The thermodynamic properties of strongly correlated system with binary type of disorder are investigated using the combination of the coherent potential approximation and dynamical mean-field theory. The specific heat has a peak at small temperatures for the concentrations close to the filling of system. This peak is associated with the local moment formation due to Coulomb interaction. The linear coefficient to the specific heat is divergent and the system stays in the non-Fermi-liquid regime.
We use a combination of the coherent potential approximation and dynamical mean field theory to study magnetic properties of the Fe$_{1-x}$Ni$_x$ alloy from a first principles. Calculated uniform magnetic susceptibilities have a Curie-Weiss-like behavior and extracted effective temperatures are in agreement with the experimental results. The individual squared magnetic moments obtained as function of nickel concentration follow the same trends as experimental data. An analysis of the ionic and spin weights shows a possibility of a high-spin to intermediate- and low-spin states transitions at high temperatures.
The puzzling absence of Pu magnetic moments in a PuAm environment is explored using the self-consistent Dynamical Mean Field Theory (DMFT) calculations in combination with the Local Density Approximation. We argue that delta-Pu -Am alloys provide an ideal test bed for investigating the screening of moments from the single impurity limit to the dense limit. Several important effects can be studied: volume expansion, shift of the bare Pu on-site f energy level, and the reduction of the hybridization cloud resulting from the collective character of the Kondo effect in the Anderson lattice. These effects compensate each other and result in a coherence scale, which is independent of alloy composition, and is around 800K. We emphasize the role of the DMFT self-consistency condition, and multiplet splittings in Pu and Am atoms, in order to capture the correct value of the coherence scale in the alloy.
The temperature and magnetic field dependence of the specific heat cp(T,H) in the superconducting mixed state as well as the upper critical field Hc2(T) have been measured for polycrystalline Y_xLu_{1-x}Ni_2B_2C and Y(Ni_{1-y}Pt_y)_2B_2C samples. The linear-in-T electronic specific heat contribution gamma(H)T exhibits significant deviations from the usual linear-in-H law for all x and y the transition metal site (T) resulting in a disorder dependent negative curvature of gamma(H). The deviations from that linear behaviour of our unsubstituted samples are the largest reported so far for any superconductor. The H_c2(T) data point to the quasi-clean limit for (Y,Lu)-substitutions and to a transition to the quasi-dirty limit for (Ni,Pt)-substitutions. The gamma(H) dependence is discussed in the unitary d-wave as well as in the quasi-clean s-wave limits. From a consideration of gamma(H) data only, d-wave pairing cannot be ruled out.
The cobaltates have demonstrated a wide variety complex behavior. The Na rich region of the phase diagram displays various degrees of anomalous behavior, such as Curie-Weiss behavior near a band insulatorcite{Foo:2004}, charge disproportionationcite{Mukhamedshin:2005}, and non-Fermi-liquid behavior in the resistivitycite{Foo:2004}. Alternatively, the Na poor region of the phase diagram appears to be a Fermi-liquid. The magnetic susceptibility displays Pauli behavior, the resistivity is roughly quadratic at low temperaturescite{Foo:2004}, and the system appears to be homogeneouscite{Mukhamedshin:2005}. Therefore, the Na poor region of the phase diagram seems like a natural starting point to attempt to explain the ARPES experiments and heat capacity measurements from a quantitative standpoint.
Low-temperature electronic states in SrRu_{1-x}Mn_xO_3 for x <= 0.6 have been investigated by means of specific-heat C_p measurements. We have found that a jump anomaly observed in C_p at the ferromagnetic (FM) transition temperature for SrRuO_3 changes into a broad peak by only 5% substitution of Mn for Ru. With further doping Mn, the low-temperature electronic specific-heat coefficient gamma is markedly reduced from the value at x=0 (33 mJ/K^2 mol), in connection with the suppression of the FM phase as well as the enhancement of the resistivity. For x >= 0.4, gamma approaches to ~ 5 mJ/K^2 mol or less, where the antiferromagnetic order with an insulating feature in resistivity is generated. We suggest from these results that both disorder and reconstruction of the electronic states induced by doping Mn are coupled with the magnetic ground states and transport properties.
Alexander I. Poteryaev
,Sergey V. Skornyakov
,Alexander S. Belozerov
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(2014)
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"Study of the specific heat for the binary alloy in the CPA+DMFT method"
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Alexander Poteryaev I.
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