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Register a new userThe magnetic moment enigma in Fe-based high temperature superconductors
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Norman Mannella
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The determination of the most appropriate starting point for the theoretical description of Fe-based materials hosting high temperature superconductivity remains among the most important unsolved problem in this relatively new field. Most of the work to date has focused on the pnictides, with LaFeAsO, BaFe2As2 and LiFeAs being representative parent compounds of three families known as 1111, 122 and 111, respectively. This Topic Review examines recent progress in this area, with particular emphasis on the implication of experimental data which have provided evidence for the presence of electron itinerancy and the detection of local spin moments. In light of the results presented, the necessity of a theoretical framework contemplating the presence and the interplay between itinerant electrons and large spin moments is discussed. It is argued that the physics at the heart of the macroscopic properties of pnictides Fe-based high temperature superconductors appears to be far more complex and interesting than initially predicted.
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A magnetic field relaxation at the center of a pulse-magnetized single-domain Y-Ba-Cu-O superconductor at 78K has been studied. In case of a weak magnetization, the magnetic flux density increases logarithmically and normalized relaxation rate defined as S=-d(lnB)/d(lnt) is negative (S=-0.037). When an external magnetic field magnitude increases, the relaxation rate first decreases in absolute value, then changes sign (becomes positive, S>0) and after reaching some maximum finally reduces to a very small value. Non-monotonous dependence of S vs Ha is explained by a non-homogeneous local temperature distribution during a pulse magnetization.
We suggest that a family of Ni-based compounds, which contain [Ni$_2$M$_2$O]$^{2-}$(M=chalcogen) layers with an antiperovskite structure constructed by mixed-anion Ni complexes, NiM$_4$O$_2$, can be potential high temperature superconductors upon doping or applying pressure. The layer structures have been formed in many other transitional metal compounds such as La$_2$B$_2$Se$_2$O$_3$(B=Mn, Fe,Co). For the Ni-based compounds, we predict that the parental compounds host collinear antiferromagnetic states similar to those in the iron-based high temperature superconductors. The electronic physics near Fermi energy is controlled by two e$_{g}$ d-orbitals with completely independent in-plane kinematics. We predict that the superconductivity in this family is characterized by strong competition between extended s-wave and d-wave pairing symmetries.
The t-t-t-J model of electrons interacting with three phonon modes (breathing, apical breathing, and buckling) is considered. The wave-vector dependence of the matrix elements of the electron-phonon interaction leads to opposite contributions to the pairing potential with the d-symmetry: the buckling mode facilitates electron pairing, while the breathing mode suppresses it. As a result, the critical temperature of La{2 - x}Sr{x}CuO{4} that is associated with the magnetic mechanism is lowered when phonons are taken into account.
A direct and element-specific measurement of the local Fe spin moment has been provided by analyzing the Fe 3s core level photoemission spectra in the parent and optimally doped CeFeAsO1-xFx (x = 0, 0.11) and Sr(Fe1 xCox)2As2 (x = 0, 0.10) pnictides. The rapid time scales of the photoemission process allowed the detection of large local spin moments fluctuating on a 10-15 s time scale in the paramagnetic, anti-ferromagnetic and superconducting phases, indicative of the occurrence of ubiquitous strong Hunds magnetic correlations. The magnitude of the spin moment is found to vary significantly among different families, 1.3 muB in CeFeAsO and 2.1 muB in SrFe2As2. Surprisingly, the spin moment is found to decrease considerably in the optimally doped samples, 0.9 muB in CeFeAsO0.89F0.11 and 1.3 muB in Sr(Fe0.9Co0.1)2As2. The strong variation of the spin moment against doping and material type indicates that the spin moments and the motion of itinerant electrons are influenced reciprocally in a self-consistent fashion, reflecting the strong competition between the antiferromagnetic super-exchange interaction among the spin moments and the kinetic energy gain of the itinerant electrons in the presence of a strong Hunds coupling. By describing the evolution of the magnetic correlations concomitant with the appearance of superconductivity, these results constitute a fundamental step toward attaining a correct description of the microscopic mechanisms shaping the electronic properties in the pnictides, including magnetism and high temperature superconductivity.
The symmetry operations of the crystal groups relevant for the high temperature superconductors HgBa2CuO4+x (Hg1201), YBa2Cu3O7-x (YBCO), and Bi2Sr2CaCu2O8+x (BSCCO) are elucidated. The allowable combinations of the superconducting order parameter (OP) components are presented for both the angular momentum and lattice representations. For tetragonal Hg1201, the spin singlet OP components are composed from four sets of compatible basis functions, which combine to give the generalized s-, dx2-y2-, dxy-, and gxy(x2-y2)- wave OPs. In YBCO, elements of s- and dx2-y2- wave sets are compatible, but in BSCCO, elements of s- and dxy- wave sets are compatible. The Josephson critical current density JcJ across c-axis twist junctions in the vicinity of Tc is then evaluated as a function of the twist angle phi0, for each allowable OP combination, for both coherent and incoherent tunneling. Recent experiments of Li et al. demonstrated the independence of JcJ(phi0)/JcS upon phi0 at and below Tc, where JcS is the critical current density of a constituent single crystal. These experiments are shown to be consistent with an OP containing an s-wave component, but inconsistent with an OP containing the purported dx2-y2-wave component. In addition, they demonstrate that the interlayer tunneling across untwisted layers in single crystal BSCCO is entirely incoherent. We propose a new type of tricrystal experiment using single crystal c-axis twist junctions, that does not employ substrate grain boundaries.
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