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Register a new userImaging surface plasmons: from leaky waves to far-field radiation
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We show that, contrary to the common wisdom, surface plasmon poles are not involved in the imaging process in leakage radiation microscopy. Identifying the leakage radiation modes directly from a transverse magnetic potential leads us to reconsider the surface plasmon field and unfold the non-plasmonic contribution to the image formation. While both contributions interfere in the imaging process, our analysis reveals that the reassessed plasmonic field embodies a pole mathematically similar to the usual surface plasmon pole. This removes a long-standing ambiguity associated with plasmonic signals in leakage radiation microscopy.
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In the past decade, advances in nanotechnology have led to the development of plasmonic nanocavities which facilitate light-matter strong coupling in ambient conditions. The most robust example is the nanoparticle-on-mirror (NPoM) structure whose geometry is controlled with subnanometer precision. The excited plasmons in such nanocavities are extremely sensitive to the exact morphology of the nanocavity, giving rise to unexpected optical behaviors. So far, most theoretical and experimental studies on such nanocavities have been based solely on their scattering and absorption properties. However, these methods do not provide a complete optical description of a NPoM. Here, the NPoM is treated as an open non-conservative system supporting a set of photonic quasinormal modes (QNMs). By investigating the morphology-dependent optical properties of nanocavities, we propose a simple yet comprehensive nomenclature based on spherical harmonics and report spectrally overlapping bright and dark nanogap eigenmodes. The near-field and far-field optical properties of NPoMs are explored and reveal intricate multi-modal interactions.
Abbes resolution limit, one of the best-known physical limitations, poses a great challenge for any wave systems in imaging, wave transport, and dynamics. Originally formulated in linear optics, this Abbes limit can be broken using nonlinear optical interactions. Here we extend the Abbe theory into a nonlinear regime and experimentally demonstrate a far-field, label-free, and scan-free super-resolution imaging technique based on nonlinear four-wave mixing to retrieve near-field scattered evanescent waves, achieving sub-wavelength resolution of $lambda/15.6$. This method paves the way for application in biomedical imaging, semiconductor metrology, and photolithography.
Recently it was reported that deeply subwavelength features of free space superoscillatory electromagnetic fields can be observed experimentally and used in optical metrology with nanoscale resolution [Science 364, 771 (2019)]. Here we introduce a new type of imaging, termed Deeply Subwavelength Superoscillatory Imaging (DSSI), that reveals the fine structure of a physical object through its far-field scattering pattern under superoscillatory illumination. The object is reconstructed from intensity profiles of scattered light recorded for different positions of the object in the superoscillatory field. The reconstruction is performed with a convolutional neural network trained on a large number of scattering events. We show that DSSI offers resolution far beyond the conventional diffraction limit. In modelling experiments, a dimer comprising two subwavelength opaque particles is imaged with a resolution exceeding ${lambda}/200$.
Infrared spectroscopy, especially for molecular vibrations in the fingerprint region between 600 and 1500 cm-1, is a powerful characterization method for bulk materials. However, molecular fingerprinting at the nanoscale level still remains a significant challenge, due to weak light-matter interaction between micron-wavelengthed infrared light and nano-sized molecules. Here, we demonstrate molecular fingerprinting at the nanoscale level using our specially designed graphene plasmonic structure on CaF2 nanofilm. This structure not only avoids the plasmon-phonon hybridization, but also provides in situ electrically-tunable graphene plasmon covering the entire infrared fingerprint region, which was previously unattainable. In addition, undisturbed and highly-confined graphene plasmon offers simultaneous detection of in-plane and out-of-plane vibrational modes with ultrahigh detection sensitivity down to the sub-monolayer level, significantly pushing the current detection limit of far-field mid-infrared spectroscopy. Our results provide a platform, fulfilling the long-awaited expectation of high sensitivity and selectivity far-field fingerprint detection of nano-scale molecules for numerous applications.
Imaging below the diffraction limit is always a public interest because of the restricted resolution of conventional imaging systems. To beat the limit, evanescent harmonics decaying in space must participate in the imaging process. Here, we introduce the method of spatial spectrum sampling, a novel far-field superresolution imaging method for microwave and terahertz regime. Strong dispersion and momentum conservation allow the spoof surface plasmon polaritons (SSP) structure to become a sensitive probe for spatial harmonics. This enables that the spatial information of the targets including both propagating and evanescent components, can be extracted by tuning and recording SSP in the far field. Then, the subwavelength resolution is constructed by the inversed Fourier transform of the sampled spatial spectrum. Using the modified subwavelength metallic grating as the spoof plasmonic structure, a far-field resolution of 0.17 wavelength is numerically and experimentally verified, and two-dimensional imaging ability is also fully discussed. The imaging ability and flexibility can be further optimizing the SSP structures. We are confident that our working mechanism will have great potentials in the superresolution imaging applications in the microwave and terahertz frequency range
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