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Register a new userInverse counting statistics for stochastic and open quantum systems: the characteristic polynomial approach
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We consider stochastic and open quantum systems with a finite number of states, where a stochastic transition between two specific states is monitored by a detector. The long-time counting statistics of the observed realizations of the transition, parametrized by cumulants, is the only available information about the system. We present an analytical method for reconstructing generators of the time evolution of the system compatible with the observations. The practicality of the reconstruction method is demonstrated by the examples of a laser-driven atom and the kinetics of enzyme-catalyzed reactions. Moreover, we propose cumulant-based criteria for testing the non-classicality and non-Markovianity of the time evolution, and lower bounds for the system dimension. Our analytical results rely on the close connection between the cumulants of the counting statistics and the characteristic polynomial of the generator, which takes the role of the cumulant generating function.
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As the dimensions of physical systems approach the nanoscale, the laws of thermodynamics must be reconsidered due to the increased importance of fluctuations and quantum effects. While the statistical mechanics of small classical systems is relatively well understood, the quantum case still poses challenges. Here we set up a formalism that allows to calculate the full probability distribution of energy exchanges between a periodically driven quantum system and a thermalized heat reservoir. The formalism combines Floquet theory with a generalized master equation approach. For a driven two-level system and in the long-time limit, we obtain a universal expression for the distribution, providing clear physical insight into the exchanged energy quanta. We illustrate our approach in two analytically solvable cases and discuss the differences in the corresponding distributions. Our predictions could be directly tested in a variety of systems, including optical cavities and solid-state devices.
The experimental verification of quantum fluctuation relations for driven open quantum system is currently a challenge, due to the conceptual and operative difficulty of distinguishing work and heat. The Nitrogen-Vacancy center in diamond has been recently proposed as a controlled test bed to study fluctuation relations in the presence of an engineered dissipative channel, in absence of work [Hernandez-Gomez et al., Phys. Rev. Research 2, 023327 (2020)]. Here, we extend those studies to exploring the validity of quantum fluctuation relations in a driven-dissipative scenario, where the spin exchanges energy both with its surroundings because of a thermal gradient, and with an external work source. We experimentally prove the validity of the quantum fluctuation relations in the presence of cyclic driving in two cases, when the spin exchanges energy with an effective infinite-temperature reservoir, and when the total work vanishes at stroboscopic times -- although the power delivered to the NV center is non-null. Our results represent the first experimental study of quantum fluctuation relation in driven open quantum systems.
The possibility of discriminating the statistics of a thermal bath using indirect measurements performed on quantum probes is presented. The scheme relies on the fact that, when weakly coupled with the environment of interest, the transient evolution of the probe toward its final thermal configuration, is strongly affected by the fermionic or bosonic nature of the bath excitations. Using figures of merit taken from quantum metrology such as the Holevo-Helstrom probability of error and the Quantum Chernoff bound, we discuss how to achieve the greatest precision in this statistics tagging procedure, analyzing different models of probes and different initial preparations and by optimizing over the time of exposure of the probe.
An open quantum system that is put in contact with an infinite bath is pushed towards equilibrium, while the state of the bath remains unchanged. If the bath is finite, the open system still relaxes to equilibrium, but it induces a dynamical evolution of the bath state. In this work, we extend the weak-coupling master equation approach of open quantum systems interacting with finite baths to include imprecise measurements of the bath energy. Those imprecise measurements are not only always the case in practice, but they also unify the theoretical description. We investigate the circumstances under which our equation reduces to the more standard Born-Markov-secular master equation. As a result, we obtain a hierarchy of master equations that improve their accuracy by including more dynamical information about the bath. We discuss this formalism in detail for a particular non-interacting environment where the Boltzmann temperature and the Kubo-Martin-Schwinger relation naturally arise. Finally, we apply our hierarchy of master equations to study the central spin model.
Perturbation theory (PT) is a powerful and commonly used tool in the investigation of closed quantum systems. In the context of open quantum systems, PT based on the Markovian quantum master equation is much less developed. The investigation of open systems mostly relies on exact diagonalization of the Liouville superoperator or quantum trajectories. In this approach, the system size is rather limited by current computational capabilities. Analogous to closed-system PT, we develop a PT suitable for open quantum systems. This proposed method is useful in the analytical understanding of open systems as well as in the numerical calculation of system properties, which would otherwise be impractical.
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