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Register a new userNon-polar Flexoelectrooptic Effect in Blue Phase Liquid Crystals
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Added by
Benjamin Outram DPhil
Publication date
2014
fields
Physics
and research's language is
English
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Blue phase liquid crystals are not usually considered to exhibit a flexoelectrooptic effect, due to the polar nature of flexoelectric switching and the cubic or amorphous structure of blue phases. Here, we derive the form of the flexoelectric contribution to the Kerr constant of blue phases, and experimentally demonstrate and measure the separate contributions to the Kerr constant arising from flexoelectric and dielectric effects. Hence, a non-polar flexoelectrooptic effect is demonstrated in blue phase liquid crystals, which will have consequences for the engineering of novel blue-phase electrooptic technology.
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Starting from a microscopic definition of an alignment vector proportional to the polarization, we discuss the hydrodynamics of polar liquid crystals with local $C_{infty v}$-symmetry. The free energy for polar liquid crystals differs from that of nematic liquid crystals ($D_{infty h}$) in that it contains terms violating the ${bf{n}}to -{bf{n}}$ symmetry. First we show that these $mathcal{Z}_2$-odd terms induce a general splay instability of a uniform polarized state in a range of parameters. Next we use the general Poisson-bracket formalism to derive the hydrodynamic equations of the system in the polarized state. The structure of the linear hydrodynamic modes confirms the existence of the splay instability.
Active fluids are intrinsically out-of-equilibrium systems due to the internal energy injection of the active constituents. We show here that a transition from a motion-less isotropic state towards a flowing polar one can be possibly driven by the sole active injection through the action of polar-hydrodynamic interactions in absence of an ad hoc free-energy which favors the development of an ordered phase. In particular, we propose an analytical argument and we perform lattice Boltzmann simulations where the appearance of large temporal fluctuations in the polar fraction of the system is observed at the transition point. Moreover, we make use of a scale-to-scale analysis to unveil the energy transfer mechanism, proving that elastic absorption plays a relevant role in the overall dynamics of the system, contrary to what reported in previous works on the usual active gel theory where this term could be factually neglected.
Liquid crystalline polymers are materials of considerable scientific interest and technological value to society [1-3]. An important subset of such materials exhibit rubber-like elasticity; these can combine the remarkable optical properties of liquid crystals with the favourable mechanical properties of rubber and, further, exhibit behaviour not seen in either type of material independently [2]. Many of their properties depend crucially on the particular mesophase employed. Stretchable liquid crystalline polymers have previously been demonstrated in the nematic, chiral nematic, and smectic mesophases [2,4]. Here were report the fabrication of a stretchable gel of blue phase I, which forms a self-assembled, three-dimensional photonic crystal that may have its optical properties manipulated by an applied strain and, further, remains electro-optically switchable under a moderate applied voltage. We find that, unlike its undistorted counterpart, a mechanically deformed blue phase exhibits a Pockels electro-optic effect, which sets out new theoretical challenges and new possibilities for low-voltage electro-optic devices.
Bulk properties of ionic liquid crystals are investigated using density functional theory. The liquid crystal molecules are represented by ellipsoidal particles with charges located in their center or at their tails. Attractive interactions are taken into account in terms of the Gay-Berne pair potential. Rich phase diagrams involving vapor, isotropic and nematic liquid, as well as smectic phases are found. The dependence of the phase behavior on various parameters such as the length of the particles and the location of charges on the particles is studied.
We analyse a recent generalised free-energy for liquid crystals posited by Virga and falling in the class of quartic functionals in the spatial gradients of the nematic director. We review some known interesting solutions, i. e., uniform heliconical structures, and we find new liquid crystal configurations, which closely resemble some novel, experimentally detected, structures called Skyrmion tubes. These new configurations are characterised by a localised pattern given by the variation of the conical angle. We study the equilibrium differential equations and find numerical solutions and analytical approximations.
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