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Register a new userAbsolute rate coefficients for photorecombination and electron-impact ionization of magnesium-like iron ions from measurements at a heavy-ion storage ring
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D. Bernhardt
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Rate coefficients for photorecombination (PR) and cross sections for electron-impact ionization (EII) of Fe$^{14+}$ forming Fe$^{13+}$ and Fe$^{15+}$, respectively, have been measured by employing the electron-ion merged-beams technique at a heavy-ion storage ring. Rate coefficients for PR and EII of Fe$^{14+}$ ions in a plasma are derived from the experimental measurements. Simple parametrizations of the experimentally derived plasma rate coefficients are provided for use in the modeling of photoionized and collisionally ionized plasmas. In the temperature ranges where Fe$^{14+}$ is expected to form in such plasmas the latest theoretical rate coefficients of Altun et al. [Astron. Astrophys. 474, 1051 (2007)] for PR and of Dere [Astron. Astrophys. 466, 771 (2007)] for EII agree with the experimental results to within the experimental uncertainties. Common features in the PR and EII resonance structures are identified and discussed.
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We report measured rate coefficients for electron-ion recombination for Si10+ forming Si9+ and for Si9+ forming Si8+, respectively. The measurements were performed using the electron-ion merged-beams technique at a heavy-ion storage ring. Electron-ion collision energies ranged from 0 to 50 eV for Si9+ and from 0 to 2000 eV for Si10+, thus, extending previous measurements for Si10+ [Orban et al. 2010, Astrophys. J. 721, 1603] to much higher energies. Experimentally derived rate coefficients for the recombination of Si9+ and Si10+ ions in a plasma are presented along with simple parameterizations. These rate coefficients are useful for the modeling of the charge balance of silicon in photoionized plasmas (Si9+ and Si10+) and in collisionally ionized plasmas (Si10+ only). In the corresponding temperature ranges, the experimentally derived rate coefficients agree with the latest corresponding theoretical results within the experimental uncertainties.
We present new experimentally measured and theoretically calculated rate coefficients for the electron-ion recombination of W$^{18+}$([Kr] $4d^{10}$ $4f^{10}$) forming W$^{17+}$. At low electron-ion collision energies, the merged-beam rate coefficient is dominated by strong, mutually overlapping, recombination resonances. In the temperature range where the fractional abundance of W$^{18+}$ is expected to peak in a fusion plasma, the experimentally derived Maxwellian recombination rate coefficient is 5 to 10 times larger than that which is currently recommended for plasma modeling. The complexity of the atomic structure of the open-$4f$-system under study makes the theoretical calculations extremely demanding. Nevertheless, the results of new Breit-Wigner partitioned dielectronic recombination calculations agree reasonably well with the experimental findings. This also gives confidence in the ability of the theory to generate sufficiently accurate atomic data for the plasma modeling of other complex ions.
We have measured electron impact ionization (EII) for Fe 7+ from the ionization threshold up to 1200 eV. The measurements were performed using the TSR heavy ion storage ring. The ions were stored long enough prior to measurement to remove most metastables, resulting in a beam of 94% ground state ions. Comparing with the previously recommended atomic data, we find that the Arnaud & Raymond (1992) cross section is up to about 40% larger than our measurement, with the largest discrepancies below about 400~eV. The cross section of Dere (2007) agrees to within 10%, which is about the magnitude of the experimental uncertainties. The remaining discrepancies between measurement and the most recent theory are likely due to shortcomings in the theoretical treatment of the excitation-autoionization contribution.
We report measurements of electron impact ionization (EII) for Fe^13+, Fe^16+, and Fe^17+ over collision energies from below threshold to above 3000 eV. The ions were recirculated using an ion storage ring. Data were collected after a sufficiently long time that essentially all the ions had relaxed radiatively to their ground state before data were collected. For single ionization of $fethirteen$ we find that previous single pass experiments are more than 40% larger than our results. Compared to our work, the theoretical cross section recommended by Arnaud & Raymond (1992) is more than 30% larger, while that of Dere (2007) is about 20% greater. Much of the discrepancy with Dere (2007) is due to the theory overestimating the contribution of excitation-autoionization via n=2 excitations. Double ionization of Fe^13+ is dominated by direct ionization of an inner shell electron accompanied by autoionization of a second electron. Our results for single ionization of Fe^16+ and Fe^17+ agree with theoretical calculations to within the experimental uncertainties.
We study double ionization of Mg by electron impact through the vantage point of classical mechanics. We consider all electron-electron correlations in a Coulomb four-body problem, where three electrons belong to the atom and the fourth electron causes the impact ionization. From our model we compute the double-ionization probability of Mg for impact energies from 15, to 125 eV. Double ionization occurs through eight double-ionization mechanisms, which we classify into four categories: inner shell capture, direct, delay and ionized inner shell mechanisms. We show that delay and ionized inner shell mechanisms require electron-electron correlations among the four electrons, and are responsible for the second increase in the double-ionization probability. Furthermore, we show that our theoretical prediction about the relative prominence of certain double ionization mechanisms is in agreement with experimental results on the relative prominence of non-first- over first-order mechanisms.
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