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Register a new userHigh-resolution imaging of velocity-controlled molecular collisions using counterpropagating beams
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Added by
Sebastiaan Y.T. van de Meerakker
Publication date
2014
fields
Physics
and research's language is
English
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We present ultrahigh-resolution measurements of state-to-state inelastic differential cross sections for NO-Ne and NO-Ar collisions, obtained by combining the Stark deceleration and velocity map imaging techniques. We show that for counterpropagating crossed beam geometries, the effect of the velocity spreads of the reagent beams on the angular resolution of the images is minimized. Futhermore, the counterpropagating geometry results in images that are symmetric with respect to the relative velocity vector. This allows for the use of inverse Abel transformation methods that enhance the resolution further. State-resolved diffraction oscillations in the differential cross sections are measured with an angular resolution approaching 0.3$^circ$. Distinct structures observed in the cross sections gauge the quality of recent emph{ab initio} potential energy surfaces for NO-rare gas atom collisions with unprecedented precision.
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Stark deceleration allows for precise control over the velocity of a pulsed molecular beam and, by the nature of its limited phase-space acceptance, reduces the energy width of the decelerated packet. We describe an alternate method of operating a Stark decelerator that further reduces the energy spread over the standard method of operation. In this alternate mode of operation, we aggressively decelerate the molecular packet using a high phase angle. This technique brings the molecular packet to the desired velocity before it reaches the end of the decelerator; the remaining stages are then used to longitudinally and transversely guide the packet to the detection/interaction region. The result of the initial aggressive slowing is a reduction in the phase-space acceptance of the decelerator and thus a narrowing of the velocity spread of the molecular packet. In addition to the narrower energy spread, this method also results in a velocity spread that is nearly independent of the final velocity. Using the alternate deceleration technique, the energy resolution of molecular collision measurements can be improved considerably.
The dynamics and radiation of ultrarelativistic electrons in strong counterpropagating laser beams are investigated. Assuming that the particle energy is the dominant scale in the problem, an approximate solution of classical equations of motion is derived and the characteristic features of the motion are examined. A specific regime is found with comparable strong field quantum parameters of the beams, when the electron trajectory exhibits ultrashort spike-like features, which bears great significance to the corresponding radiation properties. An analytical expression for the spectral distribution of spontaneous radiation is derived in the framework of the Baier-Katkov semiclassical approximation based on the classical trajectory. All the analytical results are further validated by exact numerical calculations. We consider a non-resonant regime of interaction, when the laser frequencies in the electron rest frame are far from each other, avoiding stimulated emission. Special attention is devoted to settings when the description of radiation via the local constant field approximation fails and to corresponding spectral features. Periodic and non-periodic regimes are considered, when lab frequencies of the laser waves are always commensurate. The sensitivity of spectra with respect to the electron beam spread, focusing and finite duration of the laser beams is explored.
We have imaged five compact high-velocity clouds in HI with arcmin angular- and km/s spectral-resolution using the WSRT. Supplementary total-power data, which is fully sensitive to both the cool and warm components of HI, is available for comparison for all the sources, albeit with angular resolutions that vary from 3 to 36. The fractional HI flux in compact CNM components varies from 4% to 16% in our sample. All objects have at least one local peak in the CNM column which exceeds about 10^19 cm^-2 when observed with arcmin resolution. It is plausible that a peak column density of 1-2x10^19 cm^-2 is a prerequisite for the long-term survival of these sources. One object in our sample, CHVC120-20-443 (Davies cloud), lies in close projected proximity to the disk of M31. This object is characterized by exceptionally broad linewidths in its CNM concentrations (more than 5 times greater than the median value). These CNM concentrations lie in an arc on the edge of the source facing the M31 disk, while the diffuse HI component of this source has a position offset in the direction of the disk. All of these attributes suggest that CHVC120-20-443 is in a different evolutionary state than most of the other CHVCs which have been studied. Similarly broad CNM linewidths have only been detected in one other object, CHVC111-07-466, which also lies in the Local Group barycenter direction and has the most extreme radial velocity known. A distinct possibility for Davies cloud seems to be physical interaction of some type with M31. The most likely form of this interaction might be the ram-pressure or tidal- stripping by either one of M31s visible dwarf companions, M32 or NGC205, or else by a dark companion with an associated HI condensation.
We present measurements of the velocity distribution of calcium atoms in an atomic beam generated using a dual-stage laser back-ablation apparatus. Distributions are measured using a velocity selective Doppler time-of-flight technique. They are Boltzmann-like with rms velocities corresponding to temperatures above the melting point for calcium. Contrary to a recent report in the literature, this method does not generate a sub-thermal atomic beam.
We present a robust, continuous molecular decelerator that employs high magnetic fields and few optical pumping steps. CaOH molecules are slowed, accumulating at low velocities in a range sufficient for loading both magnetic and magneto-optical traps. During the slowing, the molecules scatter only 7 photons, removing around 8 K of energy. Because large energies can be removed with only a few spontaneous radiative decays, this method can be applied to nearly any paramagnetic atomic or molecular species, opening a general path to trapping of complex molecules.
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