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We calculate the friction of fully mobile graphene flakes sliding on graphite. For incommensurately stacked flakes, we find a sudden and reversible increase in friction with load, in agreement with experimental observations. The transition from smooth sliding to stick-slip and the corresponding increase in friction is neither due to rotations to commensurate contact nor to dislocations but to a pinning caused by vertical distortions of edge atoms also when they are saturated by Hydrogen. This behavior should apply to all layered materials with strong in-plane bonding.
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Graphene nanoribbons (GNRs) physisorbed on a Au(111) surface can be picked up, lifted at one end, and made slide by means of the tip of an atomic-force microscope. The dynamical transition from smooth sliding to multiple stick-slip regimes, the pushing/pulling force asymmetry, the presence of pinning, and its origin are real frictional processes in a nutshell, in need of a theoretical description. To this purpose, we conduct classical simulations of frictional manipulations for GNRs up to 30 nm in length, one end of which is pushed or pulled horizontally while held at different heights above the Au surface. These simulations allow us to clarify theoretically the emergence of stick-slip originating from the short 1D edges rather than the 2D bulk, the role of adhesion, of lifting, and of graphene bending elasticity in determining the GNR sliding friction. The understanding obtained in this simple context is of additional value for more general cases.
We model the optical visibility of monolayer and bilayer graphene deposited on a silicon/silicon oxide substrate or thermally annealed on the surface of silicon carbide. We consider reflection and transmission setups, and find that visibility is strongest in reflection reaching the optimum conditions when the bare substrate transmits light resonantly. In the optical range of frequencies a bilayer is approximately twice as visible as a monolayer thereby making the two types of graphene distinguishable from each other.
The authors proposed a simple model for the lattice thermal conductivity of graphene in the framework of Klemens approximation. The Gruneisen parameters were introduced separately for the longitudinal and transverse phonon branches through averaging over phonon modes obtained from the first-principles. The calculations show that Umklapp-limited thermal conductivity of graphene grows with the increasing linear dimensions of graphene flakes and can exceed that of the basal planes of bulk graphite when the flake size is on the order of few micrometers. The obtained results are in agreement with experimental data and reflect the two-dimensional nature of phonon transport in graphene.
We show that the manifestation of quantum interference in graphene is very different from that in conventional two-dimensional systems. Due to the chiral nature of charge carriers, it is sensitive not only to inelastic, phase-breaking scattering, but also to a number of elastic scattering processes. We study weak localization in different samples and at different carrier densities, including the Dirac region, and find the characteristic rates that determine it. We show how the shape and quality of graphene flakes affect the values of the elastic and inelastic rates and discuss their physical origin.
We discuss the stick-slip motion of an elastic block sliding along a rigid substrate. We argue that for a given external shear stress this system shows a discontinuous nonequilibrium transition from a uniform stick state to uniform sliding at some critical stress which is nothing but the Griffith threshold for crack propagation. An inhomogeneous mode of sliding occurs, when the driving velocity is prescribed instead of the external stress. A transition to homogeneous sliding occurs at a critical velocity, which is related to the critical stress. We solve the elastic problem for a steady-state motion of a periodic stick-slip pattern and derive equations of motion for the tip and resticking end of the slip pulses. In the slip regions we use the linear viscous friction law and do not assume any intrinsic instabilities even at small sliding velocities. We find that, as in many other pattern forming system, the steady-state analysis itself does not select uniquely all the internal parameters of the pattern, especially the primary wavelength. Using some plausible analogy to first order phase transitions we discuss a ``soft selection mechanism. This allows to estimate internal parameters such as crack velocities, primary wavelength and relative fraction of the slip phase as function of the driving velocity. The relevance of our results to recent experiments is discussed.
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