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Register a new userStellar abundances and presolar grains trace the nucleosynthetic origin of molybdenum and ruthenium
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Camilla Juul Hansen
Publication date
2014
fields
Physics
and research's language is
English
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This work presents a large consistent study of molybdenum (Mo) and ruthenium (Ru) abundances in the Milky Way. These two elements are important nucleosynthetic diagnostics. In our sample of 71 Galactic metal-poor field stars, we detect Ru and/or Mo in 51 of these (59 including upper limits). The sample consists of high-resolution, high signal-to-noise spectra covering both dwarfs and giants from [Fe/H]=-0.63 down to -3.16. Thus we provide information on the behaviour of Mo I and Ru I at higher and lower metallicity than is currently known. We find a wide spread in the Mo and Ru abundances, which is typical of heavy elements. This indicates that several formation processes, in addition to high entropy winds, can be responsible for the formation of Mo and Ru. The formation processes are traced by comparing Mo and Ru to elements (Sr, Zr, Pd, Ag, Ba, and Eu) with known formation processes. We find contributions from different formation channels, namely p-, slow (s-), and rapid (r-) neutron-capture processes. Molybdenum is a highly convolved element that receives contributions from several processes, whereas Ru is mainly formed by the weak r-process as is silver. We also compare our absolute elemental stellar abundances to relative isotopic abundances of presolar grains extracted from meteorites. Their isotopic abundances can be directly linked to the formation process (e.g. r-only isotopes) providing a unique comparison between observationally derived abundances and the nuclear formation process. The comparison to abundances in presolar grains shows that the r-/s-process ratios from the presolar grains match the total elemental chemical composition derived from metal-poor halo stars with [Fe/H]~ -1.5 to -1.1 dex. This indicates that both grains and stars around and above [Fe/H]=-1.5 are equally (well) mixed and therefore do not support a heterogeneous presolar nebula... Abridged.
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We report Mo isotopic compositions of 37 presolar SiC grains of types Y (19) and Z (18), rare types commonly argued to have formed in lower-than-solar metallicity asymptotic giant branch (AGB) stars. Direct comparison of the Y and Z grain data with data for mainstream grains from AGB stars of close-to-solar metallicity demonstrates that the three types of grains have indistinguishable Mo isotopic compositions. We show that the Mo isotope data can be used to constrain the maximum stellar temperatures (TMAX) during thermal pulses in AGB stars. Comparison of FRUITY Torino AGB nucleosynthesis model calculations with the grain data for Mo isotopes points to an origin from low-mass (~1.5-3 Msun) rather than intermediate-mass (>3-~9 Msun) AGB stars. Because of the low efficiency of 22Ne({alpha},n)25Mg at the low TMAX values attained in low-mass AGB stars, model calculations cannot explain the large 30Si excesses of Z grains as arising from neutron capture, so these excesses remain a puzzle at the moment.
Among presolar materials recovered in meteorites, abundant SiC and Al$_{2}$O$_{3}$ grains of AGB origins were found. They showed records of C, N, O, $^{26}$Al and s-element isotopic ratios that proved invaluable in constraining the nucleosynthesis models for AGB stars cite{zin,gal}. In particular, when these ratios are measured in SiC grains, they clearly reveal their prevalent origin in cool AGB circumstellar envelopes and provide information on both the local physics and the conditions at the nucleosynthesis site (the H- and He-burning layers deep inside the structure). Among the properties ascertained for the main part of the SiC data (the so-called {it mainstream} ones), we mention a large range of $^{14}$N/$^{15}$N ratios, extending below the solar value cite{mar}, and $^{12}$C/$^{13}$C ratios $gtrsim$ 30. Other classes of grains, instead, display low carbon isotopic ratios ($gtrsim 10$) and a huge dispersion for N isotopes, with cases of large $^{15}$N excess. In the same grains, isotopes currently feeded by slow neutron captures reveal the characteristic pattern expected from this process at an efficiency slightly lower than necessary to explain the solar main s-process component. Complementary constraints can be found in oxide grains, especially Al$_{2}$O$_{3}$ crystals. Here, the oxygen isotopes and the content in $^{26}$Al are of a special importance for clarifying the partial mixing processes that are known to affect evolved low-mass stars. Successes in modeling the data, as well as problems in explaining some of the mentioned isotopic ratios through current nucleosynthesis models are briefly outlined.
