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Register a new userPolariton linewidth and the reservoir temperature dynamics in a semiconductor microcavity
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A method of determining the temperature of the nonradiative reservoir in a microcavity exciton-polariton system is developed. A general relation for the homogeneous polariton linewidth is theoretically derived and experimentally used in the method. In experiments with a GaAs microcavity under nonresonant pulsed excitation, the reservoir temperature dynamics is extracted from the polariton linewidth. Within the first nanosecond the reservoir temperature greatly exceeds the lattice temperature and determines the dynamics of the major processes in the system. It is shown that, for nonresonant pulsed excitation of GaAs microcavities, the polariton Bose-Einstein condensation is typically governed by polariton-phonon scattering, while interparticle scattering leads to condensate depopulation.
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We present an experimental study on the ignition and decay of a polariton optical parametric oscillator (OPO) in a semiconductor microcavity pillar. The combination of a continuous wave laser pump, under quasi-phase matching conditions, and a non-resonant, 2 ps-long pulse probe allows us to obtain the full dynamics of the system. The arrival of the probe induces a blue-shift in the polariton emission, bringing the OPO process into resonance with the pump, which triggers the OPO-process. We time-resolve the polariton OPO signal emission for more than 1 nanosecond in both real and momentum-space. We fully characterize the emission of the OPO signal with spectral tomography techniques. Our interpretations are backed up by theoretical simulations based on the 2D coupled Gross-Pitaevskii equation for excitons and photons.
The dynamics of chaotic systems are, by definition, exponentially sensitive to initial conditions and may appear rather random. In this work, we explore relations between the chaotic dynamics of an observable and the dynamics of information (entropy) contained in this observable, focussing on a disordered metal coupled to a dissipative, e.g. phononic, bath. The chaotic dynamics is characterised by Lyapunov exponents $lambda$, the rates of growth of out-of-time order correlators (OTOCs), quantities of the form $langle[hat A(t),hat B(0)]^{2}rangleproptoexp(2lambda t)$, where $hat A$ and $hat B$ are the operators of, e.g., the total current of electrons in a metallic quantum dot. We demonstrate that the Lyapunov exponent $lambda$ matches the rate of decay of information stored in the observable $langle hat A(t)rangle$ after applying a small perturbation with a small classical uncertainty. This relation suggests a way to measure Lyapunov exponents in experiment. We compute both the Lyapunov exponent and the rate of decay of information microscopically in a disordered metal in the presence of a bosonic bath, which may, in particular, represent interactions in the system. For a sufficiently short range of the correlations in the bath, the exponent has the form $lambda=lambda_{0}-1/tau$, where $lambda_{0}$ is the (temperature-independent) Lyapunov exponent in the absence of the bath and $1/tau$ is the inelastic scattering rate. Our results demonstrate also the existence of a transition between chaotic and non-chaotic behaviour at $lambda_{0}=1/tau$, which may be triggered, e.g., by changing the temperature of the bath.
Microcavity polaritons are composite half-light half-matter quasi-particles, which have recently been demonstrated to exhibit rich physical properties, such as non-equilibrium Bose-Einstein condensation, parametric scattering and superfluidity. At the same time, polaritons have some important advantages over photons for information processing applications, since their excitonic component leads to weaker diffraction and stronger inter-particle interactions, implying, respectively, tighter localization and lower powers for nonlinear functionality. Here we present the first experimental observations of bright polariton solitons in a strongly coupled semiconductor microcavity. The polariton solitons are shown to be non-diffracting high density wavepackets, that are strongly localised in real space with a corresponding broad spectrum in momentum space. Unlike solitons known in other matter-wave systems such as Bose condensed ultracold atomic gases, they are non-equilibrium and rely on a balance between losses and external pumping. Microcavity polariton solitons are excited on picosecond timescales, and thus have significant benefits for ultrafast switching and transfer of information over their light only counterparts, semiconductor cavity lasers (VCSELs), which have only nanosecond response time.
We investigate the interactions between exciton-polaritons in N two-dimensional semiconductor layers embedded in a planar microcavity. In the limit of low-energy scattering, where we can ignore the composite nature of the excitons, we obtain exact analytical expressions for the spin-triplet and spin-singlet interaction strengths, which go beyond the Born approximation employed in previous calculations. Crucially, we find that the strong light-matter coupling enhances the strength of polariton-polariton interactions compared to that of the exciton-exciton interactions, due to the Rabi coupling and the small photon-exciton mass ratio. We furthermore obtain the dependence of the polariton interactions on the number of layers N, and we highlight the important role played by the optically dark states that exist in multiple layers. In particular, we predict that the singlet interaction strength is stronger than the triplet one for a wide range of parameters in most of the currently used transition metal dichalcogenides. This has consequences for the pursuit of polariton condensation and other interaction-driven phenomena in these materials.
Atomically thin transition metal dichalcogenides possess valley dependent functionalities that are usually available only at crogenic temperatures, constrained by various valley depolarization scatterings. The formation of exciton polaritons by coherently superimposing excitons and microcavity photons potentially harnesses the valley polarized polariton polariton interactions for novel valleytronics devices. Robust EPs have been demonstrated at room temperature in TMDs microcavity, however, the coherent polariton lasing and condensation remain elusive. Herein, we demonstrate for the first time the realization of EP condensation in a TMD microcavity at room temperature. The continuous wave pumped EP condensation and lasing with ultralow thresholdsis evidenced by the macroscopic occupation of the ground state, that undergoes a nonlinear increase of the emission and a continuous blueshift, a build up of spatial coherence, and a detuning-controlled threshold. Our work presents a critically important step towards exploiting nonlinear polariton polariton interactions and polaritonic devices with valley functionality at room temperature.
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