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The radiative heat transfer between gold nanoparticle layers is presented using the coupled dipole method. Gold nanoparticles are modelled as effective electric and magnetic dipoles interacting via electromagnetic fluctuations. The effect of higher-order multipoles is implemented in the expression of electric polarizability to calculate the interactions at short distances. Our findings show that the near-field radiation reduces as the radius of the nanoparticles is increased. Also, the magnetic dipole contribution to the heat exchange becomes more important for larger particles. When one layer is displayed in parallel with respect to the other layer, the near-field heat transfer exhibits oscillatory-like features due to the influence of the individual nanostructures. Further details about the effect of the nanoparticles size are also discussed.
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Extreme near-field heat transfer between metallic surfaces is a subject of debate as the state-of-the-art theory and experiments are in disagreement on the energy carriers driving heat transport. In an effort to elucidate the physics of extreme near-field heat transfer between metallic surfaces, this Letter presents a comprehensive model combining radiation, acoustic phonon and electron transport across sub-10-nm vacuum gaps. The results obtained for gold surfaces show that in the absence of bias voltage, acoustic phonon transport is dominant for vacuum gaps smaller than ~2 nm. The application of a bias voltage significantly affects the dominant energy carriers as it increases the phonon contribution mediated by the long-range Coulomb force and the electron contribution due to a lower potential barrier. For a bias voltage of 0.6 V, acoustic phonon transport becomes dominant at a vacuum gap of 5 nm, whereas electron tunneling dominates at sub-1-nm vacuum gaps. The comparison of the theory against experimental data from the literature suggests that well-controlled measurements between metallic surfaces are needed to quantify the contributions of acoustic phonon and electron as a function of the bias voltage.
The dynamic heat transfer between two half-spaces separated by a vacuum gap due to coupling of their surface modes is modelled using the theory that describes the dynamic energy transfer between two coupled harmonic oscillators each separately connected to a heat bath and with the heat baths maintained at different temperatures. The theory is applied for the case when the two surfaces are made up of a polar crystal which supports surface polaritons that can be excited at room temperature and the predicted heat transfer is compared with the steady state heat transfer value calculated from standard fluctuational electrodynamics theory. It is observed that for small time intervals the value of heat flux can reach as high as 1.5 times that of steady state value.
We explore in the present work the near-field radiative heat transfer between two semi-infinite parallel nonlocal dielectric planes by means of fluctuational electrodynamics. We use atheory for the nonlocal dielectric permittivityfunction proposed byHalevi and Fuchs. This theory has the advantage to includedifferent models performed in the literature. According to this theory, the nonlocal dielectric function is described by a Lorenz-Drude like single oscillator model, in which the spatial dispersion effects are represented by an additional term depending on the square of the total wavevector k. The theory takes into account the scattering of the electromagneticexcitation at the surface of the dielectric material, which leads to the need of additional boundary conditions in order to solve Maxwells equations and treat the electromagnetic transmission problem. The additional boundary conditions appear as additional surface scattering parameters in the expressions of the surface impedances. It is shown that the nonlocal modeling deviates from the classical $1/d^2$ law in the nanometerrangeat distances still larger than the ones where quantum effects are expected to come into play.
Micro-nanoparticle systems have wide applications in thermal science and technology. In dense particulate system, the particle separation distance may be less than the characteristic thermal wavelength and near field effect will be significant and become a key factor to influence thermal radiation transfer in the system. In this study, radiative heat transfer (RHT) between two metallic nanoparticles clusters are explored using many-body radiative heat transfer theory implemented with the coupled electric and magnetic dipole (CEMD) approach, which effectively takes into account the contribution of magnetic polarization of metallic nanoparticles on heat exchange. As the focus, the effects of magnetic polarization and many-body interaction (MBI) on RHT were analyzed. The effects of fractal dimension and relative orientation of the clusters were also analyzed. Results show that the contribution of magnetically polarized eddy-current Joule dissipation dominates the RHT between Ag nanoparticle clusters. If only electric polarization (EP approach) is considered, the heat conductance will be underestimated as compared with the CEMD approach in both near field and far field regime. The effect of MBI on the RHT between Ag nanoparticle clusters is unobvious at room temperature, which is quite different from the SiC nanoparticle clusters. For the latter, MBI tends to suppress RHT significantly. The relative orientation has remarkable effect on radiative heat flux for clusters with lacy structure when the separation distance is in the near field. While for the separation distance in far field, both the relative orientation and the fractal dimension has a weak influence on radiative heat flux. This work will help the understanding of thermal transport in dense particulate system.
The spectral characteristics of near-field thermal emission from nanoparticle arrays are explained by comparison to the dispersions for propagating modes. Using the coupled dipole model, we analytically calculate the spectral emission from single particles, chains, planes, and 3D arrays of SiO2 and SiC. We show that the differences in their spectra are due to the existence or absence of propagating surface phonon polariton modes and that the emission is dominated by these modes when they are present. This work paves the way for understanding and control of near-field radiation in nanofluids, nanoparticle beds, and certain metamaterials.
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