No Arabic abstract
Gauge invariance was discovered in the development of classical electromagnetism and was required when the latter was formulated in terms of the scalar and vector potentials. It is now considered to be a fundamental principle of nature, stating that different forms of these potentials yield the same physical description: they describe the same electromagnetic field as long as they are related to each other by gauge transformations. Gauge invariance can also be included into the quantum description of matter interacting with an electromagnetic field by assuming that the wave function transforms under a given local unitary transformation. The result of this procedure is a quantum theory describing the coupling of electrons, nuclei and photons. Therefore, it is a very important concept: it is used in almost every fields of physics and it has been generalized to describe electroweak and strong interactions in the standard model of particles. A review of quantum mechanical gauge invariance and general unitary transformations is presented for atoms and molecules in interaction with intense short laser pulses, spanning the perturbative to highly nonlinear nonperturbative interaction regimes. Various unitary transformations for single spinless particle Time Dependent Schrodinger Equations, TDSE, are shown to correspond to different time-dependent Hamiltonians and wave functions. Accuracy of approximation methods involved in solutions of TDSEs such as perturbation theory and popular numerical methods depend on gauge or representation choices which can be more convenient due to faster convergence criteria. We focus on three main representations: length and velocity gauges, in addition to the acceleration form which is not a gauge, to describe perturbative and nonperturbative radiative interactions. Numerical schemes for solving TDSEs in different representations are also discussed.
We revisit the stabilization of ionization of atoms subjected to a superintense laser pulse using nonlinear dynamics. We provide an explanation for the lack of complete ionization at high intensity and for the decrease of the ionization probability as intensity is increased. We investigate the role of each part of the laser pulse (ramp-up, plateau, ramp-down) in this process. We emphasize the role of the choice for the ionization criterion, energy versus distance criterion.
The quasistatic limit of the velocity-gauge strong-field approximation describing the ionization rate of atomic or molecular systems exposed to linear polarized laser fields is derived. It is shown that in the low-frequency limit the ionization rate is proportional to the laser frequency, if a Coulombic long-range interaction is present. An expression for the corresponding proportionality coefficient is given. Since neither the saddle-point approximation nor the one of a small kinetic momentum is used in the derivation, the obtained expression represents the exact asymptotic limit. This result is used to propose a Coulomb correction factor. Finally, the applicability of the found asymptotic expression for non-vanishing laser frequencies is investigated.
We show that the dipole-dipole interaction between two Rydberg atoms can lead to substantial Abelian and non-Abelian gauge fields acting on the relative motion of the two atoms. We demonstrate how the gauge fields can be evaluated by numerical techniques. In the case of adiabatic motion in a single internal state, we show that the gauge fields give rise to a magnetic field that results in a Zeeman splitting of the rotational states. In particular, the ground state of a molecular potential well is given by the first excited rotational state. We find that our system realises a synthetic spin-orbit coupling where the relative atomic motion couples to two internal two-atom states. The associated gauge fields are non-Abelian.
In this work we show how constructing Wigner functions of heterogeneous quantum systems leads to new capability in the visualization of quantum states of atoms and molecules. This method allows us to display quantum correlations (entanglement) between spin and spatial degrees of freedom (spin-orbit coupling) and between spin degrees of freedom, as well as more complex combinations of spin and spatial entanglement for the first time. This is important as there is growing recognition that such properties affect the physical characteristics, and chemistry, of atoms and molecules. Our visualizations are sufficiently accessible that, with some preparation, those with a non-technical background can gain an appreciation of subtle quantum properties of atomic and other systems. By providing new insights and modelling capability, our phase-space representation will be of great utility in understanding aspects of atomic physics and chemistry not available with current techniques.
Radiative polarization of electrons and positrons through the Sokolov-Ternov effect is important for applications in high-energy physics. Radiative spin-polarization is a manifestation of quantum radiation reaction affecting the spin-dynamics of electrons. We recently proposed that an analogue of the Sokolov-Ternov effect could occur in the strong electromagnetic fields of ultra-high-intensity lasers, which would result in a build-up of spin-polarization in femtoseconds. In this paper we develop a density matrix formalism for describing beam polarization in strong electromagnetic fields. We start by using the density matrix formalism to study spin-flips in non-linear Compton scattering and its dependence on the initial polarization state of the electrons. Numerical calculations show a radial polarization of the scattered electron beam in a circularly polarized laser, and we find azimuthal asymmetries in the polarization patterns for ultra-short laser pulses. A degree of polarization approaching 9 % is achieved after emitting just a single photon. We develop the theory by deriving a local constant crossed field approximation (LCFA) for the polarization density matrix, which is a generalization of the well known LCFA scattering rates. We find spin-dependent expressions that may be included in electromagnetic charged-particle simulation codes, such as particle-in-cell plasma simulation codes, using Monte-Carlo modules. In particular, these expressions include the spin-flip rates for arbitrary initial polarization of the electrons. The validity of the LCFA is confirmed by explicit comparison with an exact QED calculation of electron polarization in an ultrashort laser pulse.