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Symmetric and asymmetric excitations of a strong-leg quantum spin ladder

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 Added by David Schmidiger
 Publication date 2013
  fields Physics
and research's language is English




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The zero-field excitation spectrum of the strong-leg spin ladder (C$_7$H$_10$N)$_2$CuBr$_4$ (DIMPY) is studied with a neutron time-of-flight technique. The spectrum is decomposed into its symmetric and asymmetric parts with respect to the rung momentum and compared with theoretical results obtained by the density matrix renormalization group method. Additionally, the calculated dynamical correlations are shown for a wide range of rung and leg coupling ratios in order to point out the evolution of arising excitations, as e.g. of the two-magnon bound state from the strong to the weak coupling limit.



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Inelastic neutron scattering is used to measure the spin excitation spectrum of the Heisenberg $S=1/2$ ladder material (C$_7$H$_10$N)$_2$CuBr$_4$ in its entirety, both in the gapped spin-liquid and the magnetic field induced Tomonaga-Luttinger spin liquid regimes. A fundamental change of the spin dynamics is observed between these two regimes. DMRG calculations quantitatively reproduce and help understand the observed commensurate and incommensurate excitations. The results validate long-standing quantum field theoretical predictions, but also test the limits of that approach.
The strong-leg S=1/2 Heisenberg spin ladder system (C7H10N)2CuBr4 is investigated using Density Matrix Renormalization Group (DMRG) calculations, inelastic neutron scattering, and bulk magneto-thermodynamic measurements. Measurements showed qualitative differences compared to the strong-rung case. A long-lived two-triplon bound state is confirmed to persist across most of the Brillouin zone in zero field. In applied fields, in the Tomonaga-Luttinger spin liquid phase, elementary excitations are attractive, rather than repulsive. In the presence of weak inter-ladder interactions, the strong-leg system is considerably more prone to 3-dimensional ordering.
Topological order, the hallmark of fractional quantum Hall states, is primarily defined in terms of ground-state degeneracy on higher-genus manifolds, e.g. the torus. We investigate analytically and numerically the smooth crossover between this topological regime and the Tao-Thouless thin torus quasi-1D limit. Using the wire-construction approach, we analyze an emergent charge density wave (CDW) signifying the break-down of topological order, and relate its phase shifts to Wilson loop operators. The CDW amplitude decreases exponentially with the torus circumference once it exceeds the transverse correlation length controllable by the inter-wire coupling. By means of numerical simulations based on the matrix product states (MPS) formalism, we explore the extreme quasi-1D limit in a two-leg flux ladder and present a simple recipe for probing fractional charge excitations in the $ u=1/2$ Laughlin-like state of hard-core bosons. We discuss the possibility of realizing this construction in cold-atom experiments. We also address the implications of our findings to the possibility of producing non-Abelian zero modes. As known from rigorous no-go theorems, topological protection for exotic zero modes such as parafermions cannot exist in 1D fermionic systems and the associated degeneracy cannot be robust. Our theory of the 1D-2D crossover allows to calculate the splitting of the degeneracy, which vanishes exponentially with the number of wires, similarly to the CDW amplitude.
We have studied electron spin resonance (ESR) absorption spectra for the nonmagnetically diluted strong-leg spin ladder magnet ({C}$_{7}$H$_{10}$N)$_{2}$Cu$_{(1-x)}$Zn$_{x}$Br$_{4}$ (abbreviated as DIMPY) down to 450 mK. Formation of the clusters with non-zero net magnetization is confirmed; the cluster-cluster interaction is evidenced by the concentration dependence of ESR absorption. High-temperature spin-relaxation time was found to increase with non-magnetic dilution. The ESR linewidth analysis proves that the Dzyaloshinskii-Moriya (DM) interaction remains the dominant spin-relaxation channel in diluted DIMPY. Experimental data indicate that the dilution results in the weakening of the effective DM interaction, which can be interpreted as total suppression of DM interaction in the close vicinity of impurity atom.
We report on zero-field muon spin rotation, electron spin resonance and polarized Raman scattering measurements of the coupled quantum spin ladder Ba2CuTeO6. Zero-field muon spin rotation and electron spin resonance probes disclose a successive crossover from a paramagnetic through a spin-liquid-like into a magnetically ordered state with decreasing temperature. More significantly, the two-magnon Raman response obeys a T-linear scaling relation in its peak energy, linewidth and intensity. This critical scaling behavior presents an experimental signature of proximity to a quantum critical point from an ordered side in Ba2CuTeO6.
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