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X-ray scattering is a weak linear probe of matter. It is primarily sensitive to the position of electrons and their momentum distribution. Elastic X-ray scattering forms the basis of atomic structural determination while inelastic Compton scattering is often used as a spectroscopic probe of both single-particle excitations and collective modes. X-ray free-electron lasers (XFELs) are unique tools for studying matter on its natural time and length scales due to their bright and coherent ultrashort pulses. However, in the focus of an XFEL the assumption of a weak linear probe breaks down, and nonlinear light-matter interactions can become ubiquitous. The field can be sufficiently high that even non-resonant multiphoton interactions at hard X-rays wavelengths become relevant. Here we report the observation of one of the most fundamental nonlinear X-ray-matter interactions, the simultaneous Compton scattering of two identical photons producing a single photon at nearly twice the photon energy. We measure scattered photons with an energy near 18 keV generated from solid beryllium irradiated by 8.8-9.75 keV XFEL pulses. The intensity in the X-ray focus reaches up to 4x20 W/cm2, which corresponds to a peak electric field two orders of magnitude higher than the atomic unit of field-strength and within four orders of magnitude of the quantum electrodynamic critical field. The observed signal scales quadratically in intensity and is emitted into a non-dipolar pattern, consistent with the simultaneous two-photon scattering from free electrons. However, the energy of the generated photons shows an anomalously large redshift only present at high intensities. This indicates that the instantaneous high-intensity scattering effectively interacts with a different electron momentum distribution than linear Compton scattering, with implications for the study of atomic-scale structure and dynamics of matter
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We lay the foundations for a new fast method to reconstruct the electron density in x-ray scanning applications using measurements in the dark field. This approach is applied to a type of machine configuration with fixed energy sensitive (or resolving) detectors, and where the X-ray source is polychromatic. We consider the case where the measurements in the dark field are dominated by the Compton scattering process. This leads us to a 2D inverse problem where we aim to reconstruct an electron density slice from its integrals over discs whose boundaries intersect the given source point. We show that a unique solution exists for smooth densities compactly supported on an annulus centred at the source point. Using Sobolev space estimates we determine a measure for the ill posedness of our problem based on the criterion given by Natterer (The mathematics of computerized tomography SIAM 2001). In addition, with a combination of our method and the more common attenuation coefficient reconstruction, we show under certain assumptions that the atomic number of the target is uniquely determined. We test our method on simulated data sets with varying levels of added pseudo random noise.
We report the observation of a novel nonlinear effect in the hard x-ray range. Upon illuminating Fe and Cu metal foils with intense x-ray pulses tuned near their respective K edges, photons at nearly twice the incoming photon energy are emitted. The signal rises quadratically with the incoming intensity, consistent with two-photon excitation. The spectrum of emitted high-energy photons comprises multiple Raman lines that disperse with the incident photon energy. Upon reaching the double K-shell ionization threshold, the signal strength undergoes a marked rise. Above this threshold, the lines cease dispersing, turning into orescence lines with energies much greater than obtainable by single electron transitions, and additional Raman lines appear. We attribute these processes to electron-correlation mediated multielectron transitions involving double-core hole excitation and various two-electron de-excitation processes to a final state involving one or more L and M core-holes.
We have performed a systematic study of the Bremsstrahlung emission from the electrons in the plasma of a commercial 14.5 GHz Electron-Cyclotron Resonance Ion Source. The electronic spectral temperature and the product of ionic and electronic densities of the plasma are measured by analyzing the Bremsstrahlung spectra recorded for several rare gases (Ar, Kr, Xe) as a function of the injected power. Within our uncertainty, we find an average temperature of ? 48 keV above 100W, with a weak dependency on the injected power and gas composition. Charge state distributions of extracted ion beams have been determined as well, providing a way to disentangle the ionic density from the electronic density. Moreover X-ray emission from highly charged argon ions in the plasma has been observed with a high-resolution mosaic crystal spectrometer, demonstrating the feasibility for high-precision measurements of transition energies of highly charged ions, in particular of the magnetic dipole (M1) transition of He-like of argon ions.
The backward Compton scattering is a basic process at future higher energy photon colliders. To obtain a high probability of e->gamma conversion the density of laser photons in the conversion region should be so high that simultaneous interaction of one electron with several laser photons is possible (nonlinear Compton effect). In this paper a detailed consideration of energy spectra, helicities of final photons and electrons in nonlinear backward Compton scattering of circularly polarized laser photons is given. Distributions of gamma-gamma luminosities with total helicities 0 and 2 are investigated. Very high intensity of laser wave leads to broadening of the energy (luminosity) spectra and shift to lower energies (invariant masses). Beside complicated exact formulae, approximate formulae for energy spectrum and polarization of backscattered photons are given for relatively small nonlinear parameter xi^2 (first order correction). All this is necessary for optimization of the conversion region at photon colliders and study of physics processes where a sharp edge of the luminosity spectrum and monochromaticity of collisions are important.
We study single, double and higher-order nonlinear Compton scattering where an electron interacts nonlinearly with a high-intensity laser and emits one, two or more photons. We study, in particular, how double Compton scattering is separated into one-step and two-step parts, where the latter is obtained from an incoherent product of two single-photon emissions. We include all contributions to double Compton scattering and show that the exchange term, which was not calculated in previous constant-crossed field studies, is in general on the same order of magnitude as the other one-step terms. Our approach reveals practically useful similarities between double Compton scattering and the trident process, which allows us to transfer some of our previous results for trident to double Compton scattering. We provide a new gluing approach for obtaining the dominant contribution to higher-order Compton scattering for long laser pulses. Unlike the standard gluing approach, our new approach does not require the intensity parameter $a_0$ to be much larger than one. For `hard photons we obtain several saddle-point approximations for various field shapes.
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