We discuss theoretical AGB predictions for hydrogen-deficient PG 1159 stars and Sakurais object, which show peculiar enhancements in He, C and O, and how these enhancements may be understood in the framework of a very late thermal pulse nucleosynthetic event. We then discuss the nucleosynthesis origin of rare subclasses of presolar grains extracted from carbonaceous meteorites, the SiC AB grains showing low 12C/13C in the range 2 to 10 and the very few high-density graphite grains with 12C/13C around 10.
Extreme excesses of $^{13}C$ ($^{12}C$/$^{13}C$<10) and $^{15}N$ ($^{14}N$/$^{15}N$<20) in rare presolar SiC grains have been considered diagnostic of an origin in classical novae, though an origin in core collapse supernovae (CCSNe) has also been proposed. We report C, N, and Si isotope data for 14 submicron- to micron-sized $^{13}C$- and $^{15}N$-enriched presolar SiC grains ($^{12}C$/$^{13}C$<16 and $^{14}N$/$^{15}N$<~100) from Murchison, and their correlated Mg-Al, S, and Ca-Ti isotope data when available. These grains are enriched in $^{13}C$ and $^{15}N$, but with quite diverse Si isotopic signatures. Four grains with $^{29,30}Si$ excesses similar to those of type C SiC grains likely came from CCSNe, which experienced explosive H burning occurred during explosions. The independent coexistence of proton- and neutron-capture isotopic signatures in these grains strongly supports heterogeneous H ingestion into the He shell in pre-supernovae. Two of the seven putative nova grains with $^{30}Si$ excesses and $^{29}Si$ depletions show lower-than-solar $^{34}S$/$^{32}S$ ratios that cannot be explained by classical nova nucleosynthetic models. We discuss these signatures within the CCSN scenario. For the remaining five putative nova grains, both nova and supernova origins are viable because explosive H burning in the two stellar sites could result in quite similar proton-capture isotopic signatures. Three of the grains are sub-type AB grains that are also $^{13}C$ enriched, but have a range of higher $^{14}N$/$^{15}N$. We found that $^{15}N$-enriched AB grains (~50<$^{14}N$/$^{15}N$<~100) have distinctive isotopic signatures compared to putative nova grains, such as higher $^{14}N$/$^{15}N$, lower $^{26}Al$/$^{27}Al$, and lack of $^{30}Si$ excess, indicating weaker proton-capture nucleosynthetic environments.
Cluster analysis of presolar silicon carbide grains based on literature data for 12C/13C, 14N/15N, {delta}30Si/28Si, and {delta}29Si/28Si including or not inferred initial 26Al/27Al data, reveals nine clusters agreeing with previously defined grain types but also highlighting new divisions. Mainstream grains reside in three clusters probably representing different parent star metallicities. One of these clusters has a compact core, with a narrow range of composition, pointing to an enhanced production of SiC grains in asymptotic giant branch (AGB) stars with a narrow range of masses and metallicities. The addition of 26Al/27Al data highlights a cluster of mainstream grains, enriched in 15N and 26Al, which cannot be explained by current AGB models. We defined two AB grain clusters, one with 15N and 26Al excesses, and the other with 14N and smaller 26Al excesses, in agreement with recent studies. Their definition does not use the solar N isotopic ratio as a divider, and the contour of the 26Al-rich AB cluster identified in this study is in better agreement with core-collapse supernova models. We also found a cluster with a mixture of putative nova and AB grains, which may have formed in supernova or nova environments. X grains make up two clusters, having either strongly correlated Si isotopic ratios or deviating from the 2/3 slope line in the Si 3-isotope plot. Finally, most Y and Z grains are jointly clustered, suggesting that the previous use of 12C/13C= 100 as a divider for Y grains was arbitrary. Our results show that cluster analysis is a powerful tool to interpret the data in light of stellar evolution and nucleosynthesis modelling and highlight the need of more multi-element isotopic data for better classification.
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