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Register a new userObservation of inhibited electron-ion coupling in strongly heated graphite
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Creating non-equilibrium states of matter with highly unequal electron and lattice temperatures allows unsurpassed insight into the dynamic coupling between electrons and ions through time-resolved energy relaxation measurements. Recent studies on low-temperature laser-heated graphite suggest a complex energy exchange when compared to other materials. To avoid problems related to surface preparation, crystal quality and poor understanding of the energy deposition and transport mechanisms, we apply a different energy deposition mechanism, via laser-accelerated protons, to isochorically and non-radiatively heat macroscopic graphite samples up to temperatures close to the melting threshold. Using time-resolved x ray diffraction, we show clear evidence of a very small electron-ion energy transfer, yielding approximately three times longer relaxation times than previously reported. This is indicative of the existence of an energy transfer bottleneck in non-equilibrium warm dense matter.
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Ultracold plasmas (UCP) provide a well-controlled system for studying multiple aspects in plasma physics that include collisions and strong coupling effects. By applying a short electric field pulse to a UCP, a plasma electron center-of-mass (CM) oscillation can be initiated. In accessible parameter ranges, the damping rate of this oscillation is determined by the electron-ion collision rate. We performed measurements of the oscillation damping rate with such parameters and compared the measured rates to both a molecular dynamic (MD) simulation that includes strong coupling effects and to Monte-Carlo collisional operator simulation designed to predict the damping rate including only weak coupling considerations. We found agreement between experimentally measured damping rate and the MD result. This agreement did require including the influence of a previously unreported UCP heating mechanism whereby the presence of a DC electric field during ionization increased the electron temperature, but estimations and simulations indicate that such a heating mechanism should be present for our parameters. The measured damping rate at our coldest electron temperature conditions was much faster than the weak coupling prediction obtained from the Monte-Carlo operator simulation, which indicates the presence of significant strong coupling influence. The density averaged electron strong coupling parameter $Gamma$ measured at our coldest electron temperature conditions was 0.35.
Motivated by the recent discovery of superconductivity in Ca- and Yb-intercalated graphite (CaC$_{6}$ and YbC$_{6}$) and from the ongoing debate on the nature and role of the interlayer state in this class of compounds, in this work we critically study the electron-phonon properties of a simple model based on primitive graphite. We show that this model captures an essential feature of the electron-phonon properties of the Graphite Intercalation Compounds (GICs), namely, the existence of a strong dormant electron-phonon interaction between interlayer and $pi ^{ast}$ electrons, for which we provide a simple geometrical explanation in terms of NMTO Wannier-like functions. Our findings correct the oversimplified view that nearly-free-electron states cannot interact with the surrounding lattice, and explain the empirical correlation between the filling of the interlayer band and the occurrence of superconductivity in Graphite-Intercalation Compounds.
The friction force on a test particle traveling through a plasma that is both strongly coupled and strongly magnetized is studied using molecular dynamics simulations. In addition to the usual stopping power component aligned antiparallel to the velocity, a transverse component that is perpendicular to both the velocity and Lorentz force is observed. This component, which was recently discovered in weakly coupled plasmas, is found to increase in both absolute and relative magnitude in the strongly coupled regime. Strong coupling is also observed to induce a third component of the friction force in the direction of the Lorentz force. These first-principles simulations reveal novel physics associated with collisions in strongly coupled, strongly magnetized, plasmas that are not predicted by existing kinetic theories. The effect is expected to influence macroscopic transport in a number of laboratory experiments and astrophysical plasmas.
Electron dynamics in Electron Cyclotron Resonance Ion Source is numerically simulated by using Particle-In-Cell code combined with simulations of the ion dynamics. Mean electron energies are found to be around 70 keV close to values that are derived from spectra of X-ray emission out of the source. Electron life time is defined by losses of low-energy electrons created in ionizing collisions; the losses are regulated by electron heating rate, which depends on magnitude of the microwave electric field. Changes in ion confinement with variations in the microwave electric field and gas flow are simulated. Influence of electron dynamics on the afterglow and two-frequency heating effects is discussed.
The full three dimensional dispersion of the pi-bands, Fermi velocities and effective masses are measured with angle resolved photoemission spectroscopy and compared to first-principles calculations. The band structure by density-functional theory strongly underestimates the slope of the bands and the trigonal warping effect. Including electron-electron calculation on the level of the GW approximation, however, yields remarkable agreement in the vicinity of the Fermi level. This demonstrates the breakdown of the independent electron picture in semi-metallic graphite and points towards a pronounced role of electron correlation for the interpretation of transport experiments and double-resonant Raman scattering for a wide range of carbon based materials.
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