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Register a new userPlasmon anomaly in the dynamical optical conductivity of graphene
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Added by
Kostyantyn Kechedzhi
Publication date
2013
fields
Physics
and research's language is
English
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We theoretically consider the effect of plasmon collective modes on the frequency-dependent conductivity of graphene in the presence of the random static potential of charged impurities. We develop an equation of motion approach suitable for the relativistic Dirac electrons in graphene that allows analytical high-frequency asymptotic solution in the presence of both disorder and interaction. We show that the presence of the acoustic plasmon pole (i.e. the plasmon frequency vanishing at long wavelengths as the square-root of wavevector) in the inverse dynamical dielectric function of graphene gives rise to a strong variation with frequency of the screening effect of the relativistic electron gas in graphene on the potential of charged impurities. The resulting frequency-dependent impurity scattering rate gives rise to a broad peak in the frequency-dependent graphene optical conductivity with the amplitude and the position of the peak being sensitive to the detailed characteristics of disorder and interaction in the system. This sample (i.e. disorder, elecron density and interaction strength) dependent redistribution of the spectral weight in the frequency-dependent graphene conductivity may have already been experimentally observed in optical measurements.
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The effect of electron-electron interaction on the low-temperature conductivity of graphene is investigated experimentally. Unlike in other two-dimensional systems, the electron-electron interaction correction in graphene is sensitive to the details of disorder. A new temperature regime of the interaction correction is observed where quantum interference is suppressed by intra-valley scattering. We determine the value of the interaction parameter, F_0 ~ -0.1, and show that its small value is due to the chiral nature of interacting electrons.
Using terahertz time-domain spectroscopy, the real part of optical conductivity [$sigma_{1}(omega)$] of twisted bilayer graphene was obtained at different temperatures (10 -- 300 K) in the frequency range 0.3 -- 3 THz. On top of a Drude-like response, we see a strong peak in $sigma_{1} (omega)$ at $sim$2.7 THz. We analyze the overall Drude-like response using a disorder-dependent (unitary scattering) model, then attribute the peak at 2.7 THz to an enhanced density of states at that energy, that is caused by the presence of a van Hove singularity arising from a commensurate twisting of the two graphene layers.
The optical properties of (001)-oriented NbP single crystals have been studied in a wide spectral range from 6 meV to 3 eV from room temperature down to 10 K. The itinerant carriers lead to a Drude-like contribution to the optical response; we can further identify two pronounced phonon modes and interband transitions starting already at rather low frequencies. By comparing our experimental findings to the calculated interband optical conductivity, we can assign the features observed in the measured conductivity to certain interband transitions. In particular, we find that transitions between the electronic bands spilt by spin-orbit coupling dominate the interband conductivity of NbP below 100 meV. At low temperatures, the momentum-relaxing scattering rate of the itinerant carriers in NbP is very small, leading to macroscopic characteristic length scales of the momentum relaxation of approximately 0.5 $mu$m.
Assuming diffusive carrier transport and employing an effective medium theory, we calculate the temperature dependence of bilayer graphene conductivity due to Fermi-surface broadening as a function of carrier density. We find that the temperature dependence of the conductivity depends strongly on the amount of disorder. In the regime relevant to most experiments, the conductivity is a function of T/T*, where T* is the characteristic temperature set by disorder. We demonstrate that experimental data taken from various groups collapse onto a theoretically predicted scaling function.
It is a fact that the minimal conductivity $sigma_0$ of most graphene samples is larger than the well-established universal value for ideal graphene $4e^2/pi h$; in particular, larger by a factor $gtrsimpi$. Despite intense theoretical activity, this fundamental issue has eluded an explanation so far. Here we present fully atomistic quantum mechanical estimates of the graphene minimal conductivity where electron-electron interactions are considered in the framework of density functional theory. We show the first conclusive evidence of the dominant role on the minimal conductivity of charged impurities over ripples, which have no visible effect. Furthermore, in combination with the logarithmic scaling law for diffusive metallic graphene, we ellucidate the origin of the ubiquitously observed minimal conductivity in the range $8e^2/h > sigma_0 gtrsim 4e^2/h$.
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