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Huge thermoelectric effects in ferromagnet-superconductor junctions in the presence of a spin-splitting field

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 Added by Asier Ozaeta
 Publication date 2013
  fields Physics
and research's language is English




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We show that a huge thermoelectric effect can be observed by contacting a superconductor whose density of states is spin-split by a Zeeman field with a ferromagnet with a non-zero polarization. The resulting thermopower exceeds $k_B/e$ by a large factor, and the thermoelectric figure of merit $ZT$ can far exceed unity, leading to heat engine efficiencies close to the Carnot limit. We also show that spin-polarized currents can be generated in the superconductor by applying a temperature bias.



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Thermoelectric effects result from the coupling of charge and heat transport, and can be used for thermometry, cooling and harvesting of thermal energy. The microscopic origin of thermoelectric effects is a broken electron-hole symmetry, which is usually quite small in metal structures, and vanishes at low temperatures. We report on a combined experimental and theoretical investigation of thermoelectric effects in superconductor/ferromagnet hybrid structures. We investigate the depencence of thermoelectric currents on the thermal excitation, as well as on the presence of a dc bias voltage across the junction. Large thermoelectric effects are observed in superconductor/ferromagnet and superconductor/normal-metal hybrid structures. The spin-independent signals observed under finite voltage bias are shown to be reciprocal to the physics of superconductor/normal-metal microrefrigerators. The spin-dependent thermoelectric signals in the linear regime are due to the coupling of spin and heat transport, and can be used to design more efficient refrigerators
65 - S. Kolenda , M. J. Wolf , 2015
We report on the experimental observation of thermoelectric currents in superconductor-ferromagnet tunnel junctions in high magnetic fields. The thermoelectric signals are due to a spin-dependent lifting of particle-hole symmetry, and are found to be in excellent agreement with recent theoretical predictions. The maximum Seebeck coefficient inferred from the data is about $-100~mathrm{mu V/K}$, much larger than commonly found in metallic structures. Our results directly prove the coupling of spin and heat transport in high-field superconductors.
233 - T. Kirzhner , G. Koren 2010
Measurements of the differential conductance spectra of YBa2Cu3O7-SrRuO3 and YBa2Cu3O7-La0.67Ca_0.33MnO3 ramp-type junctions along the node and anti-node directions are reported. The results are consistent with a crossed Andreev reflection effect only in YBa2Cu3O7-SrRuO3 junctions where the domain wall width of SrRuO3 is comparable with the coherence length of YBa2Cu3O7. No such effect was observed in the YBa2Cu3O7-La0.67Ca0.33MnO3 junctions, which is in line with the much larger (x10) domain wall width of La0.67Ca0.33MnO3. We also show that crossed Andreev exists only in the anti-node direction. Furthermore, we find evidence that crossed Andreev in YBa2Cu3O7 junctions is not sensitive to nm-scale interface defects, suggesting that the length scale of the crossed Andreev effect is larger than the coherence length, but still smaller than the La0.67Ca0.33MnO3s domain wall width.
We investigate the charge and spin transport in half-metallic ferromagnet ($F$) and superconductor ($S$) nanojunctions. We utilize a self-consistent microscopic method that can accommodate the broad range of energy scales present, and ensures proximity effects that account for the interactions at the interfaces are accurately determined. Two experimentally relevant half-metallic junction types are considered: The first is a $F_1 F_2 S$ structure, where a half-metallic ferromagnet $F_1$ adjoins a weaker conventional ferromagnet $F_2$. The current is injected through the $F_1$ layer by means of an applied bias voltage. The second configuration involves a $S F_1 F_2 F_3 S$ Josephson junction whereby a phase difference $Deltavarphi$ between the two superconducting electrodes generates the supercurrent flow. In this case, the central half-metallic $F_2$ layer is surrounded by two weak ferromagnets $F_1$ and $F_3$. By placing a ferromagnet with a weak exchange field adjacent to an $S$ layer, we are able to optimize the conversion process in which opposite-spin triplet pairs are converted into equal-spin triplet pairs that propagate deep into the half-metallic regions in both junction types. For the tunnel junctions, we study the bias-induced local magnetization, spin currents, and spin transfer torques for various orientations of the relative magnetization angle $theta$ in the $F$ layers. We find that the bias-induced equal-spin triplet pairs are maximized in the half-metal for $thetaapprox90^circ$ and as part of the conversion process, are anticorrelated with the opposite-spin pairs. We show that the charge current density is maximized, corresponding to the occurrence of a large amplitude of equal-spin triplet pairs, when the exchange interaction of the weak ferromagnet is about $0.1E_F.$
We theoretically study the electronic transport through a ferromagnet-Ising superconductor junction. A tight-binding Hamiltonian describing the Ising superconductor is presented. Then by combing the non-equilibrium Greens function method, the expressions of Andreev reflection coefficient and conductance are obtained. A strong magnetoanisotropic spin-triplet Andreev reflection is shown, and the magnetoanisotropic period is $pi$ instead of $2pi$ as in the conventional magnetoanisotropic system. We demonstrate a significant increase of the spin-triplet Andreev reflection for the single-band Ising superconductor. Furthermore, the dependence of the Andreev reflection on the incident energy and incident angle are also investigated. A complete Andreev reflection can occur when the incident energy is equal to the superconductor gap, regardless of the Fermi energy (spin polarization) of the ferromagnet. For the suitable oblique incidence, the spin-triplet Andreev reflection can be strongly enhanced. In addition, the conductance spectroscopies of both zero bias and finite bias are studied, and the influence of gate voltage, exchange energy, and spin-orbit coupling on the conductance spectroscopy are discussed in detail. The conductance reveals a strong magnetoanisotropy with period $pi$ as the Andreev reflection coefficient. When the magnetization direction is parallel to the junction plane, a large conductance peak always emerges at the superconductor gap. This work offers a comprehensive and systematic study of the spin-triplet Andreev reflection, and has underlying application of $pi$-periodic spin valve in spintronics.
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