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A subpicotesla diamond magnetometer

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 Added by Thomas Wolf
 Publication date 2014
  fields Physics
and research's language is English




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Diamond defect centers are promising solid state magnetometers. Single centers allow for high spatial resolution field imaging but are limited in their magnetic field sensitivity to around 10 nT/Hz^(1/2) at room-temperature. Using defect center ensembles sensitivity can be scaled as N^(1/2) when N is the number of defects. In the present work we use an ensemble of 1e11 defect centers for sensing. By carefully eliminating all noise sources like laser intensity fluctuations, microwave amplitude and phase noise we achieve a photon shot noise limited field sensitivity of 0.9 pT/Hz^(1/2) at room-temperature with an effective sensor volume of 8.5e-4 mm^3. The smallest field we measured with our device is 100 fT. While this denotes the best diamond magnetometer sensitivity so far, further improvements using decoupling sequences and material optimization could lead to fT/Hz^(1/2) sensitivity.



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We present a highly sensitive miniaturized cavity-enhanced room-temperature magnetic-field sensor based on nitrogen-vacancy (NV) centers in diamond. The magnetic resonance signal is detected by probing absorption on the 1042,nm spin-singlet transition. To improve the absorptive signal the diamond is placed in an optical resonator. The device has a magnetic-field sensitivity of 28 pT/$sqrt{rm{Hz}}$, a projected photon shot-noise-limited sensitivity of 22 pT/$sqrt{rm{Hz}}$ and an estimated quantum projection-noise-limited sensitivity of 0.43 pT/$sqrt{rm{Hz}}$ with the sensing volume of $sim$ 390 $mu$m $times$ 4500 $mu$m$^{2}$. The presented miniaturized device is the basis for an endoscopic magnetic field sensor for biomedical applications.
Nitrogen vacancy (NV) centers in diamond have developed into a powerful solid-state platform for compact quantum sensors. However, high sensitivity measurements usually come with additional constraints on the pumping intensity of the laser and the pulse control applied. Here, we demonstrate high sensitivity NV ensemble based magnetic field measurements with low-intensity optical excitation. DC magnetometry methods like, e.g., continuous-wave optically detected magnetic resonance and continuously excited Ramsey measurements combined with lock-in detection, are compared to get an optimization. Gradiometry is also investigated as a step towards unshielded measurements of unknown gradients. The magnetometer demonstrates a minimum detectable field of 0.3-0.7 pT in a 73 s measurement by further applying a flux guide with a sensing dimension of 2 mm, corresponding to a magnetic field sensitivity of 2.6-6 pT/Hz^0.5. Combined with our previous efforts on the diamond AC magnetometry, the diamond magnetometer is promising to perform wide bandwidth magnetometry with picotesla sensitivity and a cubic-millimeter sensing volume under ambient conditions.
Magnetometers based on nitrogen-vacancy (NV) centers in diamond are promising room-temperature, solid-state sensors. However, their reported sensitivity to magnetic fields at low frequencies (<1 kHz) is presently >10 pT s^{1/2}, precluding potential applications in medical imaging, geoscience, and navigation. Here we show that high-permeability magnetic flux concentrators, which collect magnetic flux from a larger area and concentrate it into the diamond sensor, can be used to improve the sensitivity of diamond magnetometers. By inserting an NV-doped diamond membrane between two ferrite cones in a bowtie configuration, we realize a ~250-fold increase of the magnetic field amplitude within the diamond. We demonstrate a sensitivity of ~0.9 pT s^{1/2} to magnetic fields in the frequency range between 10 and 1000 Hz, using a dual-resonance modulation technique to suppress the effect of thermal shifts of the NV spin levels. This is accomplished using 200 mW of laser power and 20 mW of microwave power. This work introduces a new dimension for diamond quantum sensors by using micro-structured magnetic materials to manipulate magnetic fields.
We present an experimental method to perform dual-channel lock-in magnetometry of time-dependent magnetic fields using a single spin associated with a nitrogen-vacancy (NV) color center in diamond. We incorporate multi-pulse quantum sensing sequences with phase estimation algorithms to achieve linearized field readout and constant, nearly decoherence-limited sensitivity over a wide dynamic range. Furthermore, we demonstrate unambiguous reconstruction of the amplitude and phase of the magnetic field. We show that our technique can be applied to measure random phase jumps in the magnetic field, as well as phase-sensitive readout of the frequency.
Magnetic field sensors that exploit quantum effects have shown that they can outperform classical sensors in terms of sensitivity enabling a range of novel applications in future, such as a brain machine interface. Negatively charged nitrogen-vacancy (NV) centers in diamond have emerged as a promising high sensitivity platform for measuring magnetic fields at room temperature. Transferring this technology from laboratory setups into products and applications, the total size of the sensor, the overall power consumption, and the costs need to be reduced and optimized. Here, we demonstrate a fiber-based NV magnetometer featuring a complete integration of all functional components without using any bulky laboratory equipment. This integrated prototype allows portable measurement of magnetic fields with a sensitivity of 344 pT/ SqrtHz.
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