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Suppression of Spin-Exchange Relaxation Using Pulsed Parametric Resonance

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 Added by Thad Walker
 Publication date 2013
  fields Physics
and research's language is English




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We demonstrate that spin-exchange dephasing of Larmor precession at near-earth-scale fields is effectively eliminated by dressing the alkali-metal atom spins in a sequence of AC-coupled 2-pi pulses, repeated at the Larmor precession frequency. The contribution of spin-exchange collisions to the spectroscopic line width is reduced by a factor of the duty cycle of the pulses. We experimentally demonstrate resonant transverse pumping in magnetic fields as high as 0.1 Gauss, present experimental measurements of the suppressed spin-exchange relaxation, and show enhanced magnetometer response relative to a light-narrowed scalar magnetometer.



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We present calculations of spin-relaxation rates of alkali-metal atoms due to the spin-axis interaction acting in binary collisions between the atoms. We show that for the high-temperature conditions of interest here, the spin relaxation rates calculated with classical-path trajectories are nearly the same as those calculated with the distorted-wave Born approximation. We compare these calculations to recent experiments that used magnetic decoupling to isolate spin relaxation due to binary collisions from that due to the formation of triplet van-der-Waals molecules. The values of the spin-axis coupling coefficients deduced from measurements of binary collision rates are consistent with those deduced from molecular decoupling experiments. All the experimental data is consistent with a simple and physically plausible scaling law for the spin-axis coupling coefficients.
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We demonstrate a substantial improvement in the spin-exchange gate using symmetric control instead of conventional detuning in GaAs spin qubits, up to a factor-of-six increase in the quality factor of the gate. For symmetric operation, nanosecond voltage pulses are applied to the barrier that controls the interdot potential between quantum dots, modulating the exchange interaction while maintaining symmetry between the dots. Excellent agreement is found with a model that separately includes electrical and nuclear noise sources for both detuning and symmetric gating schemes. Unlike exchange control via detuning, the decoherence of symmetric exchange rotations is dominated by rotation-axis fluctuations due to nuclear field noise rather than direct exchange noise.
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