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Register a new userSpin reversal in Fe8 under fast pulsed magnetic fields
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We report measurements on magnetization reversal in the Fe$_8$ molecular magnet using fast pulsed magnetic fields of 1.5 kT/s and in the temperature range of 0.6-4.1 K. We observe and analyze the temperature dependence of the reversal process, which involves in some cases several resonances. Our experiments allow observation of resonant quantum tunneling of magnetization up to a temperature of $sim$ 4 K. We also observe shifts of the resonance fields in temperature that suggest the emergence of a thermal instability---a combination of spin reversal and self-heating that may result in a magnetic deflagration process. The results are mainly understood in the framework of thermally-activated quantum tunneling transitions in combination with emergence of a thermal instability.
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The magneto-conductance of an open carbon nanotube (CNT)-quantum wire was measured in pulsed magnetic fields. At low temperatures we find a peculiar split magneto-conductance peak close to the charge neutrality point. Our analysis of the data reveals that this splitting is intimately connected to the spin-orbit interaction and the tube chirality. Band structure calculations suggest that the current in the peak regions is highly spin-polarized, which calls for application in future CNT-based spintronic devices.
The reversal of spins in a magnetic material as they relax toward equilibrium is accompanied by the release of Zeeman energy which can lead to accelerated spin relaxation and the formation of a well-defined self-sustained propagating spin-reversal front known as magnetic deflagration. To date, studies of Mn$_{12}$-acetate single crystals have focused mainly on deflagration in large longitudinal magnetic fields and found a fully spin-reversed final state. We report a systematic study of the effect of transverse magnetic field on magnetic deflagration and demonstrate that in small longitudinal fields the final state consists of only partially reversed spins. Further, we measured the front speed as a function of applied magnetic field. The theory of magnetic deflagration, together with a modification that takes into account the partial spin reversal, fits the transverse field dependence of the front speed but not its dependence on longitudinal field. The most significant result of this study is the finding of a partially spin-reversed final state, which is evidence that the spins at the deflagration front are also only partially reversed.
The synthesis, crystal structure and magnetic characterization of a high spin cluster comprising eight iron ions, are presented in this contribution. The cluster has formula [(tacn)6Fe8O2(OH)12Br4.3(ClO4)3.7]6H2O, (Fe8PCL) where tacn is the organic ligand 1,4,7-triazacyclononane. It can be considered a derivative of Fe8Br8, a cluster whose low temperature dynamics of the magnetization has been deeply investigated, where four of the bromide ions have been replaced by perchlorate anions. The structure of the central core of the two molecules, [Fe8O(OH)12(tacn)6]8+, is essentially the same, but Fe8PCL has a higher symmetry (Fe8Br8 crystallizes in the acentric P1 space group, while Fe8PCL crystallizes in the P21/c space group, monoclinic). The magnetic properties of Fe8PCL suggest it is very similar to Fe8Br having a S=10 ground state as well. The zero field splitting parameters were accurately determined by HF-EPR measurements. The two clusters have similar axial anisotropy but Fe8PCL has a larger transverse anisotropy. Ac susceptibility measurements revealed the cluster behaves like a superparamagnetic particle. However, due to the occurrence of large terms in the transverse anisotropy, the temperature dependence of the relaxation time can not be reproduced by a simple Arrhenius law. As observed in Fe8Br8, below 350 mK the relaxation time becomes temperature independent, indicating that a pure tunneling regime is attained. The comparison of the tunneling rate in the two clusters shows that in the perchlorate derivative the relaxation process is 35 times faster. The observed ratio of the tunneling rates is in reasonable agreement with that calculated from the tunneling splitting, i.e. the energy difference between the two almost degenerate lowest levels Ms = +/-10, in the two clusters.
We study the dynamics of a localized spin-1/2 driven by a time-periodic magnetic field that undergoes a topological transition. Despite the strongly non-adiabatic effects dominating the spin dynamics, we find that the fields topology appears clearly imprinted in the Floquet spin states through an effective Berry phase emerging in the quasienergy. This has remarkable consequences on the spin resonance condition suggesting a whole new class of experiments to spot topological transitions in the dynamics of spins and other two-level systems, from nuclear magnetic resonance to strongly-driven superconducting qubits.
We have measured the dynamic alignment properties of single-walled carbon nanotube (SWNT) suspensions in pulsed high magnetic fields through linear dichroism spectroscopy. Millisecond-duration pulsed high magnetic fields up to 56 T as well as microsecond-duration pulsed ultrahigh magnetic fields up to 166 T were used. Due to their anisotropic magnetic properties, SWNTs align in an applied magnetic field, and because of their anisotropic optical properties, aligned SWNTs show linear dichroism. The characteristics of their overall alignment depend on several factors, including the viscosity and temperature of the suspending solvent, the degree of anisotropy of nanotube magnetic susceptibilities, the nanotube length distribution, the degree of nanotube bundling, and the strength and duration of the applied magnetic field. In order to explain our data, we have developed a theoretical model based on the Smoluchowski equation for rigid rods that accurately reproduces the salient features of the experimental data.
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