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Proximity effect on spin-dependent conductance and thermopower of correlated quantum dots

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 Added by Ireneusz Weymann
 Publication date 2014
  fields Physics
and research's language is English




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We study the electric and thermoelectric transport properties of correlated quantum dots coupled to two ferromagnetic leads and one superconducting electrode. Transport through such hybrid devices depends on the interplay of ferromagnetic-contact induced exchange field, superconducting proximity effect and correlations leading to the Kondo effect. We consider the limit of large superconducting gap. The system can be then modeled by an effective Hamiltonian with a particle-non-conserving term describing the creation and annihilation of Cooper pairs. By means of the full density-matrix numerical renormalization group method, we analyze the behavior of electrical and thermal conductances, as well as the Seebeck coefficient as a function of temperature, dot level position and the strength of the coupling to the superconductor. We show that the exchange field may be considerably affected by the superconducting proximity effect and is generally a function of Andreev bound state energies. Increasing the coupling to the superconductor may raise the Kondo temperature and partially restore the exchange-field-split Kondo resonance. The competition between ferromagnetic and superconducting proximity effects is reflected in the corresponding temperature and dot level dependence of both the linear conductance and the (spin) thermopower.



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The electron transport through the parabolic quantum wire placed in longitudinal magnetic field in the presence of the system of short-range impurities inside the wire is investigated. Using approach based on the zero-range potential theory we obtained an exact formula for the transmission coefficient of the electron through the wire that allows to calculate such the transport characteristics as the conductance and differential thermopower. The dependencies of conductance and thermopower on the chemical potential and magnetic field are investigated. The effect of elastic scattering due to short-range impurities on low-temperature conductance and thermopower is studied. It was shown that the character of the electron transport essentially depends on the position of the every scattering center. The presence even isolated impurity leads to destruction of conductance quantization. In some cases it is possible that thermopower can change the sign in dependence on chemical potential and magnetic field.
We analyze the equilibrium and non-equilibrium frequency-dependent spin current noise and spin conductance through a quantum dot in the local moment regime. Spin current correlations are shown to behave markedly differently from charge correlations: Equilibrium spin cross-correlations are suppressed at frequencies below the Kondo scale, and are characterized by a universal function that we determine numerically for zero temperature. For asymmetrical quantum dots dynamical spin accumulation resonance is found for frequencies of the order of the Kondo energy. At higher temperatures surprising low-frequency anomalies related to overall spin conservation appear.
Quantum dots are an important model system for thermoelectric phenomena, and may be used to enhance the thermal-to-electric energy conversion efficiency in functional materials. It is therefore important to obtain a detailed understanding of a quantum-dots thermopower as a function of the Fermi energy. However, so far it has proven difficult to take effects of co-tunnelling into account in the interpretation of experimental data. Here we show that a single-electron tunnelling model, using knowledge of the dots electrical conductance which in fact includes all-order co-tunneling effects, predicts the thermopower of quantum dots as a function of the relevant energy scales, in very good agreement with experiment.
71 - R. Scheibner 2006
We have studied the temperature dependent thermopower of gate-defined, lateral quantum dots in the Coulomb blockade regime using an electron heating technique. The line shape of the thermopower oscillations depends strongly on the contributing tunneling processes. Between 1.5 K and 40 mK a crossover from a pure sawtooth- to an intermitted sawtooth-like line shape is observed. The latter is attributed to the increasing dominance of cotunneling processes in the Coulomb blockade regime at low temperatures.
72 - R. Scheibner 2004
The thermopower of a Kondo-correlated gate-defined quantum dot is studied using a current heating technique. In the presence of spin correlations the thermopower shows a clear deviation from the semiclassical Mott relation between thermopower and conductivity. The strong thermopower signal indicates a significant asymmetry in the spectral density of states of the Kondo resonance with respect to the Fermi energies of the reservoirs. The observed behavior can be explained within the framework of an Anderson-impurity model. Keywords: Thermoelectric and thermomagnetic effects, Coulomb blockade, single electron tunneling, Kondo-effect PACS Numbers: 72.20.Pa, 73.23.Hk
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