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Register a new userDynamic Spin Fluctuations at $Trightarrow 0$ in a Spin-1/2 Ferromagnetic Kagome Lattice
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We report magnetization, electron spin resonance (ESR), and muon spin relaxation ($mu $SR) measurements on single crystals of the $S=1/2$ (Cu$% ^{+2}$) kagom{e} compound Cu(1,3-benzendicarboxylate). The $mu $SR is carried to temperatures as low as 45 mK. The spin Hamiltonian parameters are determined from the analysis of the magnetization and ESR data. We find that this compound has anisotropic ferromagnetic interactions. Nevertheless, no spin freezing is observed even at temperatures two orders of magnitude lower than the coupling constants. In light of this finding, the relation between persistent spin dynamics and spin liquid are reexamined.
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The topological quantum spin liquids (SL) and the nature of quantum phase transitions between them have attracted intensive attentions for the past twenty years. The extended kagome spin-1/2 antiferromagnet emerges as the primary candidate for hosting both time reversal symmetry (TRS) preserving and TRS breaking SLs based on density matrix renormalization group simulations. To uncover the nature of the novel quantum phase transition between the SL states, we study a minimum XY model with the nearest neighbor (NN) ($J_{xy}$), the second and third NN couplings ($J_{2xy}=J_{3xy}=J_{xy}$). We identify the TRS broken chiral SL (CSL) with the turn on of a small perturbation $J_{xy}sim 0.06 J_{xy}$, which is fully characterized by the fractionally quantized topological Chern number and the conformal edge spectrum as the $ u=1/2$ fractional quantum Hall state. On the other hand, the NN XY model ($J_{xy}=0$) is shown to be a critical SL state adjacent to the CSL, characterized by the gapless spin singlet excitations and also vanishing small spin triplet excitations. The quantum phase transition from the CSL to the gapless critical SL is driven by the collapsing of the neutral (spin singlet) excitation gap. By following the evolution of entanglement spectrum, we find that the transition takes place through the coupling of the edge states with opposite chiralities, which merge into the bulk and become gapless neutral excitations. The effect of the NN spin-$z$ coupling $J_z$ is also studied, which leads to a quantum phase diagram with an extended regime for the gapless SL.
Using muon spin resonance we examine the organometallic hybrid compound Cu(1,3-benzenedicarboxylate) [Cu(1,3-bdc)], which has structurally perfect spin 1/2 copper kagome planes separated by pure organic linkers. This compound has antiferromagnetic interactions with Curie-Weiss temperature of -33 K. We found slowing down of spin fluctuations starting at T=1.8 K, and that the state at T->0 is quasi-static with no long-range order and extremely slow spin fluctuations at a rate of 3.6 1/usec. This indicates that Cu(1,3-bdc) behaves as expected from a kagome magnet and could serve as a model kagome compound.
We use inelastic neutron scattering to study acoustic phonons and spin excitations in single crystals of NaFeAs, a parent compound of iron pnictide superconductors. NaFeAs exhibits a tetragonal-to-orthorhombic structural transition at $T_sapprox 58$ K and a collinear antiferromagnetic (AF) order at $T_Napprox 45$ K. While longitudinal and out-of-plane transverse acoustic phonons behave as expected, the in-plane transverse acoustic phonons reveal considerable softening on cooling to $T_s$, and then harden on approaching $T_N$ before saturating below $T_N$. In addition, we find that spin-spin correlation lengths of low-energy magnetic excitations within the FeAs layer and along the $c$-axis increase dramatically below $T_s$, and show weak anomaly across $T_N$. These results suggest that the electronic nematic phase present in the paramagnetic tetragonal phase is closely associated with dynamic spin-lattice coupling, possibly arising from the one-phonon-two-magnon mechanism.
We study numerically the spin-1/2 XXZ model in a field on an infinite Kagome lattice. We use different algorithms based on infinite Projected Entangled Pair States (iPEPS) for this, namely: (i) with simplex tensors and 9-site unit cell, and (ii) coarse-graining three spins in the Kagome lattice and mapping it to a square-lattice model with nearest-neighbor interactions, with usual PEPS tensors, 6- and 12-site unit cells. Similarly to our previous calculation at the SU(2)-symmetric point (Heisenberg Hamiltonian), for any anisotropy from the Ising limit to the XY limit, we also observe the emergence of magnetization plateaus as a function of the magnetic field, at $m_z = frac{1}{3}$ using 6- 9- and 12-site PEPS unit cells, and at $m_z = frac{1}{9}, frac{5}{9}$ and $frac{7}{9}$ using a 9-site PEPS unit cell, the later set-up being able to accommodate $sqrt{3} times sqrt{3}$ solid order. We also find that, at $m_z = frac{1}{3}$, (lattice) nematic and $sqrt{3} times sqrt{3}$ VBC-order states are degenerate within the accuracy of the 9-site simplex-method, for all anisotropy. The 6- and 12-site coarse-grained PEPS methods produce almost-degenerate nematic and $1 times 2$ VBC-Solid orders. Within our accuracy, the 6-site coarse-grained PEPS method gives slightly lower energies, which can be explained by the larger amount of entanglement this approach can handle, even when the PEPS unit-cell is not commensurate with the expected ground state. Furthermore, we do not observe chiral spin liquid behaviors at and close to the XY point, as has been recently proposed. Our results are the first tensor network investigations of the XXZ spin chain in a field, and reveal the subtle competition between nearby magnetic orders in numerical simulations of frustrated quantum antiferromagnets, as well as the delicate interplay between energy optimization and symmetry in tensor networks.
We revisit the description of the low-energy singlet sector of the spin-1/2 Heisenberg antiferromagnet on kagome in terms of an effective quantum dimer model. With the help of exact diagonalizations of appropriate finite-size clusters, we show that the embedding of a given process in its kagome environment leads to dramatic modifications of the amplitudes of the elementary loop processes, an effect not accessible to the standard approach based on the truncation of the Hamiltonian to the nearest-neighbour valence-bond basis. The resulting parameters are consistent with a Z$_2$ spin liquid rather than with a valence-bond crystal, in agreement with the last density matrix renormalization group results.
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