1/2}$ in the shell model and {it{ab initio}} framework is also presented. item[Conclusions] The dominant component of the wave function for the odd-$A$ isotopes up to $^{45}$K is a $pi 1d_{3/2}^{-1}$ hole. For $^{47,49}$K, the main component originates from a $pi 2s_{1/2}^{-1}$ hole configuration and it inverts back to the $pi 1d_{3/2}^{-1}$ in $^{51}$K. For all even-$A$ isotopes, the dominant configuration arises from a $pi 1d_{3/2}^{-1}$ hole coupled to a neutron in the $ u 1f_{7/2}$ or $ u 2p_{3/2}$ orbitals. Only for $^{48}$K, a significant amount of mixing with $pi 2s_{1/2}^{-1} otimes u (pf)$ is observed leading to a $I^{pi}=1^{-}$ ground state. For $^{50}$K, the ground-state spin-parity is $0^-$ with leading configuration $pi 1d_{3/2}^{-1} otimes u 2p_{3/2}^{-1}$.
The calcium isotopes have emerged as an important testing ground for new microscopically derived shell-model interactions, and a great deal of focus has been directed toward this region. We investigate the relative spectroscopic strengths associated with $1f_{7/2}$ neutron hole states in $^{47, 49}$Ca following one-neutron knockout reactions from $^{48,50}$Ca. The observed reduction of strength populating the lowest 7/2$^{-}_{1}$ state in $^{49}$Ca, as compared to $^{47}$Ca, is consistent with the description given by shell-model calculations based on two- and three-nucleon forces in the neutron $pf$ model space, implying a fragmentation of the $l$=3 strength to higher-lying states. The experimental result is inconsistent with both the GXPF1 interaction routinely used in this region of the nuclear chart and with microscopic calculations in an extended model space including the $ u1g_{9/2}$ orbital.
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