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Register a new userMeasuring central-spin interaction with a spin bath by pulsed ENDOR: Towards suppression of spin diffusion decoherence
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We present pulsed electron-nuclear double resonance (ENDOR) experiments which enable us to characterize the coupling between bismuth donor spin qubits in Si and the surrounding spin bath of 29Si impurities which provides the dominant decoherence mechanism (nuclear spin diffusion) at low temperatures (< 16 K). Decoupling from the spin bath is predicted and cluster correlation expansion simulations show near-complete suppression of spin diffusion, at optimal working points. The suppression takes the form of sharply peaked divergences of the spin diffusion coherence time, in contrast with previously identified broader regions of insensitivity to classical fluctuations. ENDOR data suggest that anisotropic contributions are comparatively weak, so the form of the divergences is largely independent of crystal orientation.
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A major problem facing the realisation of scalable solid-state quantum computing is that of overcoming decoherence - the process whereby phase information encoded in a qubit is lost as the qubit interacts with its environment. Due to the vast number of environmental degrees of freedom, it is challenging to accurately calculate decoherence times $T_2$, especially when the qubit and environment are highly correlated. Hybrid or mixed electron-nuclear spin qubits, such as donors in silicon, possess optimal working points (OWPs) which are sweet-spots for reduced decoherence in magnetic fields. Analysis of sharp variations of $T_2$ near OWPs was previously based on insensitivity to classical noise, even though hybrid qubits are situated in highly correlated quantum environments, such as the nuclear spin bath of $^{29}$Si impurities. This presented limited understanding of the decoherence mechanism and gave unreliable predictions for $T_2$. I present quantum many-body calculations of the qubit-bath dynamics, which (i) yield $T_2$ for hybrid qubits in excellent agreement with experiments in multiple regimes, (ii) elucidate the many-body nature of the nuclear spin bath and (iii) expose significant differences between quantum-bath and classical-field decoherence. To achieve these, the cluster correlation expansion was adapted to include electron-nuclear state mixing. In addition, an analysis supported by experiment was carried out to characterise the nuclear spin bath for a bismuth donor as the hybrid qubit, a simple analytical formula for $T_2$ was derived with predictions in agreement with experiment, and the established method of dynamical decoupling was combined with operating near OWPs in order to maximise $T_2$. Finally, the decoherence of a $^{29}$Si spin in proximity to the hybrid qubit was studied, in order to establish the feasibility for its use as a quantum register.
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An exact reduced dynamical map along with its operator sum representation is derived for a central spin interacting with a thermal spin environment. The dynamics of the central spin shows high sustainability of quantum traits such as coherence and entanglement in the low-temperature regime. However, for sufficiently high temperature and when the number of bath particles approaches the thermodynamic limit, this feature vanishes and the dynamics closely mimics Markovian evolution. The properties of the long-time-averaged state and the trapped information of the initial state for the central qubit are also investigated in detail, confirming that the nonergodicity of the dynamics can be attributed to the finite temperature and finite size of the bath. It is shown that if a certain stringent resonance condition is satisfied, the long-time-averaged state retains quantum coherence, which can have far reaching technological implications in engineering quantum devices. An exact time-local master equation of the canonical form is derived. With the help of this master equation, the nonequilibrium properties of the central spin system are studied by investigating the detailed balance condition and irreversible entropy production rate. The result reveals that the central qubit thermalizes only in the limit of very high temperature and large number of bath spins.
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