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We investigate the thermodynamic properties and the lattice stability of two-dimensional crystalline membranes, such as graphene and related compounds, in the low temperature quantum regime $Trightarrow0$. A key role is played by the anharmonic coupling between in-plane and out-of plane lattice modes that, in the quantum limit, has very different consequences than in the classical regime. The role of retardation, namely of the frequency dependence, in the effective anharmonic interactions turns out to be crucial in the quantum regime. We identify a crossover temperature, $T^{*}$, between classical and quantum regimes, which is $sim 70 - 90$ K for graphene. Below $T^{*}$, the heat capacity and thermal expansion coefficient decrease as power laws with decreasing temperature, tending to zero for $Trightarrow0$ as required by the third law of thermodynamics.
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In this note, we reply to the comment made by E.I.Kats and V.V.Lebedev [arXiv:1407.4298] on our recent work Thermodynamics of quantum crystalline membranes [Phys. Rev. B 89, 224307 (2014)]. Kats and Lebedev question the validity of the calculation presented in our work, in particular on the use of a Debye momentum as a ultra-violet regulator for the theory. We address and counter argue the criticisms made by Kats and Lebedev to our work.
We consider open quantum systems consisting of a finite system of independent fermions with arbitrary Hamiltonian coupled to one or more equilibrium fermion reservoirs (which need not be in equilibrium with each other). A strong form of the third law of thermodynamics, $S(T) rightarrow 0$ as $Trightarrow 0$, is proven for fully open quantum systems in thermal equilibrium with their environment, defined as systems where all states are broadened due to environmental coupling. For generic open quantum systems, it is shown that $S(T)rightarrow gln 2$ as $Trightarrow 0$, where $g$ is the number of localized states lying exactly at the chemical potential of the reservoir. For driven open quantum systems in a nonequilibrium steady state, it is shown that the local entropy $S({bf x}; T) rightarrow 0$ as $T({bf x})rightarrow 0$, except for cases of measure zero arising due to localized states, where $T({bf x})$ is the temperature measured by a local thermometer.
This work brings together Keldysh non-equilibrium quantum theory and thermodynamics, by showing that a real-time diagrammatic technique is an equivalent of stochastic thermodynamics for non-Markovian quantum machines (heat engines, refrigerators, etc). Symmetries are found between quantum trajectories and their time-reverses on the Keldysh contour, for any interacting quantum system coupled to ideal reservoirs of electrons, phonons or photons. These lead to quantum fluctuation theorems the same as the well-known classical ones (Jarzynski and Crooks equalities, integral fluctuation theorem, etc), whether the systems dynamics are Markovian or not. Some of these are also shown to hold for non-factorizable initial states. The sequential tunnelling approximation and the cotunnelling approximation are both shown to respect the symmetries that ensure the fluctuation theorems. For all initial states, energy conservation ensures that the first law of thermodynamics holds on average, while the above symmetries ensures that the second law of thermodynamics holds on average, even if fluctuations violate it. [ERRATUM added: March 2021]
We provide a thermodynamically consistent description of energy, charge and spin transfers in a thermoelectric quantum-dot spin valve in the collinear configuration based on nonequilibrium Greens function and full counting statistics. We use the fluctuation theorem symmetry and the concept of entropy production to characterize the efficiency with which thermal gradients can transduce charges or spins against their chemical potentials, arbitrary far from equilibrium. Close to equilibrium, we recover the Onsager reciprocal relations and the connection to linear response notions of performance such as the figure of merit. We also identify regimes where work extraction is more efficient far then close from equilibrium.
We report on fabrication and characterization of ultra-thin suspended single crystalline flat silicon membranes with thickness down to 6 nm. We have developed a method to control the strain in the membranes by adding a strain compensating frame on the silicon membrane perimeter to avoid buckling of the released membranes. We show that by changing the properties of the frame the strain of the membrane can be tuned in controlled manner. Consequently, both the mechanical properties and the band structure can be engineered and the resulting membranes provide a unique laboratory to study low-dimensional electronic, photonic and phononic phenomena.
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