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Register a new userUPt$_3$ as a Topological Crystalline Superconductor
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We investigate the topological aspect of the spin-triplet $f$-wave superconductor UPt$_3$ through microscopic calculations of edge- and vortex-bound states based on the quasiclassical Eilenberger and Bogoliubov-de Gennes theories. It is shown that a gapless and linear dispersion exists at the edge of the $ab$-plane. This forms a Majorana valley, protected by the mirror chiral symmetry. We also demonstrate that, with increasing magnetic field, vortex-bound quasiparticles undergo a topological phase transition from topologically trivial states in the double-core vortex to zero-energy states in the normal-core vortex. As long as the $d$-vector is locked into the $ab$-plane, the mirror symmetry holds the Majorana property of the zero-energy states, and thus UPt$_3$ preserves topological crystalline superconductivity that is robust against the crystal field and spin-orbit interaction.
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Motivated by a recent angle-resolved thermal conductivity experiment that shows a twofold gap symmetry in the high-field and low-temperature C phase in the heavy-fermion superconductor UPt$_3$, we group-theoretically identify the pairing functions as $E_{1u}$ with the $f$-wave character for all the three phases. The pairing functions are consistent with the observation as well as with a variety of existing measurements. By using a microscopic quasi-classical Eilenberger equation with the identified triplet pairing function under applied fields, we performed detailed studies of the vortex structures for three phases, including the vortex lattice symmetry, the local density of states, and the internal field distribution. These quantities are directly measurable experimentally by SANS, STM/STS, and NMR, respectively. It is found that, in the B phase of low $H$ and low $T$, the double-core vortex is stabilized over a singular vortex. In the C phase, thermal conductivity data are analyzed to confirm the gap structure proposed. We also give detailed comparisons of various proposed pair functions, concluding that the present scenario of $E_{1u}$ with the $f$-wave, which is an analogue to the triplet planar state, is better than the $E_{2u}$ or $E_{1g}$ scenario. Finally, we discuss the surface topological aspects of Majorana modes associated with the $E_{1u}^f$ state of planar like features.
The field-orientation dependent thermal conductivity of the heavy-fermion superconductor UPt$_3$ was measured down to very low temperatures and under magnetic fields throughout three distinct superconducting phases: A, B, and C phases. In the C phase, a striking twofold oscillation of the thermal conductivity within the basal plane is resolved reflecting the superconducting gap structure with a line of node along the a axis. Moreover, we find an abrupt vanishing of the oscillation across a transition to the B phase, as a clear indication of a change of gap symmetries. We also identify extra two line nodes below and above the equator in both B and C phases. From these results together with the symmetry consideration, the gap function of UPt$_3$ is conclusively determined as a $E_{1u}$ representation characterized by a combination of two line nodes at the tropics and point nodes at the poles.
The symmetry properties of the order parameter characterize different phases of unconventional superconductors. In the case of the heavy-fermion superconductor UPt$_3$, a key question is whether its multiple superconducting phases preserve or break time-reversal symmetry (TRS). We tested for asymmetry in the phase shift between left and right circularly polarized light reflected from a single crystal of UPt$_3$ at normal incidence, finding that this so-called polar Kerr effect appears only below the lower of the two zero-field superconducting transition temperatures. Our results provide evidence for broken TRS in the low-temperature superconducting phase of UPt$_3$, implying a complex two-component order parameter for superconductivity in this system.
A well-established way to find novel Majorana particles in a solid-state system is to have superconductivity arising from the topological electronic structure. To this end, the heterostructure systems that consist of normal superconductor and topological material have been actively explored in the past decade. However, a search for the single material system that simultaneously exhibits intrinsic superconductivity and topological phase has been largely limited, although such a system is far more favorable especially for the quantum device applications. Here, we report the electronic structure study of a quasi-one-dimensional (q1D) superconductor TaSe$_3$. Our results of angle-resolved photoemission spectroscopy (ARPES) and first-principles calculation clearly show that TaSe$_3$ is a topological superconductor. The characteristic bulk inversion gap, in-gap state and its shape of non-Dirac dispersion concurrently point to the topologically nontrivial nature of this material. The further investigations of the Z$_2$ indices and the topologically distinctive surface band crossings disclose that it belongs to the weak topological insulator (WTI) class. Hereby, TaSe$_3$ becomes the first verified example of an intrinsic 1D topological superconductor. It hopefully provides a promising platform for future applications utilizing Majorana bound states localized at the end of 1D intrinsic topological superconductors.
Recent discovery of superconductivity in CeRh$_2$As$_2$ clarified an unusual $H$-$T$ phase diagram with two superconducting phases [Khim et al. arXiv:2101.09522]. The experimental observation has been interpreted based on the even-odd parity transition characteristic of locally noncentrosymmetric superconductors. Indeed, the inversion symmetry is locally broken at the Ce site, and CeRh$_2$As$_2$ molds a new class of exotic superconductors. The low-temperature and high-field superconducting phase is a candidate for the odd-parity pair-density-wave state, suggesting a possibility of topological superconductivity as spin-triplet superconductors are. In this paper, we first derive the formula expressing the $mathbb{Z}_2$ invariant of glide symmetric and time-reversal symmetry broken superconductors by the number of Fermi surfaces on a glide invariant line. Next, we conduct a first-principles calculation for the electronic structure of CeRh$_2$As$_2$. Combining the results, we show that the field-induced odd-parity superconducting phase of CeRh$_2$As$_2$ is a platform of topological crystalline superconductivity protected by the nonsymmorphic glide symmetry and accompanied by boundary Majorana fermions.
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