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Topological quantum phases of ${^4}$He confined to nanoporous materials

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 Added by Lode Pollet
 Publication date 2014
  fields Physics
and research's language is English




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The ground state of $^4$He confined in a system with the topology of a cylinder can display properties of a solid, superfluid and liquid crystal. This phase, which we call compactified supersolid (CSS), originates from wrapping the basal planes of the bulk hcp solid into concentric cylindrical shells, with several central shells exhibiting superfluidity along the axial direction. Its main feature is the presence of a topological defect which can be viewed as a disclination with Frank index $n=1$ observed in liquid crystals, and which, in addition, has a superfluid core. The CSS as well as its transition to an insulating compactified solid with a very wide hysteresis loop are found by ab initio Monte Carlo simulations. A simple analytical model captures qualitatively correctly the main property of the CSS -- a gradual decrease of the superfluid response with increasing pressure.



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$^4$He confined in nanoporous Gelsil glass is a unique, strongly correlated Bose system exhibiting quantum phase transition (QPT) by controlling pressure. Previous studies revealed that the QPT occurs with four - dimensional (4D) XY criticality, which appears in the zero-temperature limit of the superfluid density. However, the $P-T$ phase diagram also suggested that 4D XY nature appears at finite temperatures. Here, we have determined the critical exponent of the superfluid density of $^4$He in two Gelsil samples that have pore diameter to be about 3 nm, using a newly developed mechanical resonator technique. The critical exponent $zeta$ in the powerlaw fitting $rho_{mathrm s} propto left| 1 - T/T_{mathrm c} right| ^{zeta}$, where $T_{mathrm c}$ is the superfluid transition temperature, was found to be 1.0 $pm$ 0.1 for all pressures realized in this experiment, 0.1 $<$ $P$ $<$ 2.4 MPa. This value of $zeta$ gives a decisive evidence that the finite-temperature superfluid transition belongs to 4D XY universality class. The emergence of the 4D XY criticality is explained by the existence of many nanoscale superfluid droplets, the so called localized Bose - Einstein condensates (LBECs), above $T_{mathrm c}$. Due to the large energy cost for $^4$He atoms to move between the LBECs, the phase of the LBEC order parameters fluctuates not only in spatial (3D) but imaginary time ($+1$D) dimensions, resulting in the 4D XY criticality by a temperature near $T_{mathrm c}$, which is determined by the finite size of the system in the imaginary time dimension. Below $T_{mathrm c}$, macroscopic superfluidity grows in the nanopores of Gelsil by the alignment of the phases of the LBEC order parameters. An excess dissipation peak observed below $T_{mathrm c}$ is well explained by this phase matching process.
The low temperature phase diagram of $^4$He adsorbed on a single graphene sheet is studied by computer simulation of a system comprising nearly thousand helium atoms. In the first layer, two commensurate solid phases are observed, with fillings 1/3 and 7/16 respectively, separated by a domain wall phase, as well as an incommensurate crystal at higher coverage. No evidence of a thermodynamically stable superfliuid phase is found for the first adlayer. Second layer promotion occurs at a coverage of 0.111(4) $AA^{-2}$. In the second layer two phases are observed, namely a superfluid and an incommensurate solid, with no commensurate solid intervening between these two phases. The computed phase diagram closely resembles that predicted for helium on graphite.
$^4$He confined in nanoporous media is a model Bose system that exhibits quantum phase transition (QPT) by varying pressure. We have precisely determined the critical exponent of the superfluid density of $^4$He in porous Gelsil glasses with pore size of 3.0 nm using the Helmholtz resonator technique. The critical exponent $zeta$ of the superfluid density was found to be 1.0 $pm$ 0.1 for the pressure range 0.1 < P < 2.4 MPa. This value provides decisive evidence that the finite-temperature superfluid transition belongs to the four-dimensional (4D) XY universality class, in contrast to the classical 3D XY one in bulk liquid 4He, in which $zeta$ = 0.67. The quantum critical behavior at a finite temperature is understood by strong phase fluctuation in local Bose-Einstein condensates above the superfluid transition temperature. $^4$He in nanoporous media is a unique example in which quantum criticality emerges not only at 0 K but at finite temperatures.
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We describe the first observations on the time-dependent dissipation when the drive level of a torsional oscillator containing solid He-4 is abruptly changed. The relaxation of dissipation in solid He-4 shows rich dynamical behavior including exponential and logarithmic time-dependent decays, hysteresis, and memory effects.
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The non-classical rotational inertia fraction of the identical cylindrical solid $^4$He below 300 mK is studied at 496 and 1173 Hz by a double resonance torsional oscillator. Below 35 mK, the fraction is the same at sufficiently low rim velocities. Above 35 mK, the fraction is greater for the higher than the lower mode. The dissipation peak of the lower mode occurs at a temperature $sim$ 4 mK lower than that of the higher mode. The drive dependence of the two modes shows that the reduction of the fraction is characterized by critical velocity, textit{not} amplitude nor acceleration.
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