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Register a new userProcessing of analogues of plume fallout in cold regions of Enceladus by energetic electrons
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Alexandre Bergantini
Publication date
2014
fields
Physics
and research's language is
English
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Enceladus, a small icy moon of Saturn, is one of the most remarkable bodies in the solar system. This moon is a geologically active object, and despite the lower temperatures on most of its surface, the geothermally heated south polar region presents geysers that spouts a plume made of water (approximately ninety percent), carbon dioxide, methane, ammonia, and methanol, among other molecules. Most of the upward-moving particles do not have the velocity to escape from the gravitational influence of the moon and fall back to the surface. The molecules in the ice are continuously exposed to ionizing radiation, such as UV and X-rays photons, cosmic rays, and electrons. Over time, the ionizing radiation promotes molecular bond rupture, destroying and also forming molecules, radicals, and fragments. We analyse the processing of an ice mixture analogue to the Enceladus fallout ice in cold resurfaced areas (north pole) by 1 keV electrons. The main goal is to search for complex species that have not yet been detected in this moon, and to determine relevant physico-chemical parameters, such as destruction and formation cross-sections and the half-life of the studied molecules in the ice. The experiment consisted of the electron irradiation of an Enceladus-like ice mixture (H2O,CO2,CH4,NH3, and CH3OH) in an ultra-high vacuum chamber at 20 K. The analysis was made by infrared spectrometry in the mid-infrared region (4000-800 cm-1 or 2.5-12.5 microns).The absolute dissociation cross-sections of the parent molecules, the formation cross-section of daughter species, and the half-life of the parental species in a simulated Enceladus irradiation scenario were determined. Among the produced species, CO (carbon monoxide), OCN- (cyanate anion), HCONH2 (formamide), and H2CO (formaldehyde) were tentatively detected.
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Formic acid (HCOOH) has been extensively detected in space environments, including interstellar medium (gas and grains), comets and meteorites. Such environments are often subjected to the action of ionizing agents, which may cause changes in the molecular structure, thus leading to formation of new species. Formic acid is a possible precursor of pre-biotic species, such as Glycine (NH2CH2COOH). This work investigates experimentally the physicochemical effects resulting from interaction of heavy and energetic cosmic ray analogues (46MeV 58Ni11+) in H2O:HCOOH (1:1) ice, at 15 K, in ultrahigh vacuum regime, using Fourier transform infrared spectrometry in the mid-infrared region (4000-600 cm-1 or 2.5-12.5 microns). After the bombardment, the sample was slowly heated to room temperature. The results show the dissociation cross-section for the formic acid of 2.4x10^-13 cm2, and half-life due to galactic cosmic rays of 8x10^7 yr. The IR spectra show intense formation of CO and CO2, and small production of more complex species at high fluences.
Sulfur is an abundant element in the cosmos and it is thus an important contributor to astrochemistry in the interstellar medium and in the Solar System. Astronomical observations of the gas and of the solid phases in the dense interstellar/circumstellar regions have evidenced that sulfur is underabundant. The hypothesis to explain such a circumstance is that it is incorporated in some species in the solid phase (i.e. as frozen gases and/or refractory solids) and/or in the gas phase, which for different reasons have not been observed so far. Here we wish to give a contribution to the field by studying the chemistry induced by thermal and energetic processing of frozen mixtures of sulfur dioxide (one of the most abundant sulfur-bearing molecules observed so far) and water. We present the results of a series of laboratory experiments concerning thermal processing of different H2O:SO2 mixtures and ion bombardment 30 keV He$^+$ of the same mixtures. We used in situ FTIR spectroscopy to investigate the induced effects. The results indicate that ionic species such as HSO$_{3}^{-}$, HSO$_{4}^{-}$, and S$_2$O$_{5}^{2-}$ are easily produced. Energetic processing also produces SO$_3$ polymers and a sulfurous refractory residue. The produced ionic species exhibit spectral features in a region that, in astronomical spectra of dense molecular clouds, is dominated by strong silicate absorption. However, such a dominant feature is associated with some spectral features, some of which have not yet been identified. We suggest adding the sulfur-bearing ionic species to the list of candidates to help explain some of those features.
In the preceding paper (Efroimsky 2017), we derived an expression for the tidal dissipation rate in a homogeneous near-spherical Maxwell body librating in longitude. Now, by equating this expression to the outgoing energy flux due to the vapour plumes, we estimate the mean tidal viscosity of Enceladus, under the assumption that the Enceladean mantle behaviour is Maxwell. This method yields a value of $,0.24times 10^{14};mbox{Pa~s},$ for the mean tidal viscosity, which is very close to the viscosity of ice near the melting point.
Context. The origin of water in the stratospheres of Giant Planets has been an outstanding question ever since its first detection by ISO some 20 years ago. Water can originate from interplanetary dust particles, icy rings and satellites and large comet impacts. Analysis of Herschel Space Observatory observations have proven that the bulk of Jupiters stratospheric water was delivered by the Shoemaker-Levy 9 impacts in 1994. In 2006, the Cassini mission detected water plumes at the South Pole of Enceladus, placing the moon as a serious candidate for Saturns stratospheric water. Further evidence was found in 2011, when Herschel demonstrated the presence of a water torus at the orbital distance of Enceladus, fed by the moons plumes. Finally, water falling from the rings onto Saturns uppermost atmospheric layers at low latitudes was detected during the final orbits of Cassinis end-of-mission plunge into the atmosphere. Aims. In this paper, we use Herschel mapping observations of water in Saturns stratosphere to identify its source. Methods. Several empirical models are tested against the Herschel-HIFI and -PACS observations, which were collected on December 30, 2010, and January 2nd, 2011 (respectively). Results. We demonstrate that Saturns stratospheric water is not uniformly mixed as a function of latitude, but peaking at the equator and decreasing poleward with a Gaussian distribution. We obtain our best fit with an equatorial mole fraction 1.1 ppb and a half-width at half-maximum of 25{deg}, when accounting for a temperature increase in the two warm stratospheric vortices produced by Saturns Great Storm of 2010-2011. Conclusions. This work demonstrates that Enceladus is the main source of Saturns stratospheric water.
In Huybrighs et al., 2020 we investigated energetic proton depletions along Galileos Europa flyby E26. Based on a particle tracing analysis we proposed that depletions are caused by perturbed electrogmagnetic fields combined with atmospheric charge exchange and possible plumes. One depletion feature identified as a plume signature was shown to be an artefact Jia et al., 2021. Despite that, here we emphasize that Huybrighs et al., 2020 demonstrates that plumes can cause proton depletions and that these features should be sought after. Furthermore, the conclusions on the importance of perturbed electromagnetic fields and atmospheric charge exchange on the depletions are unaffected. We suggest that the artefacts cause is a mistagging of protons as heavier ions by EPD. The artefact prevents us from confirming or excluding that there is a plume associated depletion. We also address comments on the MHD simulations and demonstrate that 540-1040 keV losses are not necessarily inconsistent with 115-244 keV losses by plume associated charge exchange.
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